key: cord-0732173-cbs33dk3
authors: Fan, Zhiyu; Zhan, Qingming; Yang, Chen; Liu, Huimin; Zhan, Meng
title: How Did Distribution Patterns of Particulate Matter Air Pollution (PM(2.5) and PM(10)) Change in China during the COVID-19 Outbreak: A Spatiotemporal Investigation at Chinese City-Level
date: 2020-08-28
journal: Int J Environ Res Public Health
DOI: 10.3390/ijerph17176274
sha: d60f4f83ac0adcc79c107ba99c491f11b3b50cbf
doc_id: 732173
cord_uid: cbs33dk3

Due to the suspension of traffic mobility and industrial activities during the COVID-19, particulate matter (PM) pollution has decreased in China. However, rarely have research studies discussed the spatiotemporal pattern of this change and related influencing factors at city-scale across the nation. In this research, the clustering patterns of the decline rates of PM(2.5) and PM(10) during the period from 20 January to 8 April in 2020, compared with the same period of 2019, were investigated using spatial autocorrelation analysis. Four meteorological factors and two socioeconomic factors, i.e., the decline of intra-city mobility intensity (dIMI) representing the effect of traffic mobility and the decline rates of the secondary industrial output values (drSIOV), were adopted in the regression analysis. Then, multi-scale geographically weighted regression (MGWR), a model allowing the particular processing scale for each independent variable, was applied for investigating the relationship between PM pollution reductions and influencing factors. For comparison, ordinary least square (OLS) regression and the classic geographically weighted regression (GWR) were also performed. The research found that there were 16% and 20% reduction of PM(2.5) and PM(10) concentration across China and significant PM pollution mitigation in central, east, and south regions of China. As for the regression analysis results, MGWR outperformed the other two models, with R(2) of 0.711 and 0.732 for PM(2.5) and PM(10), respectively. The results of MGWR revealed that the two socioeconomic factors had more significant impacts than meteorological factors. It showed that the reduction of traffic mobility caused more relative declines of PM(2.5) in east China (e.g., cities in Jiangsu), while it caused more relative declines of PM(10) in central China (e.g., cities in Henan). The reduction of industrial operation had a strong relationship with the PM(10) drop in northeast China. The results are crucial for understanding how the decline pattern of PM pollution varied spatially during the COVID-19 outbreak, and it also provides a good reference for air pollution control in the future.

China, as the largest developing country in the world [1] , has experienced a rapid process of urbanization and suffered from the accompanying air pollution problems. Among them, particulate availability and reliability and is hard to measure, especially during a relatively short period. As the development of mobile Internet technology, traffic mobility can be perceived easily by the data from location-based service (LBS) [27] . Moreover, it can present the change of traffic mobility with high temporal resolution, thus possibly being the solution for the short-period research studies, like ours.

In terms of investigation methods, some scholars used classic statistical methods, such as ordinary least square (OLS) model and stochastic impacts by regression on population, affluence, and technology (STIRPAT) model, for relationship analysis [23, 28] . These models indicate the overall influence of different factors by some global coefficients and cannot depict the spatial heterogeneity among different geographical objects. To solve this issue, geographically weighted regression (GWR), a local regression method, indicating the influence of factors by many spatial coefficients, were introduced in some research studies [29, 30] . However, there are also some disadvantages for GWR. For example, GWR assumes that all influencing factors affect the result at the same scale, which may induce some errors. For the research studies of air pollution underlying mechanism analysis, the relationship between pollutants and different influencing factors usually varies in spatial scales [31] . Therefore, GWR may not perform well for the influencing factors analysis in our research. Recently, an improved model of GWR, multi-scale geographically weighted regression (MGWR), was developed [32] . This model can obtain the optimal bandwidth for each influencing factor and address the issue of imposed scale heterogeneity, which might be the better choice in our research.

In this study, our goal was to derive the pattern of PM 2.5 and PM 10 change by comparing the concentrations in two study periods of 2019 and 2020, respectively, for prefecture cities of China and to further analyze the influencing factors. The study period was set from 20 January to 8 April, when the COVID-19 virus spread seriously in China and related control measures were the strictest during this period in 2020. Firstly, spatial autocorrelation analysis was conducted to recognize the PM concentration change pattern of all prefecture cities in China. Then, for reflecting the traffic mobility reduction, we collected intra-city mobility intensity of Chinese prefecture cities from the Baidu platform and used the average difference between 2019 and 2020 as the indicator for the regression analysis in the next stage. Lastly, MGWR was applied for the relationship investigation between the decline rates of both PM 2.5 and PM 10 and the influencing factors, including meteorological factors and socioeconomic factors.

Hourly PM 2.5 and PM 10 concentration data from 20 January to 8 April in 2018, 2019, and 2020 were downloaded from China National Environmental Monitoring Center (CNEMC, http://www.cnemc.cn). The reason for adding the data of 2018 is to compare the difference in the change between 2019 and 2020 and the change between 2019 and 2018. It includes more than 1500 ground sites established by Chinese government in all 337 prefectural cities of China (excluding Hong Kong, Macau, and Taiwan). The number of sites in each city is given by Figure 1 . Among them, there are 232 background sites and the others are non-background sites. At each site, data of PM 2.5 and PM 10 were calibrated by automated monitoring systems according to HJ 655-2013 [33] . We first excluded the null data in the original dataset. Then, the daily average PM 2.5 and PM 10 concentrations of each site were calculated. Based on daily average data of sites, we further calculated the average concentrations of each city. Due to data deficiency, the average PM 2.5 and PM 10 concentrations of 336 cities, in total, for the study period were obtained as final. Given the distinct concentration variations among different cities of China and two PM pollutants, relative decline rates of the two pollutants, respectively, presenting the temporal changes from 2018 to 2019 and 2019 to 2020, were calculated using formula (1) . Here, drPM is the decline rate of PM pollutants (PM2.5 or PM10) concentration of city i, and PMa and PMb are the average concentrations of the prior year (2018 or 2019) and this year (2019 or 2020) of city i, respectively. Besides, for analyzing the hourly change of PM pollution, average concentrations of each hour were also calculated. drPM = (PMa − PMb )/PMa (i = 1, 2, 3 … , 336).

(1)

Multiple meteorological indexes were used for relationship investigation, including relative humidity, air temperature, wind speed, and total precipitation. Data of the meteorological indexes were obtained from the China Meteorological Data Network (CMDN, http://data.cma.cn). This website provides historical daily meteorological observations of all prefectural cities in China. Then, we averaged the daily observations from January 20 to April 8 in both 2019 and 2020 to obtain the mean of each city during the study period. Furthermore, the decline values of four meteorological indicators were derived by using the mean of 2019 minus that of 2020.

During the outbreak of COVID-19, emission reduction of industry and traffic mobility were the two major reasons reducing air pollution [19] . It has been confirmed that the emission of the industry has a close relationship with the secondary industrial output values (SIOV, i.e., the gross product of secondary industry of each city) [22, 34, 35] . Therefore, for indicating the decrease of PM concentration caused by the reduction of industrial operation, decline rates of the secondary industrial output values (drSIOV) in the first quarter in 2020 (compared with the first quarter in 2019) of prefectural cities were obtained from the socio-economic operation bulletins. In China, drSIOV were directly announced by each local government statistics office. Limited by data availability, the drSIOV of 264 prefecture cities in total were obtained. Thus, the regression analysis would be conducted on these 264 cities, rather than all 336 cities.

Nevertheless, the traffic mobility reduction can't be reflected effectively by government documents in this relatively short period of COVID-19 outbreak. Fortunately, mobility data based on LBS provides a solution for this issue. Given the easy contagiousness and the fast spread of COVID-19, some scholars have adopted some mobility data from mobile phones or the Internet to figure out the epidemic and obtained some crucial findings of the spread of COVID-19 in different regions [36] [37] [38] . Similar to the spread of COVID-19, traffic PM emission also has a close relationship with mobility [39] , thus using these mobility data may also work out in detecting the change of PM pollution caused Given the distinct concentration variations among different cities of China and two PM pollutants, relative decline rates of the two pollutants, respectively, presenting the temporal changes from 2018 to 2019 and 2019 to 2020, were calculated using formula (1) . Here, drPM i is the decline rate of PM pollutants (PM 2.5 or PM 10 ) concentration of city i, and PMa i and PMb i are the average concentrations of the prior year (2018 or 2019) and this year (2019 or 2020) of city i, respectively. Besides, for analyzing the hourly change of PM pollution, average concentrations of each hour were also calculated.

Multiple meteorological indexes were used for relationship investigation, including relative humidity, air temperature, wind speed, and total precipitation. Data of the meteorological indexes were obtained from the China Meteorological Data Network (CMDN, http://data.cma.cn). This website provides historical daily meteorological observations of all prefectural cities in China. Then, we averaged the daily observations from 20 January to 8 April in both 2019 and 2020 to obtain the mean of each city during the study period. Furthermore, the decline values of four meteorological indicators were derived by using the mean of 2019 minus that of 2020.

During the outbreak of COVID-19, emission reduction of industry and traffic mobility were the two major reasons reducing air pollution [19] . It has been confirmed that the emission of the industry has a close relationship with the secondary industrial output values (SIOV, i.e., the gross product of secondary industry of each city) [22, 34, 35] . Therefore, for indicating the decrease of PM concentration caused by the reduction of industrial operation, decline rates of the secondary industrial output values (drSIOV) in the first quarter in 2020 (compared with the first quarter in 2019) of prefectural cities were obtained from the socio-economic operation bulletins. In China, drSIOV were directly announced by each local government statistics office. Limited by data availability, the drSIOV of 264 prefecture cities in total were obtained. Thus, the regression analysis would be conducted on these 264 cities, rather than all 336 cities.

Nevertheless, the traffic mobility reduction can't be reflected effectively by government documents in this relatively short period of COVID-19 outbreak. Fortunately, mobility data based on LBS provides a solution for this issue. Given the easy contagiousness and the fast spread of COVID-19, some scholars have adopted some mobility data from mobile phones or the Internet to figure out the epidemic and obtained some crucial findings of the spread of COVID-19 in different regions [36] [37] [38] . Similar to the spread of COVID-19, traffic PM emission also has a close relationship with mobility [39] , thus using these mobility data may also work out in detecting the change of PM pollution caused by traffic mobility reduction. We obtained daily intra-city mobility intensity (IMI) data of the corresponding 264 prefectural cities in the study period of 2019 and 2020 from the Baidu platform. Baidu is an Internet company in China and provides the LBS for 195 million people in mainland China. The daily IMI provided by Baidu is the intensity of residents' traffic travel of a city, which is recognized by origin and destination (OD) pairs of residents based on Baidu LBS data. The higher the index is, the more people go outside (with a relatively long distance) in a city. The mobility data of Baidu also played an important role in other studies about predicting the spread of COVID-19 indicating high data quality [36] . For depicting the change of IMI, we further calculated the decline IMI of each city by using the average IMI of 2019 minus that of 2020.

To sum up, there are two separate dependent variables and six independent variables. The dependent variables comprise the decline rates of two PM pollutants (drPM 2.5 and drPM 10 ). The independent variables include (1) Meteorological variables, including the decline of relative humidity (dHUM), air temperature (dTEM), wind speed (dWS), and total precipitation (dTP).

(2) Socioeconomic variables, including the decline rates of the secondary industrial output values (drSIOV) and the decline of IMI (dIMI). These variables would be applied for the regression analysis investigation further. As mentioned in Section 2.1.3, we only obtained the data of 264 cities in China. Fortunately, these 264 cities are mainly located in the areas where the COVID-19 epidemic was serious during the study period, so the analysis was still representative. Some statistics about the six influencing factors, including dIMI, drSIOV, dTEM, dHUM, dWS, and dTP and two dependent variables, drPM 2.5 and drPM 10 , in 2019-2020 are shown in Table 1 . 

In order to figure out the characteristics of two PM pollutants' temporal change spatially, spatial autocorrelation analysis was applied. Specifically, the global Moran's index (Moran's I) [40] , which is widely used for spatial dependence detection, was calculated for drPM 2.5 and drPM 10 . The calculated formulation is shown as (2) and (3):

Here, I global is the global Moran's index, n is the number of all prefecture cities (n = 336). x i and x j are the observations of city i and city j, respectively. W ij represents the neighboring relationship between city i and city j. If city i is adjacent to city j, then W ij = 1; otherwise, W ij = 0. The range of global Moran's index is between −1 and 1. If the value of global Moran's index is positive (negative), it indicates that there is a positive (negative) correlation among all observations. If the value is closed to 1 (−1), the positive (negative) correlation relationship is strong. In addition, it shows a random distribution of observations in space when the value is closed to 0.

The global Moran's index can only demonstrate the overall intensity of spatial correlation, so we calculated local Moran's index [41] further for each city. The formulation is shown in (4):

Here, x, x i , x j , W ij are derived the same as mentioned above. I i local is the local Moran's index of city i.

The significance of I global and I i local can be measured by Z value. The formulation of Z value is given by (5) .

where I is I global or I i local , E(I) is the expected value of I, and VAR(I) is the variance of I. For the Z value of global Moran's index, at the significance level is 0.05, it shows a significant result if the Z value is higher than 1.96 or less than −1.96, while a not significant result otherwise. For the Z value of local Moran's index, at the significance level is 0.05, if the Z value is higher than 1.96, then it shows that a city with high (low) drPM 2.5 or drPM 10 is surrounded by other cities with high (low) drPM 2.5 or drPM 10 . If the Z value is less than −1.96, then it shows that a city with high (low) drPM 2.5 or drPM 10 is surrounded by other cities with low (high) drPM 2.5 or drPM 10 . If the Z value is between −1.96 and 1.96, it shows that the correlation relationship of a city with surrounding cities is not significant.

Correlation analysis was used for detecting the relationship between the decline rates of PM concentration (drPM 2.5 or drPM 10 ) and influencing factor variables. Here, we selected Pearson Correlation Coefficients as the measurement, and the formulation is given by (6):

where x = 1 n n i=1 x i , and y = 1 n n i=1 y i . x and y represent the two compared variables. Here, n = 264 which is corresponded with the number of cities in regression analysis. R xy is the Pearson Correlation Coefficients and its range is between −1 and 1. It represents a negative relationship between two variables (x and y) when R xy < 0, and a positive relationship when R xy > 0. If the absolute value of R xy is close to 1, then it shows a strong correlation relationship between variable x and variable y. If the absolute value of R xy is close to 0, then the correlation relationship is weak.

The relationships between the decline rates of PM pollutants and related influencing factors were investigated by OLS, GWR, and MGWR. We would compare the performance of them and use the best model for analyzing further. OLS is a widely used global model for relationship analysis and the formulation can be shown as (7):

where Y is the dependent variable and, specifically, is the PM pollutants decline rate (drPM 2.5 or drPM 10 ). X k is the independent variable k. β k is the coefficient of X k . ε is the random error item.

GWR is the extension of OLS regression in space. Compared to OLS with a set of constant parameters for all locations, in GWR, each sampling location has their own parameters [42] . Through this, the characteristics of spatial variation can be depicted. The formulation of GWR is given by (8):

where (u i , v i ) is the coordinate of the local sampling location. In our research, (u i , v i ) of each city is the centroid of all ground PM pollutants observation sites. n is the number of city (n = 264).

can be estimated by the data from neighboring locations, and the spatial weight of the estimated data can be measured by distance weighting functions. Here, we used Bi-square function in our research for weight calculation, which is given by (9) .

where d ij is the Euclidean distance between location i and location j. b i is the adaptive bandwidth of location i. Although GWR can depict the spatial heterogeneity, the assumption that all relationships between the dependent variable and influencing factors operate at the same spatial scale limits the performance and reliability of the regression result. For addressing this issue, MGWR [32] , which relaxes the "same spatial scale" assumption and allows specific bandwidths of different independent variables' relationship with the dependent variable to be optimized, was applied in our research. The formulation of MGWR is given by (10):

Other than β bw0 and β bwk , other parts of (10) are the same as (8), where bw0 is the bandwidth of intercept and bwk is the bandwidth of variable k. Therefore, different from GWR, each local parameter β k is obtained under the condition of a set of optimal specific bandwidths rather than one bandwidth for all relationships between independent variables and the dependent variable.

We used 3 measurements for evaluating these 3 regression models, including the coefficient of determination (R 2 ), the corrected Akaike information criterion (AICc), and the residual sum of squares (RSS). The MGWR model was conducted using the software MGWR2.1 provided by the School of Geographical Sciences and Urban Planning at Arizona State University (https://sgsup.asu.edu).

The spatial distribution of PM 2.5 and PM 10 , the decline in the study period of 2020 compared with 2019 (hereafter 2019-2020) was more notable with decline rates of 16% and 20% for PM 2.5 and PM 10 , respectively. According to the Chinese Ambient Air Quality Standards (CAAQS) [43] , there were only 6 (10), 15 (29) , and 20 (73) cities reaching the annual "good" level of PM 2.5 (PM 10 ) standard, respectively (<15 µg/m 3 for PM 2.5 and <40 µg/m 3 for PM 10 ) in the study period of 2018, 2019, and 2020. In terms of space, the spatial patterns of both PM 2.5 and PM 10 were similar for these 3 study periods with high PM pollution areas in the North China Plain and Xinjiang and low PM pollution areas in coastal and southwest regions. Except some northwest cities located in the desert, it is noted that most cities in China had experienced a huge improvement of PM pollution in 2019-2020. A comparison at national scale between background sites (BS) and non-background sites (NS) was also conducted and is shown in Table 2 . Here, Avg_PM 2.5 and Avg_PM 10 represent the average PM 2.5 concentration and PM 10 concentration, respectively. Results illustrate that there was a consistent decrease in PM concentrations of both two type sites. It is noted that the decreased concentrations of NS in 2019-2020 (about 10 µg/m 3 for PM 2.5 and 19 µg/m 3 for PM 10 , respectively) were much higher than that in 2018-2019 (about 3 µg/m 3 for PM 2.5 and 11 µg/m 3 for PM 10 , respectively), while the decreased concentrations of BS were relatively constant (about 6-9 µg/m 3 for PM 2.5 and 18 µg/m 3 for PM 10 , respectively, for both 2018-2019 and 2019-2020). This is related with the location of background sites. Generally, for better representing the air pollution in large areas, background sites in China were established in the areas that are far away from urban centers. These areas are of relatively low population density and were affected less during the COVID-19 period, so the decreased concentrations in background sites were not significant as that in non-background sites. In terms of temporal perspectives, the daily average and hourly PM concentration over China was calculated and some related statistics are shown in Figure 3 . According to the 24-h average PM2.5 standard in CAAQS, there were 4%, 10%, and 38% days in the study periods reaching the "good" level (<35μg/m 3 ) for 2018, 2019, and 2020, respectively. As for PM10, there were 12% days in the study period of 2020 reaching the "good" level (<50μg/m 3 ), and there was no day reaching this level in 2018 and 2019. As for the hourly change, both PM2.5 and PM10 showed a shape of the "W" trend from 0:00 to 23:00 with reaching the peak at 0:00 and 10:00 and reaching the valley at 6:00 and 16:00. In addition, the decreasing concentrations in 2019-2020 were much higher than that of 2018-2019 at all-time points with about 10μg/m 3 and 20μg/m 3 for PM2.5 and PM10, respectively. In terms of temporal perspectives, the daily average and hourly PM concentration over China was calculated and some related statistics are shown in Figure 3 . According to the 24-h average PM 2.5 standard in CAAQS, there were 4%, 10%, and 38% days in the study periods reaching the "good" level (<35 µg/m 3 ) for 2018, 2019, and 2020, respectively. As for PM 10 , there were 12% days in the study period of 2020 reaching the "good" level (<50 µg/m 3 ), and there was no day reaching this level in 2018 and 2019. As for the hourly change, both PM 2.5 and PM 10 showed a shape of the "W" trend from 0:00 to 23:00 with reaching the peak at 0:00 and 10:00 and reaching the valley at 6:00 and 16:00. In addition, the decreasing concentrations in 2019-2020 were much higher than that of 2018-2019 at all-time points with about 10 µg/m 3 and 20 µg/m 3 for PM 2.5 and PM 10 

The change distribution of PM pollutants, including drPM2.5 and drPM10, were derived as shown in Figure 4 . It can be found that the change distribution of 2019-2020 is totally different from that of 2018-2019 for both PM pollutants. In 2018-2019, the areas with decline rates higher than 30% were mainly located in some western regions, like Tibet and Xinjiang. The PM pollution in north of China especially Heilongjiang, Jilin, Liaoning, Shandong, and Henan were getting worse compared to the study period of 2018. However, the decline rates of 2019-2020 in these northern regions came to more than 20% for both PM pollutants. This is a very interesting phenomenon. These regions always suffer from PM pollution caused by high-emission industrial plants and inappropriate energy consumption structure [44, 45] , but the COVID-19 control measures became a very effective solution for this issue by accident. In addition, in central and southeast of China, PM pollution also showed a tremendous decline in 2019-2020. As for the comparison of two pollutants, the spatial distribution of drPM2.5 and drPM10 were similar in 2018-2019 but was observed with some differences in 2019-2020, showing that PM10 pollution was improved better than PM2.5 pollution in some northern areas. This is because heating from coal burning in north China continued during the COVID-19 outbreak, which still produced much PM2.5 [44] . There was a big difference of PM changed patterns between 2018-2019 and 2019-2020 in north western regions, which may be related to some random natural factors, like the sandstorms in spring. As for the city affected most significantly by the COVID-19, Wuhan, drPM2.5 and drPM10 were 2% and 12% in 2018-2019, respectively, while at 36% and 39% in 2019-2020. This demonstrated a notable PM pollution reduction during the COVID-19 outbreak period. 

The change distribution of PM pollutants, including drPM 2.5 and drPM 10 , were derived as shown in Figure 4 . It can be found that the change distribution of 2019-2020 is totally different from that of 2018-2019 for both PM pollutants. In 2018-2019, the areas with decline rates higher than 30% were mainly located in some western regions, like Tibet and Xinjiang. The PM pollution in north of China especially Heilongjiang, Jilin, Liaoning, Shandong, and Henan were getting worse compared to the study period of 2018. However, the decline rates of 2019-2020 in these northern regions came to more than 20% for both PM pollutants. This is a very interesting phenomenon. These regions always suffer from PM pollution caused by high-emission industrial plants and inappropriate energy consumption structure [44, 45] , but the COVID-19 control measures became a very effective solution for this issue by accident. In addition, in central and southeast of China, PM pollution also showed a tremendous decline in 2019-2020. As for the comparison of two pollutants, the spatial distribution of drPM 2.5 and drPM 10 were similar in 2018-2019 but was observed with some differences in 2019-2020, showing that PM 10 pollution was improved better than PM 2.5 pollution in some northern areas. This is because heating from coal burning in north China continued during the COVID-19 outbreak, which still produced much PM 2.5 [44] . There was a big difference of PM changed patterns between 2018-2019 and 2019-2020 in north western regions, which may be related to some random natural factors, like the sandstorms in spring. As for the city affected most significantly by the COVID-19, Wuhan, drPM 2.5 and drPM 10 were 2% and 12% in 2018-2019, respectively, while at 36% and 39% in 2019-2020. This demonstrated a notable PM pollution reduction during the COVID-19 outbreak period. 

Global Moran's indexes for drPM2.5 and drPM10 in 2018-2019 and 2019-2020 were calculated to identify whether the declines of PM2.5 and PM10 are clustered overall. The result is shown in Table 3 . All changes of PM pollutants saw global Moran's indexes much higher than 0, thus indicating the existence of spatial clustering. The spatial autocorrelation degree of drPM2.5 showed a slight increase in 2019-2020 compared to 2018-2019, whereas that of drPM10 decreased. Z values of four distribution were higher than 13, which means they all passed the significance test (P<0.001). In order to better display the spatial distribution pattern of drPM2.5 and drPM10, the clustering results were derived by local Moran's indexes and were shown in Figure 5 . The clustering pattern of local spatial autocorrelation can be categorized as 5 types: "high-high" (high observations surrounded by high observations), "high-low" (high observations surrounded by low observations), "low-high" (low observations surrounded by high observations), "low-low" (low observations surrounded by low observations), and not significant areas. Here, the observation is the drPM, i.e., the decline rate of PM. It can be found that the "high-high" and "low-low" are the main clustering types in all results of the local spatial autocorrelation analysis. Moreover, both two PM pollutants have similar spatial distribution patterns, indicating the close relationship between PM2.5 and PM10 [46] . The "high-high" clusters were in south, southwest, and some northwest areas, while the "lowlow" clusters were in northeast, central, and north areas in 2018-2019. This distribution pattern was also similar with some findings in other researches [47] [48] [49] . However, in the results of 2019-2020, the "high-high" clusters were mainly located in central, east, and south areas. This was related to the strong and enduring control measures of COVID-19 in these areas. The "low-low" clusters are mainly located in inner-Mongolia, northwest, and southwest areas in 2019-2020. Combined with Figure 4 , although it showed a decline trend of PM concentrations in these areas, the degree of decline was not 

Global Moran's indexes for drPM 2.5 and drPM 10 in 2018-2019 and 2019-2020 were calculated to identify whether the declines of PM 2.5 and PM 10 are clustered overall. The result is shown in Table 3 . All changes of PM pollutants saw global Moran's indexes much higher than 0, thus indicating the existence of spatial clustering. The spatial autocorrelation degree of drPM 2.5 showed a slight increase in 2019-2020 compared to 2018-2019, whereas that of drPM 10 decreased. Z values of four distribution were higher than 13, which means they all passed the significance test (p < 0.001). In order to better display the spatial distribution pattern of drPM 2.5 and drPM 10 , the clustering results were derived by local Moran's indexes and were shown in Figure 5 . The clustering pattern of local spatial autocorrelation can be categorized as 5 types: "high-high" (high observations surrounded by high observations), "high-low" (high observations surrounded by low observations), "low-high" (low observations surrounded by high observations), "low-low" (low observations surrounded by low observations), and not significant areas. Here, the observation is the drPM, i.e., the decline rate of PM. It can be found that the "high-high" and "low-low" are the main clustering types in all results of the local spatial autocorrelation analysis. Moreover, both two PM pollutants have similar spatial distribution patterns, indicating the close relationship between PM 2.5 and PM 10 [46] . The "high-high" clusters were in south, southwest, and some northwest areas, while the "low-low" clusters were in northeast, central, and north areas in 2018-2019. This distribution pattern was also similar with some findings in other researches [47] [48] [49] . However, in the results of 2019-2020, the "high-high" clusters were mainly located in central, east, and south areas. This was related to the strong and enduring control measures of COVID-19 in these areas. The "low-low" clusters are mainly located in inner-Mongolia, northwest, and southwest areas in 2019-2020. Combined with Figure 4 , although it showed a decline trend of PM concentrations in these areas, the degree of decline was not as large as the "high-high" clustering areas and the distribution of the PM pollution decreasing cities was not as dense as that In the "high-high" clustering areas. The "low-low" clustering areas were also the areas affected less by COVID-19 during the study period. as large as the "high-high" clustering areas and the distribution of the PM pollution decreasing cities was not as dense as that In the "high-high" clustering areas. The "low-low" clustering areas were also the areas affected less by COVID-19 during the study period.

. 

Before regression analysis, correlation analysis based on the Pearson Correlation Coefficient was conducted and the results are shown in Table 4 . It can be found that the coefficients between two socioeconomic factors and both decline rates of PM pollutants are positive, which means that the reduction of residents' travel mobility and industrial production have a strong positive relationship with the drop of PM pollutants. A previous study conducted in North America also confirmed that socioeconomic indicators tend to explain more variations of air pollutants and the findings of ours also are coherent with that view [22] . Additionally, it reflected that dIMI and drSIOV were appropriate as the influencing factors for detecting the changed pattern of PM pollutants caused by COVID-19 control measures. As for the meteorological factors, except dHUM, others have negative relationships with drPM2.5 and drPM10; so, the higher these meteorological observation values are, the lower PM concentration is in general. This is also consistent with some previous studies [50] . For examining whether the independent variables were fit for linear regressions, multicollinearity was detected using variance inflation factor (VIF) [51] . If the VIF value of an independent variable is higher than 7.5, then there exists multicollinearity, and the variable cannot be used with some other independent variables at the same time. The result is shown in Table 5 . It 

Before regression analysis, correlation analysis based on the Pearson Correlation Coefficient was conducted and the results are shown in Table 4 . It can be found that the coefficients between two socioeconomic factors and both decline rates of PM pollutants are positive, which means that the reduction of residents' travel mobility and industrial production have a strong positive relationship with the drop of PM pollutants. A previous study conducted in North America also confirmed that socioeconomic indicators tend to explain more variations of air pollutants and the findings of ours also are coherent with that view [22] . Additionally, it reflected that dIMI and drSIOV were appropriate as the influencing factors for detecting the changed pattern of PM pollutants caused by COVID-19 control measures. As for the meteorological factors, except dHUM, others have negative relationships with drPM 2.5 and drPM 10 ; so, the higher these meteorological observation values are, the lower PM concentration is in general. This is also consistent with some previous studies [50] . Table 4 . Pearson Correlation Coefficients between 6 independent variables and 2 dependent variables. For examining whether the independent variables were fit for linear regressions, multicollinearity was detected using variance inflation factor (VIF) [51] . If the VIF value of an independent variable is higher than 7.5, then there exists multicollinearity, and the variable cannot be used with some other independent variables at the same time. The result is shown in Table 5 . It shows that there are no variables with VIF higher than 7.5, so all these variables can be used for linear regression analysis. The abbreviations and the specific meanings can refer to the Section 2.1.4. 

Three regression models, including OLS, GWR, and MGWR, were conducted based on the normalized independent variables and the performances are summarized in Table 6 . The performance of OLS was very poor with R 2 of 0.227 and 0.217, respectively, for drPM 2.5 and drPM 10 . Two local regression models performed much better than OLS indicating the superiority of considering spatial heterogeneity. The performance of MGWR further outperforms GWR, with R 2 of 0.711 and 0.732 for drPM 2.5 and drPM 10 . In addition to R 2 , the results of RSS and AICc also illustrated the performance of MGWR to be the best among three models. Consequently, the strategy that produces the particular bandwidth for the relationship between each independent variable and the dependent variable in MGWR was effective in our research, and the results of MGWR would be applied for the analysis next. 

MGWR generated many local coefficients of different independent variables and some related statistics are listed in Table 7 . It includes three basic statistics including the minimum, maximum, and mean of each variable's coefficients in the PM 2.5 model and the PM 10 model. In addition, the optimal bandwidth (BW) (represents the number of neighboring cities whose data used for constructing local models) and the proportion of coefficients (PC) that passed by significance test (α = 0.05) of each independent variable were also shown in Table 7 . Table 7 . Some information about the coefficients in two MGWR models. BW is the optimal bandwidth of each variable, and PC is the proportion of coefficients passed by significance test (α = 0.05). The different optimal bandwidths of 6 variables in two MGWR models presented large variations in optimal spatial process scale. The bandwidth of dIMI was the smallest among all variables demonstrating the great spatial non-stationarity of traffic mobility caused by different levels of COVID-19 control measures in different areas. The process scale of drSIOV was larger with the optimal bandwidth of 73 in the PM 2.5 model and 127 in the PM 10 model, which exhibited the similar effects of industrial activity reduction spatially. As for meteorological variables, for the PM 10 model, both the imposed scales of dTEM and dWS were almost as large as the global scale with the number of neighboring of 263 and 229, respectively, while, in the PM 2.5 model, the optimal scales of all variables were relatively small, except dHUM. This presented that the other three meteorological factors affected the reduction of PM 2.5 at a relatively local scale compared with that of PM 10 .

In terms of PC, the great difference existed between socioeconomic variables and meteorological variables. The PCs of meteorological variables were all lower than 20% in both PM 2.5 and PM 10 models. While for the two socioeconomic variables, it can be found that the estimation of them were significant for more cities especially dIMI with 51% and 56% for the PM 2.5 model and the PM 10 model, respectively. Thus, the PM pollutants' concentration changes in the COVID-19 outbreak period have more closed relationship with the two socioeconomic influencing factors and were slightly affected by meteorology. Figure 6 shows the spatial coefficients of three variables with the highest PC, including dIMI, drSIOV, and dHUM, in two PM pollutants' models. The significance of the spatial coefficients was sometimes ignored in some previous researches using local regression, such as GWR and MGWR, and this will lead to questionable results [52] . In our research, despite some "not significant" coefficients, others that passed the p-value examination were reliable. In Figure 6 , the significant imposed range of different influencing factors varied spatially. The imposed ranges of two socioeconomic factors were much wider than dHUM. Although some meteorological factors like relative humidity are related to the formation of substances in PM, it may affect PM concentration notably at a shorter temporal scale. In addition, it is noted that coefficients of all three factors imposed significantly in southwest regions. On one hand, the cities in these regions are at the relatively primary stage of rapid socioeconomic development and were affected less by the COVID-19 so the influence of socioeconomic factors on PM pollution is remarkable [53] . On the other hand, most cities in these regions with low urbanization rates are surrounded by rainforests so the natural factors, like relative humidity, also play vital roles. The decline of IMI imposed the most significantly impact on the changes of PM pattern with the widest imposed range. In addition, it showed that the coefficient values' range of dIMI was also the widest in Figure 6 . Therefore, the relationship between dIMI and the change of PM during the COVID-19 outbreak is not only the most relevant but also owing the strongest spatial heterogeneity.

From Figure 6a ,b, the impacts of traffic mobility reduction on PM pollutants demonstrated great spatial heterogeneity. For both two pollutants, the impacts of traffic mobility were not significant in northwest and northeast regions. In addition, it saw a negative relationship with PM concentration in southwest regions, such as Yunnan and Guizhou. There are two aspect reasons for explaining this. On one hand, the PM pollutants reduction during the COVID-19 outbreak period was not obvious and even showed increased trends in these regions, which may be related with some exterior pollutants from southeast Asian countries [54] . On the other hand, the population density in these regions is relatively low, which means the reduction of residents' travel did not contribute too much to the PM pollutant emission [29] . Thus, despite a little PM decrease caused by traffic mobility reduction, the overall PM pollution did not decrease too much. On the contrary, traffic reduction had a notable effect on PM pollution drop in central, south, and east of China. It can be found that a decrease of 0.1 in IMI would lead to a decline in PM concentrations by higher than 5% in these regions. These regions with the highest population density suffered the COVID-19 control measures for a long time and both the decreases of IMI and PM pollution were very significant. Although the decline of traffic mobility made a great contribution to PM decline during the COVID-19 outbreak, it must be recognized that it is not a long-term effective solution. The government should further widely promote the application of electrical and hydrogen vehicles and encourage residents to use more public transportation [55, 56] .

There were also some differences between the two PM pollutants. Except for the south regions, the cities with high coefficients in the PM 2.5 model were mainly distributed in eastern regions, such as Jiangsu and Zhejiang, while those in the PM 10 model were mainly in central regions, such as Henan and Shandong. This may be related to the different main emissions of traffic [57, 58] . Compared with using complex traditional traffic emission inventories, it is more convenient to apply intra-city mobility intensity obtained based on real-time LBS data to measure the influence of traffic mobility on PM pollution during a relatively short time like the COVID-19 outbreak period. In addition, there is also some uncertainty about the applicability of traditional emission inventories [59] . Thus, in terms of presenting the relationship of traffic mobility and PM pollution, LBS data, like IMI, may be the best choice in our research. 

In this study, we obtained the changed pattern of PM2.5 and PM10 concentration at city-scale in China during the COVID-19 outbreak compared with the same period of 2019 by spatial autocorrelation analysis. In addition, an improved model of GWR, MGWR, was applied for detecting the influence of four meteorological factors and two socioeconomic factors on the drop of PM pollution. The main findings are as follows:

(1) The decline changes of both PM2.5 and PM10 presented a totally different spatiotemporal pattern in 2019-2020 compared with that of 2018-2019. In the result of 2018-2019, obvious "low-low" clustering patterns were found in north, central and east regions of China, whereas, in 2019-2020, it showed strong clustering patterns of high decline rates of PM2.5 and PM10 in these regions (2) IMI derived from Baidu and secondary industrial output values derived from local government bulletins were adopted to measure the influence of the decline of traffic mobility and industrial operation. These two variables showed an obvious positive relationship with the decline Figure 6c ,d present the spatial local coefficients of drSIOV. The reduction of industrial production led to a great impact on PM 10 drop in northeast China where is the basis of the Chinese heavy industry with very large secondary industry share. The local economic development mainly relies on mining, metal process, and machine manufacturing, which are the main sources of PM 10 pollution [60] . The COVID-19 control measures hindered the industrial operation thus making a significant contribution to PM 10 pollution improvement. In addition, the industrial operation has a strong relationship with PM 2.5 pollution concentration in southwest regions where the industrial operation was less affected and PM 2.5 pollution also showed a slightly increasing trend. In recent years, due to some restricted policies of central government on air pollution, many industrial enterprises were transferred from some developed regions like east of China to the southwest and this led to some serious air pollution issues [53] . Despite relative low PM concentrations in the COVID-19 outbreak, local government in southwest of China should be alert to the deterioration of PM pollution caused by industrial emissions. For both two pollutants' models, the "not significant" cities are mainly in northwest, south, and east regions. Due to the advanced technology and economy, industrial operation in south and east regions may not be closely related to PM pollutants. This is also corresponded with the EKC model (as the economic development, the pollution became worse first and then is alleviated) and some other previous findings in certain areas and other countries, like Canada [53, 61, 62] . As for northwest regions, the reason may be related to some other natural factors, such as the deserts in inner-Mongolia [63] . Figure 6e ,f show the local coefficients of dHUM. It can be found that there was mainly a negative relationship with PM pollution for relative humidity in the cities located in the forest and plateau. In addition, the relationship between relative humid with PM 10 is positive for cities located in the Qinling Mountains and west of Sichuan. For dHUM, there are only 12% and 14% of PC for PM 2.5 and PM 10 , respectively, although it is the factor with the highest PC among all four meteorological factors.

In this study, we obtained the changed pattern of PM 2.5 and PM 10 concentration at city-scale in China during the COVID-19 outbreak compared with the same period of 2019 by spatial autocorrelation analysis. In addition, an improved model of GWR, MGWR, was applied for detecting the influence of four meteorological factors and two socioeconomic factors on the drop of PM pollution. The main findings are as follows:

(1) The decline changes of both PM 2.5 and PM 10 presented a totally different spatiotemporal pattern in 2019-2020 compared with that of 2018-2019. In the result of 2018-2019, obvious "low-low" clustering patterns were found in north, central and east regions of China, whereas, in 2019-2020, it showed strong clustering patterns of high decline rates of PM 2.5 and PM 10 in these regions (2) IMI derived from Baidu and secondary industrial output values derived from local government bulletins were adopted to measure the influence of the decline of traffic mobility and industrial operation. These two variables showed an obvious positive relationship with the decline of PM 2.5 and PM 10 .

(3) MGWR outperformed OLS and GWR, with R 2 of 0.711 and 0.732 for drPM 2.5 and drPM 10 , respectively. This reflected that the strategy that releases the restriction of constant scales was very effective in our research. Thus, the results of MGWR were applied in the analysis of influencing factors.

(4) In the results of MGWR, compared with meteorological variables, the decline of IMI and the decline rate of secondary industrial output values had a more significant impact on PM pollution reduction. It showed that the reduction of traffic mobility caused more reduction of PM 2.5 in east China, such as Jiangsu and Zhejiang, while more reduction of PM 10 in central regions, such as Shandong and Henan, were observed. In addition, it was found that the reduction of secondary industrial output values caused more PM 2.5 drop in southwest regions of China and more PM 10 drop in northeast of China.

This study also has some limitations. First, limited by data, this study only adopted the data of 264 prefectural cities, which may cause some biases. Second, there are some other influencing factors, such as biomass burning, sand dust, and biogenic and biological PM, were not involved. Third, most PM observation sites are in urban areas while sparsely distributed in rural areas. This may also induce some uncertainty to the results. Last, some other meteorological factors, like atmosphere stability, which are also related with PM are not involved in this study, and we will consider these when data is available.

In general, although the COVID-19 control measures restricted travel freedom and economic development and forced people to conduct tele-work and tele-study, it provided an excellent and precious opportunity for observing PM pollution improvement. The findings of our research reflect the spatiotemporal PM pollution decline pattern and the impact of related influencing factors, thus being helpful for air pollution mitigation and control for the government. However, it also should be recognized that, despite the remarkable reduction, the concentrations of PM 2.5 and PM 10 were several times higher than the WHO standards during the COVID-19 outbreak. Therefore, there is still a long way to go to limit the PM pollution of China in the future. 

PM2.5Constituents and Hospital Emergency-Room Visits in Shanghai

Regional differences of pollution emissions in China: Contributing factors and mitigation strategies

Evolution of the spatiotemporal pattern of PM2.5 concentrations in China-A case study from the Beijing-Tianjin-Hebei region

Air conditioning and source-specific particles as modifiers of the effect of PM(10) on hospital admissions for heart and lung disease

Systematic review and meta-analysis of the adverse health effects of ambient PM2.5 and PM10 pollution in the Chinese population

Lung cancer, cardiopulmonary mortality, and long-term exposure to fine particulate air pollution

Burden of disease attributed to ambient PM2.5 and PM10 exposure in 190 cities in

Changes in spatial patterns of PM2.5 pollution in China

Separating contributions from anthropogenic emissions and meteorology

Air pollution reduction in China: Recent success but great challenge for the future

Impact of clean air action on PM2.5 pollution in China

Drivers of improved PM2.5 air quality in China from 2013 to 2017

Air Quality Guidelines; World Health Organization

Coronavirus Disease 2019 (COVID-19) Situation Report

Identifying airborne transmission as the dominant route for the spread of COVID-19

Air pollution reduction and mortality benefit during the COVID-19 outbreak in China

Decline in PM2.5 concentrations over major cities around the world associated with COVID-19

Effect of lockdown amid COVID-19 pandemic on air quality of the megacity Delhi

Air quality changes during the COVID-19 lockdown over the Yangtze River Delta Region: An insight into the impact of human activity pattern changes on air pollution variation

Characteristics of particulate matter (PM10) and its relationship with meteorological factors during 2001-2012 in Beijing

Humidity plays an important role in the PM 2.5 pollution in Beijing

Multi-year objective analyses of warm season ground-level ozone and PM2.5 over North America using real-time observations and Canadian operational air quality models

Spatio-temporal variation and influence factors of PM 2.5 concentrations in China from 1998 to

Impacts of energy consumption structure, energy intensity, economic growth, urbanization on PM2.5 concentrations in countries globally

The contributions of socioeconomic indicators to global PM2.5 based on the hybrid method of spatial econometric model and geographical and temporal weighted regression

Spatial-temporal characteristics and determinants of PM2.5 in the Bohai Rim Urban Agglomeration. Chemosphere

Activity-Based Human Mobility Patterns Inferred from Mobile Phone Data: A Case Study of Singapore

Has urbanization accelerated PM2.5 emissions? An empirical analysis with cross-country data

Application of geographically weighted regression (GWR) in the analysis of the cause of haze pollution in China

Investigation of the spatially varying relationships of PM2.5 with meteorology, topography, and emissions over China in 2015 by using modified geographically weighted regression

Examining the influences of air quality in China's cities using multi-scale geographically weighted regression

Multiscale Geographically Weighted Regression (MGWR)

Technical Specifications for Installation and Acceptance of Ambient Air Quality Continuous Automated Monitoring System for PM10 and PM2.5; Ministry of Environmental Protection

Manufacturing industrial structure and pollutant emission: An empirical study of China

An analysis of the driving forces behind pollutant emission reduction in Chinese industry

The effect of human mobility and control measures on the COVID-19 epidemic in China

Identification of COVID-19 can be quicker through artificial intelligence framework using a mobile phone-based survey when cities and towns are under quarantine

An investigation of transmission control measures during the first 50 days of the COVID-19 epidemic in China

When urban air quality inference meets big data

The Interpretation of Statistical Maps

Local Indicators of Spatial Association-LISA

Geographically Weighted Regression: The Basics. In Geographically Weighted Regression: The Analysis of Spatially Varying Relationships

Ministry of Environmental Protection jointly promote 'nationwide cleanliness, and water-saving initiatives'

Characteristics of trace elements in PM 2.5 and PM 10 of Chifeng, northeast China: Insights into spatiotemporal variations and sources

Sources apportionment of PM 2.5 in a background site in the North China Plain

Modeling the spatio-temporal heterogeneity in the PM10-PM2.5 relationship

La Niña on PM2.5 concentrations across China

Spatiotemporal patterns of recent PM2.5 concentrations over typical urban agglomerations in China

Temporal Variation Characteristics of PM2.5 in the Beijing-Tianjin-Hebei Region

The Relationships between PM2.5 and Meteorological Factors in China: Seasonal and Regional Variations

Linear-model Diagnostics. In Applied Regression Analysis and Generalized Linear Models

The Multiple Testing Issue in Geographically Weighted Regression

Spatiotemporal variation of PM2.5 concentrations and its relationship to urbanization in the Yangtze river delta region

Chemical composition and seasonal variations of PM2.5 in an urban environment in Kunming, SW China: Importance of prevailing westerlies in cold season

Examining the effects of socioeconomic development on fine particulate matter (PM2.5) in China's cities using spatial regression and the geographical detector technique

The influential factors of urban PM2.5 concentrations in China: A spatial econometric analysis

Vehicle emission trends and spatial distribution in Shandong province

Chemical Characterization and Source Apportionment of PM2.5 during Spring and Winter in the Yangtze River Delta

A highly resolved temporal and spatial air pollutant emission inventory for the Pearl River Delta region, China and its uncertainty assessment

Trends in China's anthropogenic emissions since 2010 as the consequence of clean air actions

Anthropogenic factors of PM2.5 distributions in China's major urban agglomerations: A spatial-temporal analysis

Proximate determinants of particulate matter (PM2.5) emission, mortality and life expectancy in Europe, Central Asia, Australia, Canada and the US

Atmospheric pollution assessment near potential source of natural aerosols in the South Gobi Desert region

We are sincerely appreciated Baidu for mobility data provision and the anonymous reviewers for their excellent comments and efforts.

The authors declare no conflict of interest.