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T i . -..-...- .. - Y . ...compe · . I As : • 650 [129 SG i . 125 1.4 LE i ki . C AC MICROCOPY RESOLUTION TEST CHART NATIONAL BUREAU OF STANDARUS -1963 -, ------- 16.1 - -- SEP 27 ORNL-Q. 2355 CONf 660336-1 CFSTI PRICES · MA3.00 ; WN.65 OSNL CLADDING AND DISPERSION FUEL DEVELOPMETT AT CRNL * J. E. Cunningham and J. W. Ullmann Oak Ridge National Laboratory Oak Ridge, Tennessee ciniai mieste santi e memorie meski atas believe in the content RELEASED FOR ANNOUNCEMENT IN NUCLEAR SCIENCE ABSTRACTS con LEGAL NOTICE . ..- - This report was prepared as an account of Government sponsored work. Neither the United States, nor the Commission, nor any person acung on behalf of the Commission: A. Makes any warranty or representation, expressed or implied, with respect to the accu- racy, completeness, or usefulness of the information contained in this report, or that the use of any information, apparatus, method, or process disclosed in this report may not Infringe privately owned rigbls; or B. Assumes any liabilities with respect to the use of, or for damages ieswing from the use of any information, apparatus, method, or process disclosed in this report. As used in the above, "person acting on bebalf of the Commission" includ:8 any em- ployce or contractor of the Commission, or employee of such contractor, to the extent that such employee or contractor of the Commission, or employee of such contractor prepares, disseminates, or provides access to, any information pursuant to his employment or contract with the Commission, or his employment on to such contractor. entiislamatwa na * Research sponsored by the U.S. Atomic Energy Commission under contract with the Union Carbide Corporation. d i si . - ORNL-AEC - OFFICIAL , INTRODUCTION .... The presentation from Oak Ridge National Laboratory will be given in three parts. The subject and speaker for each part is as follows: 1) Dispersion Fuel Technology by J. E. Cunningham, 2) Fuel Reprocessing by J. W. Ullmann, and 3) Fuel Cycle Economics and Radiation Effects in Cladding Materials by D. A. Douglas. · ORNS - AEC - OFFICIAL - -- 002-Stainless Steel Cermet Fuel Experience at ORNL - J. E. Cunningham miccamento consistence in umiwa na miaka minis na haitatis. ln elle In reviewing the technology of the UO - tainless steel dispersion fuel, I shall cor.fine my remarks mainly to irradiation experience accumulated over the past 15 years and attempt to point up shortcomings of this iuel type for application in FFTF. As most of you know, the stainless steal-uranium dioxide dispersion fuel technology for the Army Water Reactor Program was developed in the early 1950's. The product that evolved for startup of the SM-1 reactor at Fort Belvoir, Virginia, was a brazed assembly of chin' plates. A representative cross section of such a composite fuel plete is shown in Fig. 1 (LS-4278, Y-25961) for reference. It consists mainly of a 20-mil-thick fuel-bearing section with 5-mil cladding of type 304L stainless steel on each face to give an overall plate thickness of 30 mils. The fuel is incorporated into the fuel-bearing section in the form of 26 wt% or 19 vol % UO2. The matrix material is type 302B stainless steel ponder, which contains 2.5 wt % silicon. r minimalna kiselina imani nim AT These composite fuel plates were prepared by the conventional roll-bonding technique. Most of the fragmentation and stringering of the oxide that is apparent in Fig. 1 occurred during cold rolling (25% reduction) to final thickness. These composite fuel plates of 1950 design performed quite well in the 10-Mw thermal reactor at Fort Belvoir; in fact, they accummulated a total power output of over 60,000 Mwd (10% greater than the expected design 11fetime of 15 Mwyr) before discharge at burnout. The operating conditions were not very severe. At a power level of 10 MW, for instance, the heat flux .. - ... --' . :* ' - . . E .ORNLAEC - OFFICIAL ORNL - AEC - OFFICIAL TEL ... .. ...--.---... . ... .. . A . . . . . . .... . . . . was only 55,000 Btu nr-lt. The average surface temporature was 450°F, while the maximum centerline temperature of the fuel was 6500F. The elements were subjected to over 3000 thermal cyclay during startup and shutdown of the reactor, because the reactor was used primarily as an operator-training facility. The initial core loading accummulated a total reactivity lifetime of 16.4 Mwyr. batore discharge. The average fuoi burnup in terms of depletion of 2300 atoms was 26% or 1 x 1021 fissions/cc. The effect of irradiation on dimensional stability and structural integrity was checked by hot-cell examination of stationary fuel elements that had been removed after various levels of exposure in the roactor. The first fuel component was removed after 10.3 mwyr life, the second at the end of the core life or 16.5 Mwyr, and the third after 19.5 Mwyr (higher exposure was achieved by reinsertion in Core II). In-cell examination revealed the following: . . 1) progressively greater tendency toward plate rippling with increasing exposure. Maximum ripple amplitudes of 23, 33, and 45 mils were observed, respectively, for 10.5, 16.5, and 19.5 Mwyr exposures. 2) A maximum plate increase in thickness of 3 mils or 10% occurred at the axial peak furnup position in the fuel element with the greatest neutron exposure. The burnup at this location was 62% depletion of 2350 atoms or 2.2 x 1021 flasions/cc. 3) The frequency of intergranular cracks in the cladding varied directly with burnup. In a few instances, cracking was so severe that whole grains were removed at the cladding surface.. Some transgranular cracking was noted in the grain structure of the low-cobalt low-carbon stainless steel cladding in the high burnup fuel element. · QUNI - AEC - OFFICIAL No evidence was found of matrix cracking nor sign of gross deterioration in these dispersion fuel plates. Yet, swelling of the order of 10% did occur under the modest operating conditions prevailing in the SM-1 reactor, and such behavior must be factored into the design of the FFTF if the dis- persion 18 used for the driver fuel. W171130 - 13V – 1N1O . In 1962, we examined 34 disparsion fuel specimens contained in six Nak- filled capsules that had been irradiated to relatively high burnup in the ETR. These irradiation tests were initiated by BMI to evaluate various parameters in connection with their program to develop an improved dis- pers:on fuel for service in the Army SM-2 reactor. The cermet specimens were clad with type 347 stainless steel and contained either to or UN dispersed in type 347 stainless steel along with small but varying amounts of burnable pois01, in the form of B,C, NbB2, and ZrBz. In addition, the behavior of fused and hydrothermal oxides was compared. The highly en- richeu fuel was incorporated in the fuel-bearing section to a nominal composition of 26 and 38 wt% UO2 or 34 wt % UN. of the 34 specimens examined, 11 showed failure. These specimens varied in degree of failure from surface blistering to complete disintegration, as shown in Fig. 2 (LS-13896, R-9043, R-3045). The six specimens with the high' fuel loading operated at a surface temperature of 950°F, and all six failed. Four of these were badly swollen and the other two completely disintegrated. of the remaining five failed specimens, which contained 24 or 25 wt% UO,, three were severely damaged and one developed a large blister over the fuel region. The micrograph in Fig. 3 (LS-8870, R-11235) shows the degree of swelling noted ac the edge of a specimen loaded with 26 wt% UC12 and exposed to a. fuel depletion of 74% of the 2350 atoms (2.9 x 1021 8188ions/ce) at 10000F. Matrix cracking was observed toward the center of this specimen. A typical picture of severe cracking is shown in Fig. 4 (L8-13897, R-11229). This particular specimen contained 34 wt % UN, oporated at a peak temperature of 950°F, and achieved 63 at. % burnup. ORNL - AEC - OFFICIAL OONI - AC - OFFICIAL W121110 - DIV-INIO . Metallographic examination of the 23 undamaged specimens revealed no evidence of matrix cracking or blistering. These specimens all contained 24.2 or 26 wt % 102, operated in the temperature region of 420 to 600°F, and achieved burnups of 52 to 67% of the 2350 atoms (1.9 to 2.6 x 1021 fissions/cc). No significant difference was noted between specimens prepared with spherical (fuwed) or irregular-shapod (hyurothermal) vog partioles nor botwoon specimons containing burnablo poison of different chemical form. The microstructure 11lustrated in Fig. 5 (18-9601, R-11306) 18 typica), for these specimens and is quite similar in appearance to that found in the high burnup region of the SM-1 fuel elements. From mid-1959 to 1962, we worked on a cooperative program with APDA to develop an improved Vorstainless steel fuol dispersion for use in Core B of the Fermi Reactor. The scope of the program embodied 1) characterization of spheroidal UO2 particles, 2) fabrication of composite plates, 3) feasibility studies on nondestructive testing, 4) establishment oi suitable assembly procedures, 5) measurement of fuel material mechanical properties, and 6) irradiation testing. Early in the development program, the concentration of fuel was limited to 27.5 vol % (34.5 wt%) VO2 in order to enhance radiation performance. Spheroidal fuel particles is the 105 to 149-size range were chosen, because we felt that this shape would minimize stress concentration and reduce radiation damage in the fuel matrix. Type 347 stainless steel was selected as the structural material because of its superior strength compared to other conventional grades of austenitic steels in the 800 to 1000°F temp. erature range. The effect of cold deformation on the integrity and shape of the oxide in the finished plate was investigated and the results are summarized in Fig. 6 (LS-7260, Photo 52670). Cracking of the oxide was noted at all reductions investigated and stringering became pronounced at 20 to 30% reduction in thickness; hence, we decided to hot toll the fuel plates to finish size to minimize oxide fragmentation and stringering. During plate development, ORNI - AEC - OFFICIAL OINL - AEC - We also noticed a wide variation in the behavior during hot working of spheroldal 1o, particles procured from different vendors, as illustrated in Fig. 7 (18-7021, Y-38004, Y-38989). Our characterization studies showed that we nended some means to separate good from bad quai- ity starting powder; hence, a new techãique based on solid embedment and density was dovolopod to serve this purpose. A spooilication was also written that allowed us to procure good quality spheroidal particles with a high degree of confidence. ORNL - A1C - OMFICIAL Three instrumented capsules were irradiated in the MTR to assess the in- reactor performance of the Fermi Core 8 fuel plate. Each capsule contained two miniature plates, 2 x 0.6 x 0.116 in. The fuel-bearing section con- tained 33 wt % spheroidal 10% af 105- to 1490 lı particle size, homogen- eously dispersed in type 347 stainless steel as shown in Fig. 8 (18-6980, Y-35413). Two thermocouples were attached to each specimen. The nominal irradiation condition selected for in-reactor testing were three different burnup levels - 10, 20, and 25% of the 2350 atoms - and a surface temperatura of 925 to 950°7. These conditions were chosen on the basis that Core B would be used to operate the Fermi reactor at a maximum core thermal power of 270 MW. At this level, the calculated throughput burnup would be 20.7% of the initial 2350 a tons; hence, our burnup targets bracketed this level. Nominal fuel temperatures at the reactor center would be 750°F at the plate surface and 970°F at the fuel centerline. Hot spot and hot channel factors increased the centerline temperature to a maximum of about 1040°F. . .- - - - - - - -- - The first capsule was discharged after an estimated burnup of 9.5% of the 2350 atoms. Subsequent measurement revealod, however, that the actual fl8sion burnup was only 6.3% (average of two samples.) Conse- quen'ily, an experience factor of 6.3/9.5 or 0.66 was applied in fixing the discharge dates for the remaining capsules. On this basis, the other two capsules were discharged after an estimated fuel depletion of ORNL - AEC - OFFICIAL ORNL - AEC - OFFICIAL - - . -. 16 and 26% of the 2350 atoms. JINI - AC - OFFICIAL Specimene 1 and 10, which were contained in capsule ORNL-MTR-64-4 were unaffected by the irradiation. The burnup of 235U atoms was 6.3%. The general appearance of spocimen 10 18 shown in Fig. 9 (LS-8898, R-4349). All icur thermocouplo, romainod operational throughout tho tont and in- d'icated that the surface temperature on those specimens ranged from 800 to 950°F. The appearance of the microstructure was as expected. Specimen 6 from ORNL-NTR-46-2 showed severe damage, as illustrated in Fig. 10 (LS-8902, R-11567). Twr, full-penetration holes were noted in the test plate. A major crack also developed at one edge of the specimen, as shown in Fig. 11 (LS-13898, R-11569). Marked swelling was noted in specimen 5 located at the bottom of the capsule. The appearance of specimen 5 in transverse section 18 depicted in Fig. 12 (18-13899, R-13091). Gross swelling (ale -13%) and matrix cracking are apparent. In this specimen the surface temperature ranged between 850 and 1150°F throughout the life of test and the measured vurnup was 29% of the su atoms. Specimens 8 and 9 in the remaining capsule showed obvious swelling after a burnup of 33% of the 2350 atoms. This behavior 18 illustrated in Fig. 13 (LS-13903, B-14325) which shows specimen 9 in transverse section. Specimen 9 increased 6% in volwe. A longitudinal section of specimen 8, which increased 27% in thickness is shown in Fig. 14 (LS-13901, R-14261). Temperature ranged from 950 to 1050°F during test; the average temperature was 1000°F. These irradiation test results indicate that the temperature-burnup limitation of the improved stainless steel-U02 cermet fuel for Fermi Core B was definitely exceeded. Moreover, it should be noted that the specimen size was relatively small, 80 one would expect better performance due to the restraint offered by the cladding and frame material. In addition, control of particle shape and distribution of fuel appeared to offer only marginal improvement in performance. Tissu-doi-indu · OANL - AEC - OFFICIAL During the development of the Fermi Core B fuel element, several advances were made in the developrent of nondestructive testing techniques to ensure compliance with specifications and as-manufactured product reliability. Among the developments were ONNI AEC - OFFICIAL 1) an ultransonso toonnique that is capable of detecting core-cladding interface nonbond areas 1/8 in. diameter or larger, 2) an eddy-current technique capable of measuring the fuel plate thickness to within an accuracy of * I mil, . 3) a radiographic technique to detect UO2 concentration in- homogeneities in excess of the specified = 5% tolerance, 4) a spacing measuring device, based on recently improved eddy-current theory, that moasures coplant-channel gaps between plates to + 0.5' mil, and methods for characterization of UO, powder so that par- ticles of the desired shape and integrity can be pro- oured from the vendors with a high degree of confidence that the material is of high quality. An analysis of pertinent irradiation data on the performance of 10,-stainless . steel dispersions has been compiled at ORNL. These data are plotted in Fig. 15 (ORNL-LR-DWG-75068R3). It should be noted, however, that the temp- erature points plotted in this figure are based on estimated values since only limited data are available on actual surface temperature measurements during irradiation. The curve indicates that to achieve a burnup of 2 x 10% fissions/oc the maximum surface temperature of the fuel should be less than 800°F. At a surface temperature of 1200°F, the maximum burnup that can be achieved bolore uncontrolled swelling occurs 18 about 0.8 x 1024 1188ions/cc. 1 ORRI - AEC - OFFICIAL DRNI ~ AEC - OFFICIAL -..-. - XML Ideally, a dispersion fuel should consist of components that are in equi- librium with one another as well as with their environment at all times. Chemical stability of the components, for instance, must be maintained in fabrication and during the lifetime of the fuel in the reactor. Plutonia and urania exhibit notable differences with rogard to phase stability. Uranium dioxide is the oxide of lowest oxide content in the uranium-oxygen system whereas PuO2 is the highest oxide in the plutonium-oxygen system. Silicon, a tramp constituent in stainless steel, will reduce Puoz. Finally, I would like to state that in my considered opinion, the Puog- stainless steel dispersion fuel is a questionable fuel concept for FFTF operation at 1200°F. At best its development to provide adequate service will be an expensive and uncertain proposition. Radiation-induced swelling of Puo, and severe thermal stress under condition of high power density are likely to lead to premature failure of the potentially em- brittled stainless steel matrix and cladding. It is true that certain measures can be taken to improve performance at 1200°F, such as built-in void space to accommodate fission gas and reduce swelling. Unfortunately, no one has come up with a practical way of achieving this objective despite the fact that its effect on performance has been suggested for some time. Other parameters that potentially influence or upgrade per- formance are: 1) higher strength matrix and cladding material, 2) lower concentration of the f1881le phase, and 3) lower temperature. Yet when all these factors are considered, the Pu0g-stainless steel carnet fuel concept appears marginal for application in FFTT at temperatures of approximately 1200°F. ORNI - AEC - OFFICIAL :: ORNL - AEC - OFFICIAL ORNI -ALC - OFFICIAL : A, Bibliography of References on trounicom Dioxide-Stainless Steel Dispersion Fuel Technology 1. M. J. Feldman, R. J. Boavar, and J. E. Cunningham, "Radiation Damage to Solid Fuel Elements - The Effect of particle Size on the Mechanical Behavior of Irradiated Stainless Steel-102 Fuel Elements," TID-7526, Part 3, (February 1957). 2. R. J. Beaver, R. C. Waugh, and C. F. Leitten, Jr., Specifications for Army Package Power Reactor Juel and Control Rod Components, ORNL-2225, (July 24, 1957). 3. R. J. Beaver et al, Investigation of Factors Affecting Sensitiza- tion of Army Package Power Reactor Fuel Elements, ORNL-2302 (Sept. 18, 1957). 4. 'J. E. Cunningham et al., "Fuel Dispersions in Stainless Steel Components for Power Reactors," Fuel Element Conference, Paris, November 18-23, 1957, T1-75146, Book I, PP. 273-268 (March 1958). 5. J. E. Cunningham and R. J. Beaver, "APPR Fuel Technology," Pro- ceedings, UN International Conference on Peaceful Uses of Atomic Pnergy, Second Geneva, Vol 6, p. 521 (1958) ATA .6. v. 0. Haynes, F. H. Neill, and I. D. Schaffer, Summary of 102, U ORNL-CF-58-2-71 (March 18, 1998). 7. J. E. Cunningham and R. J. Beaver, "Stainless Steel-Uranium Dioxide Fuel Conponents for the APPR," Nuclear Metallurgy V, pp. 29-40, Series No. 7, AIME-IMD Special Report (1958). - - -- - - - lam 8. J. E. Cunningham et al, Specificacions and Fabrication Frocedures for APPR-1 Core II Stationary Fuel Elements, ORNL-2649 (Jan. 1959). iner 9. A. E. Richt, Pontirradiation Fxomination of APPR Fuel. Elcment Irra. diation Program Specimene, ORNL-CF-59-3-33 (Mirch 9, 1959). 10. J. R. Weir, A Failure Analysis for the Low-Temperature Performance of Dispersion Fuel Elements, ORA L-2902 (Mey 27, 1960) Voitur 11. J. H. Cherubini, R. J. Beaver, ond C. F. Leitten, Jr., Fabrication • Development of 102-Stainless Steel Composite Plates for Core B of the Earico Fermi Fast Breeder Reactor, ORNIM GOT7 (April 4, 1961). e .. . .. ORNL - AEC - OFFICIAL .. ORNI - AEC - OFFICIAL . ...... ORNI - AIC - OFFICIAL 12. J. E. Cunningham, R. J. Beaver, and A. C. Waugh, "Dispersion in Metals, Uranium Dioxide: Properties and Nuclear Applications Ed:. by J. Belle, Naval Reactors, Division of Reactor Development, USAEC, Washington, (September 1961). 13. R. W. McClung, Feasibility Studies for the Nondestructive Testing of the Enrico Fermd Poactor Core Vol Element, ORPL-3221, (December 21, 1961). lk. R. J. Beaver, C. F. Leitten, Jr., and J. L. English, An Investiga- tion of the Corrosion Reoistince of Brazing Alloys for Austenitic Stainless Steel Fucl Elementi for Service in 565 F Pressurized Water, ORNL-2834 (March 29, 1962). 15. J. 8. Cherubini and S. Peterson, A Technique for the Quantitative Characterization of Dispersions, ORNI-TM-446 (February 28, 1963). 16. Army Reactors Program Annual Progress Report for Period Ending October 31, 1962, ORNL-3386 (April 2, 1963). 17 ; R. J. Beaver and C. F. Leitten, Jr., A Survey of Corrosion of Martensitic and Ferritic Staj.nless Steels in Pressurized Water, ORNL-TM-539 (July 16, 1963). 18. R. G. Donnelly, W. C. Thurber', And Q. M. Slaughter, Development of Fabrication Procedures for Corc B Friel Elements for the Enrico Fermi Fast Brceder Reactor, CANL-3475 (July 1961). 19. . W. C. Thurber et al, Irradiation Testine of Fuel for Core B of the Enrico Ferm 1. Fast Breeder Reactor, ORNL-3709 (November, 1954). 20. A. J. Taylor et ailey Characterization of Spheroidal UO2 Particles and Studies of Fabrication Variables for Corc B Fuel Plates of the Enrico Fermi Fast Breeder Reactor, ORNL-3645, (August 1964). 21. v. 0. Haynes and A. E. Richt, Preirradiation Data for the Fuel Specimens for the Army PM Fuel Experiment in the ORK Preseurized Water Loca, TORNL-TM in process of publication). 5. Blbliography of References on Irradiation Damage of Stainless Steel in W. R. Martin ard J. R. Weir, "Effect of Postirradiation Heat Treat- ment on the elevated Temperature Erbrittlement of Irradiated Stainless Steel," Nature, 202 (4936), 997 (June 1964). ----*** .com **** - ------- wm.com. ... ..... ------- powerpoint prennent pouw program 181)1310- 33V.INIO . · ORNL - AEC - OFFICIAL 2 W. R. Martin and J. R. Wcir, "The Effect of Irradiation Temperature on the Postirradiation Stress-Stirain Behavior of Stainless Steel," Pp. 251-268, Flow and Fracture of Metals and Alloys in Nuclear Environmento, Special Technical Publication No. 380, American Society for Testing Materials, Philadelphia, Pa., (1965). ?60-33W-ME . J. 1. Venard, C. R. Kennedy, and J. R. Weir, Effect of Irradiation on the Mechanical properties of Stainless Steel at 750 C Under Constant Stross Rate Conditione, ORNL-TM-1216 September 1965). 4. W. R. Martin and J. R. Weir, Effect of Irradiation Temperature on tnc Postirradiation Strc88-Strain Behavior of Stainless Steel, ORNL-IM-906 (October 1964). : 5. W. R. Martin and J. A. Weir, Influence of Grain Size on the Irra- diation Embrittlement of Statnless Steel E! Elevated Temperaturas, ORNI-TM-1043 (March 1965). - - - - - - -- 6. 'W. R. Martin and J. R. Weir, "Influence of Preirradiation Heat Treatment on the Postirradiation Ductility of Stainless Steel," . · Nucl. Appl. 1, pp. 478-483 (October 1965). - - - - - - . 7. W. R. Martin, J. R. Weir, and R. E. McDonald, "Irradiation En- brittlement of Low-Boron Type 304 Stainless Steel," Nature, 208 (5005), pp. 73-74, (October 2, 1965). 8. J. T. Venard and J. R. Weir) Efect of Irradletion on the stress... Rupture Characteristics of a 20%C 2599 NI Niobium-Stabilized Stainless Steel, ORNI-IM-1359 (Foaruary 1966). .. .... .- .-.-.- .-.-.....--- - IV2133 OINI - A&C - OFFICIAL NI - AEC - OFFICIAL FFICIAL OINLON OIN - AEC " 3:48-53459 | 4 | พ t, ระนง ! ; " " " " " " " " .. 4 . ' (4ษ" + * 1 " ": “ (AH1: : 11 - 4 (ชม : 1 . . พบป" : " " " " ?" "" “ !" + " " เ เ * เ ! 1 " - ---- - ------- ระยะ ๆ • • • . . "" -- - -0.035 INCHES [ +0ox บางนาม "TITV。 { " d " . . 1. " . 1 一件事是​, 14. : : qi ''''' 重 ​** * Myw世 ​PS . , 「. 了 ​| 。 | , 「 . 11 .. , 小 ​TIT": 11 , . " - 事事​,裡面 ​ups. 中的 ​+1 i - . 人 ​. . , hr: I °k 14 - . 「. ” , $ . . , . 字 ​: ……. " { . :", " w : ; : / 事 ​| , 才 ​。 。 :傅it ,4 , .. 心​, 1 、 ] Air tttt", , . 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" = " - . . ج مرغ .. ! .. : .. . . ۴ هال ز ا دين أشا: ت و : n " ، ". : . 1 1 1 " "- . 1 .1 ا ... و " 1 تا 5 دن ته و : . : ***** |. الب ** .: ::.: . ' '', 1, . اور ف 10 1 " له " F : " ..ية : . .هم " و من '' ن ن ا :" د . 1 به خون :5 :: م . ن : . .. . . : "" "" .ا" " :اج. ؟ نانو " .. دوا ۹۱ اهمل الصان دین رات 3- . . } - ای - : . - م E * " . : ا * : ن] بر ایرانوند و را ا * ة " . . . . عم مذہ نیمه بهمن . . " هم . . . . + ام ۲۰ ا " . \ 1 ة و - . . م . هو . و و و و . . 1 " ن... ... .. : .. .. . .... - به - -- -- " اند. " پر م بسته ، با از 1 f' ۱ ,F I 1 . - م . . الد : ' : اور ا له .. و ب ا رام و ... :. 1 . به == = ا ا | . اما I ' ' : .. و حههمر . ' ' هم " هند - - د ند. .۱ . * هستند. بیٹی ام می م فيلم * نسنین " -مد:. د و ا ا ام . ب ا ا م ا اعلا ن '' ... . ا . ا ا . هو ا با من الله " ا اله - ممد ع باد ... ع دد ورود به ، و به : . : .. * * . , . " * , .. 1:11 + . . ن = ** .. 1 = ۹۱ : . . در وم 4 ' ما ' ::: " : . , لا , , , , ' , . مها: ۱ ۰ ی ملا ا ا ا ا ایرانی " ! تازه . . سلامت : ان دا "" إنهم ** " دلم مداد س مت ها م برنامه ... , ' ان خیابان ۱۷ عدنان اليو را مهاباد ها و ماهی . 1 أما - ل . . . . . . او با ... ؟ وهله I' :: * ** . '' " . E ما ما برام الهلال بابت " ا ' ' ' ' ' ' ' ' ' ' ' .' ' .' |_ '' : . . . . ا ا . " الاسنان و ر . او 1 الم ا :: وا د : و . " . * * الان | ۴ ما و :: سی ' '. \ * . م . ومنها م ! . 1 - ا ہے : 4- * : اه : . - . " نور = . و ..) : . ، . د * همراه " " . . به ا . باران حمل . 1 لط سه : وطن " 1 F * | * . '| اااه .. وه .. . . ::: : : FA, , مجد . .. .. : و : " ما : ' . بهمن ماه : * * * , ۴. جنش و . . - . . . . . . .. ع " م . م و هم به ه مه . هی هم دم - دلامونه کده مه رو به یه 7 ,:؟ احمد . هو F : ه 4 . .1 4 2 - : '' لند + انا : الله : و " و " علم کا 1 , 1 . ، .. .. بهمگا وات ' ما .1 . در ماه سر برده .. به اپ و ۱۰ انه : 1 و با مزه 1II " : ا : عليها - :: ! . . "" . . " - "" طر... " " م . میر و .ها و== - ا ! + . . r - ه ت اج عمان- نانو اهور * .3 / : معمر هم . ب ود . و * .... " . ... - أ مما "... "ل + ۱۰ گ ا ۔ - " "" : : : استاد امان : غدد " التي ا أ | | | ''ز ا . ع ا ا ا ا ا ا ا ا ا " " " " . . . " " الف. با. 18 1 . وم : '' . م وا انی " : : يا و لا رها 11* ۱ ، ۱ 1 " ر . " . . . اله بالا . ا , 1 , م ! علی.. ..... د - ورود ۴۴ ماز ا ۱۰۰ " " " ت هما 1 با : 1 " " . . ولا.. * " یه * ه است 'امنا ا . : ه ا " الان واتا ا ' اه "" " ار ار در فيلو اور میرا وا این خود و با دقت و ظالم سما ... اما بعد: ۲۰۰ ، و : امدید !و / مل ومما " وااار و و مهمه .. بال و را " دیا ' ' | . . . 4 د. و دام : مه مر . 1 1 امام رهام.۱۰ ۰۰ مه ک ا ا ا ا , ا ه 1 . | | دار و ... را به * . هیات بات ۱ :الم ,اج ا ل ا . 4. ء " لو ن اسرا ، داوا" '' را .1 دولا ن ه : " با " با امام ماند ا ، ا : را از ۱۴ دیدنی ا یران . فهد مر ا ر دی . . و - ني هام وخ- -- , , و . ، اور ' ' . م . . . . شر وه و ا هلا / ا ۱ ا ا " : . . . . . برادو . . . .. .. .. .. ( . 2 ا ا ا لیس - -- . . " و .11 -- : . - و . . . * - . . . - ب - ب ن ر ا ر " " " ا " " ا " - " و ا ا ، . ا " . . . :۰۰ ب . . . : . " . . . .. . . " ا ا ا ل لا نوجوان ط "" " : و مر گر " : . 11 . ا ر - اہد، ا=:=:= د الزي FF" ... " * ..؟ اتر " ا اد : ده 8 و بار ، علما ن -نها . د و ا . " " : ،،، اس ، س , . ,وء ولا . .: اعمال ساعة و 11 م : همه . : اب 4 .. ' 3 . خ دا : - ده در ه - - د " : - - - - - . د .. .د. -. پیمب :. ' : دو T = ' : 1 اتناش : - - - * * لا اله و ته . د عم مج خيخ مه - . - . . - . - - . - . . و ... . - ا ، : . : . . T ها . . . دوه " وہ : نا .اه م ۱۰۰۰ ۴. .. . . ۲ , ۰۰۰ : ۱۶ . د ای به 3 :" و"؟" . م " : " و 5 . P | و | . " . " " . - . . " . بي .دند و ... .. ، , : ' : اف فر .. ا. .. " :: :: ". . " " ا :: 1 ::" | و ، الا ( . امی م م تحلل.. ". وب . . . مد - .. " ,+4 . + + 1 خطتهم ت لام، . ب | ه . .. با ...... بار '' اور .." . ! :على ام ا 2. . '', " لو " في . . و . . : د : | . * . ' , . اند . ر .. . , " " - مه و . . . . .. .۔ * . . . ه . 7 . د د الزينة "الا.. ا پ در: ۴ ل ه ا يرد ... ..لا .. را .. د .. ا رد . ۱۱ ماما تمام شده ا و باران به نام من می بازی . ها 5 " ان ما ... " اما خ ان " ". " ! . - له "ن ها . . . . .. ها . د ملا | لیا و ان . ترین . . -. - T F با الا . . . . . دین هم د مجاه " ( امممممممممهممممم : 1 1 : ونے . د . أ . د علم د. عبر عهده :این :. به . م ن ربه " " میان = = : " .. "م if و .. .: * : ول ..... .... .. . . از : به به سی ' . . , * ... " , م ا , , و " ادو » | و مال لاء - { "T -۱۹ .. زر " - و | دوم ا . . بالبالون | ، ! . . ' . . . . . . ؟' . ... . . ! ! : ۰۱ ویر :: دبی 5 :د , وهو - ولا . ع . ا ا عر لانے . * .. - * * * : ... . .ل ... ' عده ای ... . :. ام I . ،، ۱۰ د . . . . و . . . . . س . ' ' . حمية بمصدومه * " . " الله مجید میبینید . . وفق" - و ما هي .. اسدا. : .. : " ۰۰:۰۰ * * * TE لما اليد . مجلة . . برای . . و مطار المطعم و مد* . '' و = . . 1 . - 4 - .م .. . . ! ... و | || | .. . نن . - : لا دا | . . ۱۲ كل ا="" بدلے . م.، ة رو . و " ! E ... : : : : ارا . | : : : ایمان : ": :. : - . | - ها .. : و ۲۰۶ - ہم سپرده : : 'اء * : ' ' * . . ما ۔ . . . به همهمه این همه باید به مصر خمسه . : 1 . " : . * معده ": اولا ا ا . . ... ! و بخرم . * + " . 1" * . . . - و + و . ": . لملامین ، که ۱۰ به . ا :اول , بدء ، ، '': . م. ... وما کی . ...... ان . . . . . دن ا و ر ۱۰ و من ء ا : . . مم من . .- ہو. 4 : * * * با : : الراي الدوامة ردم با ER : او ۲۲ ! را که ..! 1 را { t ، + دولار -A ] 1" ", . ن . ',' تا حالا . ** وم و .. + + مه . . : : أن ان) باء - کو با جواب .. همه ا هما " " : _ ... . :: .. ا ا ا : 1 . ' . و ۲۰ هواء و : . : + , : : " .. ' : و " 1 : ا م جملایا و ؟ ه : 1 * . : ادار * ب "-بند والا ا . . ." ور ::.:. - : : انه من ...... و الا به :: .1 ا ا . . ا عا . ا :1 1 به " t ده ها ولاد .. " - ان . محمد، " 1 - 1 شاهد ... امام . . . ! .۱ . ! ... ... ... . . . . واژه و . . . . . دندان , . = ام تر 0 دارد (1) "الننناير - - ! جدا,, 'اب در " ." ز درمان امام و باطن 51 " ' د ناد تجاری ' و: " " I. . .. . ' 1 س ال ۹۷ تا ۱۹۹۰ جاتا او با ایران را ادا - مالی ,1"== 1 | باد در ال له .. ' به - . " . . ا ، ا ء " 1 * ... - مد ا * زاد :... لا ، } ين : + . - امام : 1 ء دیا' . . اره . . ... ... . .. : با * بن و ..... م - بندر : د و ' 4 . n = ا *4 و ومي، و اور حس جما . خانواده : ما * م ء این . ه * م | . F | ی م - : - - له :۱ ده .... م : له خه که " " . : داد ماه : مسجد مه : وطن C رد من " بمطعم " ژ . . .. .ه - 1 . 4 في - - - - .- . ۱۰۰ : لا .. .. .. .. . - هم " ي سيرا . 14 سنه = = FIF * همه جانبه به ما ص فوی | . وء . ی -- . = 1 - .. . عمله + ++ ++ اسم مع مواصم + انعم الله عنهما ان بار * 4. . تب : اه. الغد".. ... " ، ، . . " . . . . 'ر : ۹۰ دلاليه . . آل * . . : .... الم . ::. ا ا و " " . . ي . اسما ء : ا ... ܕܕܪܐܪ ܕ . . '' . 1 داع ء ". " "- I' . شد ، شان - و ، . ۲ . . . - - را - . . و " :: . : : ۱۰۰ ' . " " . و " له l سار , :i " :. : ' ا نا ء . ا ا- ر ۰۴:L: : " ا ا . . لا . آن اج - ا د ارا ان را رو ا ا ا ا م ا :- اجلاس """ """"""""""""" 1 . : ا لرابط اي انا و مهار * ور عالم | . . * . ا. ا " . . . . . . . ما ' امام ل .. ز مر و مهنده منافسه مما الح . . * . . . . . it :: اعت . ا : . | کو , . ا | | . ها | | رها انا :i والد ... نه : " . " محمد و م ا ا رها ا ا . یه و ه .. '' ملا: " " " " " " !او " ... " ا م . . , موخ و 1 ته 4 ' . الوا .... : ار ا ما * : حجم و - اور "" '\.\ بد نیز به رام حد } * t; .. .. ORNL--LR-DWG 75068R3 100 300 SURFACE TEMPERATURE (°C) 500 700 900 (x102011 PROBABLY STABLE PROBABLY UNSTABLE • BMI-32 • ORNL-46 À BMI-33 8 BMI-GCRE G KAPL X NDA-1 PWAC I ORNL-21 FISSION DENSITY (fissions/cc) NUMBER OF SAMPLES *(8) ORNL (1963) ORNL (1958) BM! (1961) --- (12) _ OPEN SYMBOLS INDICATE FAILURE F!LLED SYMBOLS INDICATE NON-FAILURE (8) (8)* 18 (2)x (2)x. ! (2) I (2)* OO 200 400 600 1800 2000 2200 2400 800 1000 1200 1400 1600 SURFACE TEMPERATURE (°F) Irradiation Stability of UO 2 - Stainless Steel Dispersions. = . ... .. . . . . . . . se. --:- - . . . . . . . at - - 3/ 17 / 167 DATE FILMED . 511 END . . WA YLE 11 446