id	sid	tid	token	lemma	pos
xk81jh37c5q	1	1	the	the	DET
xk81jh37c5q	1	2	continued	continue	VERB
xk81jh37c5q	1	3	environmental	environmental	ADJ
xk81jh37c5q	1	4	,	,	PUNCT
xk81jh37c5q	1	5	technological	technological	ADJ
xk81jh37c5q	1	6	,	,	PUNCT
xk81jh37c5q	1	7	and	and	CCONJ
xk81jh37c5q	1	8	industrial	industrial	ADJ
xk81jh37c5q	1	9	importance	importance	NOUN
xk81jh37c5q	1	10	of	of	ADP
xk81jh37c5q	1	11	actinide	actinide	ADJ
xk81jh37c5q	1	12	materials	material	NOUN
xk81jh37c5q	1	13	sustains	sustain	VERB
xk81jh37c5q	1	14	the	the	DET
xk81jh37c5q	1	15	need	need	NOUN
xk81jh37c5q	1	16	for	for	ADP
xk81jh37c5q	1	17	understanding	understand	VERB
xk81jh37c5q	1	18	their	their	PRON
xk81jh37c5q	1	19	behavior	behavior	NOUN
xk81jh37c5q	1	20	from	from	ADP
xk81jh37c5q	1	21	the	the	DET
xk81jh37c5q	1	22	nanoscale	nanoscale	NOUN
xk81jh37c5q	1	23	to	to	PART
xk81jh37c5q	1	24	macroscale	macroscale	VERB
xk81jh37c5q	1	25	.	.	PUNCT
xk81jh37c5q	2	1	understanding	understand	VERB
xk81jh37c5q	2	2	the	the	DET
xk81jh37c5q	2	3	physical	physical	ADJ
xk81jh37c5q	2	4	and	and	CCONJ
xk81jh37c5q	2	5	chemical	chemical	NOUN
xk81jh37c5q	2	6	properties	property	NOUN
xk81jh37c5q	2	7	of	of	ADP
xk81jh37c5q	2	8	actinides	actinide	NOUN
xk81jh37c5q	2	9	is	be	AUX
xk81jh37c5q	2	10	a	a	DET
xk81jh37c5q	2	11	necessary	necessary	ADJ
xk81jh37c5q	2	12	step	step	NOUN
xk81jh37c5q	2	13	towards	towards	ADP
xk81jh37c5q	2	14	predicting	predict	VERB
xk81jh37c5q	2	15	their	their	PRON
xk81jh37c5q	2	16	longand	longand	PROPN
xk81jh37c5q	2	17	short	short	ADJ
xk81jh37c5q	2	18	-	-	PUNCT
xk81jh37c5q	2	19	term	term	NOUN
xk81jh37c5q	2	20	behavior	behavior	NOUN
xk81jh37c5q	2	21	in	in	ADP
xk81jh37c5q	2	22	different	different	ADJ
xk81jh37c5q	2	23	environments	environment	NOUN
xk81jh37c5q	2	24	.	.	PUNCT
xk81jh37c5q	3	1	determination	determination	NOUN
xk81jh37c5q	3	2	of	of	ADP
xk81jh37c5q	3	3	thermodynamic	thermodynamic	ADJ
xk81jh37c5q	3	4	properties	property	NOUN
xk81jh37c5q	3	5	of	of	ADP
xk81jh37c5q	3	6	uranium	uranium	NOUN
xk81jh37c5q	3	7	minerals	mineral	NOUN
xk81jh37c5q	3	8	and	and	CCONJ
xk81jh37c5q	3	9	associated	associated	ADJ
xk81jh37c5q	3	10	compounds	compound	NOUN
xk81jh37c5q	3	11	is	be	AUX
xk81jh37c5q	3	12	fundamental	fundamental	ADJ
xk81jh37c5q	3	13	for	for	ADP
xk81jh37c5q	3	14	understanding	understand	VERB
xk81jh37c5q	3	15	the	the	DET
xk81jh37c5q	3	16	alteration	alteration	NOUN
xk81jh37c5q	3	17	pathways	pathway	NOUN
xk81jh37c5q	3	18	of	of	ADP
xk81jh37c5q	3	19	uranium	uranium	NOUN
xk81jh37c5q	3	20	in	in	ADP
xk81jh37c5q	3	21	geological	geological	ADJ
xk81jh37c5q	3	22	systems	system	NOUN
xk81jh37c5q	3	23	,	,	PUNCT
xk81jh37c5q	3	24	predicting	predict	VERB
xk81jh37c5q	3	25	transport	transport	NOUN
xk81jh37c5q	3	26	of	of	ADP
xk81jh37c5q	3	27	uranium	uranium	NOUN
xk81jh37c5q	3	28	in	in	ADP
xk81jh37c5q	3	29	the	the	DET
xk81jh37c5q	3	30	environment	environment	NOUN
xk81jh37c5q	3	31	,	,	PUNCT
xk81jh37c5q	3	32	and	and	CCONJ
xk81jh37c5q	3	33	ultimately	ultimately	ADV
xk81jh37c5q	3	34	developing	develop	VERB
xk81jh37c5q	3	35	a	a	DET
xk81jh37c5q	3	36	geologic	geologic	ADJ
xk81jh37c5q	3	37	repository	repository	NOUN
xk81jh37c5q	3	38	for	for	ADP
xk81jh37c5q	3	39	spent	spend	VERB
xk81jh37c5q	3	40	nuclear	nuclear	ADJ
xk81jh37c5q	3	41	fuel	fuel	NOUN
xk81jh37c5q	3	42	in	in	ADP
xk81jh37c5q	3	43	the	the	DET
xk81jh37c5q	3	44	us	us	PROPN
xk81jh37c5q	3	45	.	.	PUNCT
xk81jh37c5q	4	1	towards	towards	ADP
xk81jh37c5q	4	2	this	this	DET
xk81jh37c5q	4	3	end	end	NOUN
xk81jh37c5q	4	4	,	,	PUNCT
xk81jh37c5q	4	5	i	i	PRON
xk81jh37c5q	4	6	focus	focus	VERB
xk81jh37c5q	4	7	on	on	ADP
xk81jh37c5q	4	8	experimentally	experimentally	ADV
xk81jh37c5q	4	9	determining	determine	VERB
xk81jh37c5q	4	10	the	the	DET
xk81jh37c5q	4	11	thermodynamic	thermodynamic	ADJ
xk81jh37c5q	4	12	properties	property	NOUN
xk81jh37c5q	4	13	of	of	ADP
xk81jh37c5q	4	14	uranyl	uranyl	ADJ
xk81jh37c5q	4	15	compounds	compound	NOUN
xk81jh37c5q	4	16	in	in	ADP
xk81jh37c5q	4	17	this	this	PRON
xk81jh37c5q	4	18	research.the	research.the	DET
xk81jh37c5q	4	19	work	work	NOUN
xk81jh37c5q	4	20	described	describe	VERB
xk81jh37c5q	4	21	in	in	ADP
xk81jh37c5q	4	22	this	this	DET
xk81jh37c5q	4	23	dissertation	dissertation	NOUN
xk81jh37c5q	4	24	explores	explore	VERB
xk81jh37c5q	4	25	two	two	NUM
xk81jh37c5q	4	26	major	major	ADJ
xk81jh37c5q	4	27	topics	topic	NOUN
xk81jh37c5q	4	28	in	in	ADP
xk81jh37c5q	4	29	actinide	actinide	ADJ
xk81jh37c5q	4	30	geochemistry	geochemistry	NOUN
xk81jh37c5q	4	31	.	.	PUNCT
xk81jh37c5q	5	1	the	the	DET
xk81jh37c5q	5	2	first	first	ADJ
xk81jh37c5q	5	3	theme	theme	NOUN
xk81jh37c5q	5	4	is	be	AUX
xk81jh37c5q	5	5	focused	focus	VERB
xk81jh37c5q	5	6	on	on	ADP
xk81jh37c5q	5	7	determination	determination	NOUN
xk81jh37c5q	5	8	of	of	ADP
xk81jh37c5q	5	9	standard	standard	ADJ
xk81jh37c5q	5	10	-	-	PUNCT
xk81jh37c5q	5	11	state	state	NOUN
xk81jh37c5q	5	12	thermodynamic	thermodynamic	ADJ
xk81jh37c5q	5	13	properties	property	NOUN
xk81jh37c5q	5	14	of	of	ADP
xk81jh37c5q	5	15	the	the	DET
xk81jh37c5q	5	16	zippeite	zippeite	ADJ
xk81jh37c5q	5	17	-	-	PUNCT
xk81jh37c5q	5	18	group	group	NOUN
xk81jh37c5q	5	19	minerals	mineral	NOUN
xk81jh37c5q	5	20	from	from	ADP
xk81jh37c5q	5	21	the	the	DET
xk81jh37c5q	5	22	uranyl	uranyl	ADJ
xk81jh37c5q	5	23	sulfate	sulfate	NOUN
xk81jh37c5q	5	24	family	family	NOUN
xk81jh37c5q	5	25	that	that	PRON
xk81jh37c5q	5	26	form	form	NOUN
xk81jh37c5q	5	27	on	on	ADP
xk81jh37c5q	5	28	uranium	uranium	NOUN
xk81jh37c5q	5	29	mine	mine	NOUN
xk81jh37c5q	5	30	wastes	waste	NOUN
xk81jh37c5q	5	31	and	and	CCONJ
xk81jh37c5q	5	32	that	that	PRON
xk81jh37c5q	5	33	may	may	AUX
xk81jh37c5q	5	34	be	be	AUX
xk81jh37c5q	5	35	important	important	ADJ
xk81jh37c5q	5	36	in	in	ADP
xk81jh37c5q	5	37	nuclear	nuclear	ADJ
xk81jh37c5q	5	38	waste	waste	NOUN
xk81jh37c5q	5	39	disposal	disposal	PROPN
xk81jh37c5q	5	40	.	.	PUNCT
xk81jh37c5q	6	1	the	the	DET
xk81jh37c5q	6	2	result	result	NOUN
xk81jh37c5q	6	3	of	of	ADP
xk81jh37c5q	6	4	the	the	DET
xk81jh37c5q	6	5	experimental	experimental	ADJ
xk81jh37c5q	6	6	thermochemistry	thermochemistry	NOUN
xk81jh37c5q	6	7	of	of	ADP
xk81jh37c5q	6	8	four	four	NUM
xk81jh37c5q	6	9	members	member	NOUN
xk81jh37c5q	6	10	of	of	ADP
xk81jh37c5q	6	11	the	the	DET
xk81jh37c5q	6	12	zippeite	zippeite	PROPN
xk81jh37c5q	6	13	group	group	NOUN
xk81jh37c5q	6	14	with	with	ADP
xk81jh37c5q	6	15	zippeite	zippeite	ADJ
xk81jh37c5q	6	16	-	-	PUNCT
xk81jh37c5q	6	17	type	type	NOUN
xk81jh37c5q	6	18	uranyl	uranyl	NOUN
xk81jh37c5q	6	19	sulfate	sulfate	NOUN
xk81jh37c5q	6	20	sheets	sheet	NOUN
xk81jh37c5q	6	21	and	and	CCONJ
xk81jh37c5q	6	22	different	different	ADJ
xk81jh37c5q	6	23	interlayer	interlayer	NOUN
xk81jh37c5q	6	24	cations	cation	NOUN
xk81jh37c5q	6	25	is	be	AUX
xk81jh37c5q	6	26	presented	present	VERB
xk81jh37c5q	6	27	in	in	ADP
xk81jh37c5q	6	28	this	this	DET
xk81jh37c5q	6	29	work	work	NOUN
xk81jh37c5q	6	30	.	.	PUNCT
xk81jh37c5q	7	1	pure	pure	ADJ
xk81jh37c5q	7	2	zippeite	zippeite	NOUN
xk81jh37c5q	7	3	,	,	PUNCT
xk81jh37c5q	7	4	natrozippeite	natrozippeite	PROPN
xk81jh37c5q	7	5	,	,	PUNCT
xk81jh37c5q	7	6	cobaltzippeite	cobaltzippeite	PROPN
xk81jh37c5q	7	7	,	,	PUNCT
xk81jh37c5q	7	8	and	and	CCONJ
xk81jh37c5q	7	9	zinczippeite	zinczippeite	PROPN
xk81jh37c5q	7	10	mineral	mineral	NOUN
xk81jh37c5q	7	11	analogs	analog	NOUN
xk81jh37c5q	7	12	were	be	AUX
xk81jh37c5q	7	13	hydrothermally	hydrothermally	ADV
xk81jh37c5q	7	14	synthesized	synthesize	VERB
xk81jh37c5q	7	15	and	and	CCONJ
xk81jh37c5q	7	16	thoroughly	thoroughly	ADV
xk81jh37c5q	7	17	characterized	characterize	VERB
xk81jh37c5q	7	18	using	use	VERB
xk81jh37c5q	7	19	x	x	NOUN
xk81jh37c5q	7	20	-	-	NOUN
xk81jh37c5q	7	21	ray	ray	NOUN
xk81jh37c5q	7	22	diffraction	diffraction	NOUN
xk81jh37c5q	7	23	and	and	CCONJ
xk81jh37c5q	7	24	analytical	analytical	ADJ
xk81jh37c5q	7	25	chemistry	chemistry	NOUN
xk81jh37c5q	7	26	methods	method	NOUN
xk81jh37c5q	7	27	(	(	PUNCT
xk81jh37c5q	7	28	icp	icp	PROPN
xk81jh37c5q	7	29	-	-	PUNCT
xk81jh37c5q	7	30	oes	oes	PROPN
xk81jh37c5q	7	31	,	,	PUNCT
xk81jh37c5q	7	32	tga	tga	PROPN
xk81jh37c5q	7	33	)	)	PUNCT
xk81jh37c5q	7	34	.	.	PUNCT
xk81jh37c5q	8	1	the	the	DET
xk81jh37c5q	8	2	standard	standard	ADJ
xk81jh37c5q	8	3	-	-	PUNCT
xk81jh37c5q	8	4	state	state	NOUN
xk81jh37c5q	8	5	enthalpy	enthalpy	NOUN
xk81jh37c5q	8	6	of	of	ADP
xk81jh37c5q	8	7	formation	formation	NOUN
xk81jh37c5q	8	8	of	of	ADP
xk81jh37c5q	8	9	each	each	DET
xk81jh37c5q	8	10	sample	sample	NOUN
xk81jh37c5q	8	11	was	be	AUX
xk81jh37c5q	8	12	determined	determine	VERB
xk81jh37c5q	8	13	using	use	VERB
xk81jh37c5q	8	14	high	high	ADJ
xk81jh37c5q	8	15	-	-	PUNCT
xk81jh37c5q	8	16	temperature	temperature	NOUN
xk81jh37c5q	8	17	calorimetry	calorimetry	NOUN
xk81jh37c5q	8	18	.	.	PUNCT
xk81jh37c5q	9	1	solubility	solubility	NOUN
xk81jh37c5q	9	2	experiments	experiment	NOUN
xk81jh37c5q	9	3	were	be	AUX
xk81jh37c5q	9	4	carried	carry	VERB
xk81jh37c5q	9	5	out	out	ADP
xk81jh37c5q	9	6	for	for	ADP
xk81jh37c5q	9	7	zippeite	zippeite	PROPN
xk81jh37c5q	9	8	to	to	PART
xk81jh37c5q	9	9	measure	measure	VERB
xk81jh37c5q	9	10	it	it	PRON
xk81jh37c5q	9	11	solubility	solubility	NOUN
xk81jh37c5q	9	12	product	product	NOUN
xk81jh37c5q	9	13	and	and	CCONJ
xk81jh37c5q	9	14	hence	hence	ADV
xk81jh37c5q	9	15	calculate	calculate	VERB
xk81jh37c5q	9	16	its	its	PRON
xk81jh37c5q	9	17	standard	standard	ADJ
xk81jh37c5q	9	18	state	state	NOUN
xk81jh37c5q	9	19	gibbs	gibbs	PROPN
xk81jh37c5q	9	20	free	free	ADJ
xk81jh37c5q	9	21	energy	energy	NOUN
xk81jh37c5q	9	22	of	of	ADP
xk81jh37c5q	9	23	formation	formation	NOUN
xk81jh37c5q	9	24	.	.	PUNCT
xk81jh37c5q	10	1	calorimetric	calorimetric	ADJ
xk81jh37c5q	10	2	data	datum	NOUN
xk81jh37c5q	10	3	revealed	reveal	VERB
xk81jh37c5q	10	4	that	that	SCONJ
xk81jh37c5q	10	5	there	there	PRON
xk81jh37c5q	10	6	is	be	VERB
xk81jh37c5q	10	7	a	a	DET
xk81jh37c5q	10	8	linear	linear	ADJ
xk81jh37c5q	10	9	relationship	relationship	NOUN
xk81jh37c5q	10	10	between	between	ADP
xk81jh37c5q	10	11	the	the	DET
xk81jh37c5q	10	12	formation	formation	NOUN
xk81jh37c5q	10	13	enthalpies	enthalpy	NOUN
xk81jh37c5q	10	14	from	from	ADP
xk81jh37c5q	10	15	oxides	oxide	NOUN
xk81jh37c5q	10	16	and	and	CCONJ
xk81jh37c5q	10	17	the	the	DET
xk81jh37c5q	10	18	acidity	acidity	NOUN
xk81jh37c5q	10	19	of	of	ADP
xk81jh37c5q	10	20	cation	cation	NOUN
xk81jh37c5q	10	21	oxides	oxide	NOUN
xk81jh37c5q	10	22	,	,	PUNCT
xk81jh37c5q	10	23	as	as	ADV
xk81jh37c5q	10	24	well	well	ADV
xk81jh37c5q	10	25	as	as	ADP
xk81jh37c5q	10	26	the	the	DET
xk81jh37c5q	10	27	ionic	ionic	ADJ
xk81jh37c5q	10	28	radius	radius	NOUN
xk81jh37c5q	10	29	of	of	ADP
xk81jh37c5q	10	30	charge	charge	NOUN
xk81jh37c5q	10	31	-	-	PUNCT
xk81jh37c5q	10	32	balancing	balance	VERB
xk81jh37c5q	10	33	alkalis	alkali	NOUN
xk81jh37c5q	10	34	,	,	PUNCT
xk81jh37c5q	10	35	indicating	indicate	VERB
xk81jh37c5q	10	36	the	the	DET
xk81jh37c5q	10	37	importance	importance	NOUN
xk81jh37c5q	10	38	of	of	ADP
xk81jh37c5q	10	39	the	the	DET
xk81jh37c5q	10	40	nature	nature	NOUN
xk81jh37c5q	10	41	and	and	CCONJ
xk81jh37c5q	10	42	coordination	coordination	NOUN
xk81jh37c5q	10	43	environment	environment	NOUN
xk81jh37c5q	10	44	of	of	ADP
xk81jh37c5q	10	45	the	the	DET
xk81jh37c5q	10	46	interstitial	interstitial	ADJ
xk81jh37c5q	10	47	complex	complex	NOUN
xk81jh37c5q	10	48	in	in	ADP
xk81jh37c5q	10	49	determining	determine	VERB
xk81jh37c5q	10	50	the	the	DET
xk81jh37c5q	10	51	thermodynamic	thermodynamic	ADJ
xk81jh37c5q	10	52	properties	property	NOUN
xk81jh37c5q	10	53	of	of	ADP
xk81jh37c5q	10	54	these	these	DET
xk81jh37c5q	10	55	minerals.in	minerals.in	NUM
xk81jh37c5q	10	56	the	the	DET
xk81jh37c5q	10	57	second	second	ADJ
xk81jh37c5q	10	58	component	component	NOUN
xk81jh37c5q	10	59	of	of	ADP
xk81jh37c5q	10	60	this	this	DET
xk81jh37c5q	10	61	work	work	NOUN
xk81jh37c5q	10	62	,	,	PUNCT
xk81jh37c5q	10	63	i	i	PRON
xk81jh37c5q	10	64	studied	study	VERB
xk81jh37c5q	10	65	the	the	DET
xk81jh37c5q	10	66	chemical	chemical	NOUN
xk81jh37c5q	10	67	thermodynamics	thermodynamic	NOUN
xk81jh37c5q	10	68	of	of	ADP
xk81jh37c5q	10	69	selected	select	VERB
xk81jh37c5q	10	70	members	member	NOUN
xk81jh37c5q	10	71	of	of	ADP
xk81jh37c5q	10	72	the	the	DET
xk81jh37c5q	10	73	family	family	NOUN
xk81jh37c5q	10	74	of	of	ADP
xk81jh37c5q	10	75	nanoscale	nanoscale	ADJ
xk81jh37c5q	10	76	uranyl	uranyl	ADJ
xk81jh37c5q	10	77	peroxide	peroxide	NOUN
xk81jh37c5q	10	78	cage	cage	NOUN
xk81jh37c5q	10	79	clusters	cluster	NOUN
xk81jh37c5q	10	80	.	.	PUNCT
xk81jh37c5q	11	1	uranyl	uranyl	NOUN
xk81jh37c5q	11	2	nanoclusters	nanocluster	NOUN
xk81jh37c5q	11	3	,	,	PUNCT
xk81jh37c5q	11	4	that	that	PRON
xk81jh37c5q	11	5	are	be	AUX
xk81jh37c5q	11	6	proposed	propose	VERB
xk81jh37c5q	11	7	to	to	PART
xk81jh37c5q	11	8	be	be	AUX
xk81jh37c5q	11	9	energetic	energetic	ADJ
xk81jh37c5q	11	10	intermediates	intermediate	NOUN
xk81jh37c5q	11	11	between	between	ADP
xk81jh37c5q	11	12	dissolved	dissolve	VERB
xk81jh37c5q	11	13	aqueous	aqueous	ADJ
xk81jh37c5q	11	14	uranyl	uranyl	NOUN
xk81jh37c5q	11	15	species	specie	NOUN
xk81jh37c5q	11	16	and	and	CCONJ
xk81jh37c5q	11	17	uranyl	uranyl	NOUN
xk81jh37c5q	11	18	minerals	mineral	NOUN
xk81jh37c5q	11	19	,	,	PUNCT
xk81jh37c5q	11	20	have	have	VERB
xk81jh37c5q	11	21	potential	potential	ADJ
xk81jh37c5q	11	22	importance	importance	NOUN
xk81jh37c5q	11	23	in	in	ADP
xk81jh37c5q	11	24	an	an	DET
xk81jh37c5q	11	25	advanced	advanced	ADJ
xk81jh37c5q	11	26	nuclear	nuclear	ADJ
xk81jh37c5q	11	27	fuel	fuel	NOUN
xk81jh37c5q	11	28	cycle	cycle	NOUN
xk81jh37c5q	11	29	and	and	CCONJ
xk81jh37c5q	11	30	environmental	environmental	ADJ
xk81jh37c5q	11	31	transport	transport	NOUN
xk81jh37c5q	11	32	of	of	ADP
xk81jh37c5q	11	33	actinides	actinide	NOUN
xk81jh37c5q	11	34	following	follow	VERB
xk81jh37c5q	11	35	nuclear	nuclear	ADJ
xk81jh37c5q	11	36	accidents	accident	NOUN
xk81jh37c5q	11	37	.	.	PUNCT
xk81jh37c5q	12	1	their	their	PRON
xk81jh37c5q	12	2	structures	structure	NOUN
xk81jh37c5q	12	3	are	be	AUX
xk81jh37c5q	12	4	composed	compose	VERB
xk81jh37c5q	12	5	of	of	ADP
xk81jh37c5q	12	6	uranyl	uranyl	ADJ
xk81jh37c5q	12	7	polyhedra	polyhedron	NOUN
xk81jh37c5q	12	8	bridged	bridge	VERB
xk81jh37c5q	12	9	by	by	ADP
xk81jh37c5q	12	10	bidentate	bidentate	ADJ
xk81jh37c5q	12	11	peroxide	peroxide	NOUN
xk81jh37c5q	12	12	,	,	PUNCT
xk81jh37c5q	12	13	and	and	CCONJ
xk81jh37c5q	12	14	other	other	ADJ
xk81jh37c5q	12	15	types	type	NOUN
xk81jh37c5q	12	16	of	of	ADP
xk81jh37c5q	12	17	bridges	bridge	NOUN
xk81jh37c5q	12	18	in	in	ADP
xk81jh37c5q	12	19	addition	addition	NOUN
xk81jh37c5q	12	20	to	to	ADP
xk81jh37c5q	12	21	peroxide	peroxide	NOUN
xk81jh37c5q	12	22	ligands	ligand	NOUN
xk81jh37c5q	12	23	in	in	ADP
xk81jh37c5q	12	24	many	many	ADJ
xk81jh37c5q	12	25	cases	case	NOUN
xk81jh37c5q	12	26	,	,	PUNCT
xk81jh37c5q	12	27	that	that	PRON
xk81jh37c5q	12	28	are	be	AUX
xk81jh37c5q	12	29	charge	charge	NOUN
xk81jh37c5q	12	30	-	-	PUNCT
xk81jh37c5q	12	31	balanced	balance	VERB
xk81jh37c5q	12	32	by	by	ADP
xk81jh37c5q	12	33	metal	metal	NOUN
xk81jh37c5q	12	34	cations	cation	NOUN
xk81jh37c5q	12	35	.	.	PUNCT
xk81jh37c5q	13	1	six	six	NUM
xk81jh37c5q	13	2	members	member	NOUN
xk81jh37c5q	13	3	of	of	ADP
xk81jh37c5q	13	4	this	this	DET
xk81jh37c5q	13	5	family	family	NOUN
xk81jh37c5q	13	6	were	be	AUX
xk81jh37c5q	13	7	selected	select	VERB
xk81jh37c5q	13	8	,	,	PUNCT
xk81jh37c5q	13	9	synthesized	synthesize	VERB
xk81jh37c5q	13	10	under	under	ADP
xk81jh37c5q	13	11	ambient	ambient	ADJ
xk81jh37c5q	13	12	conditions	condition	NOUN
xk81jh37c5q	13	13	,	,	PUNCT
xk81jh37c5q	13	14	and	and	CCONJ
xk81jh37c5q	13	15	well	well	ADV
xk81jh37c5q	13	16	-	-	PUNCT
xk81jh37c5q	13	17	characterized	characterize	VERB
xk81jh37c5q	13	18	using	use	VERB
xk81jh37c5q	13	19	single	single	ADJ
xk81jh37c5q	13	20	crystal	crystal	NOUN
xk81jh37c5q	13	21	x	x	NOUN
xk81jh37c5q	13	22	-	-	NOUN
xk81jh37c5q	13	23	ray	ray	NOUN
xk81jh37c5q	13	24	diffraction	diffraction	NOUN
xk81jh37c5q	13	25	,	,	PUNCT
xk81jh37c5q	13	26	icp	icp	PROPN
xk81jh37c5q	13	27	-	-	PUNCT
xk81jh37c5q	13	28	oes	oes	PROPN
xk81jh37c5q	13	29	,	,	PUNCT
xk81jh37c5q	13	30	esi	esi	PROPN
xk81jh37c5q	13	31	-	-	PROPN
xk81jh37c5q	13	32	ms	ms	PROPN
xk81jh37c5q	13	33	,	,	PUNCT
xk81jh37c5q	13	34	and	and	CCONJ
xk81jh37c5q	13	35	tga	tga	PROPN
xk81jh37c5q	13	36	.	.	PUNCT
xk81jh37c5q	14	1	our	our	PRON
xk81jh37c5q	14	2	calorimetric	calorimetric	ADJ
xk81jh37c5q	14	3	data	datum	NOUN
xk81jh37c5q	14	4	shows	show	VERB
xk81jh37c5q	14	5	that	that	SCONJ
xk81jh37c5q	14	6	the	the	DET
xk81jh37c5q	14	7	enthalpies	enthalpy	NOUN
xk81jh37c5q	14	8	of	of	ADP
xk81jh37c5q	14	9	formation	formation	NOUN
xk81jh37c5q	14	10	of	of	ADP
xk81jh37c5q	14	11	the	the	DET
xk81jh37c5q	14	12	cluster	cluster	NOUN
xk81jh37c5q	14	13	compounds	compound	VERB
xk81jh37c5q	14	14	from	from	ADP
xk81jh37c5q	14	15	oxides	oxide	NOUN
xk81jh37c5q	14	16	become	become	VERB
xk81jh37c5q	14	17	more	more	ADV
xk81jh37c5q	14	18	negative	negative	ADJ
xk81jh37c5q	14	19	as	as	ADP
xk81jh37c5q	14	20	the	the	DET
xk81jh37c5q	14	21	charge	charge	NOUN
xk81jh37c5q	14	22	on	on	ADP
xk81jh37c5q	14	23	the	the	DET
xk81jh37c5q	14	24	cluster	cluster	NOUN
xk81jh37c5q	14	25	increases	increase	NOUN
xk81jh37c5q	14	26	.	.	PUNCT
xk81jh37c5q	15	1	the	the	DET
xk81jh37c5q	15	2	results	result	NOUN
xk81jh37c5q	15	3	obtained	obtain	VERB
xk81jh37c5q	15	4	from	from	ADP
xk81jh37c5q	15	5	this	this	DET
xk81jh37c5q	15	6	work	work	NOUN
xk81jh37c5q	15	7	demonstrate	demonstrate	VERB
xk81jh37c5q	15	8	that	that	SCONJ
xk81jh37c5q	15	9	the	the	DET
xk81jh37c5q	15	10	energetics	energetic	NOUN
xk81jh37c5q	15	11	of	of	ADP
xk81jh37c5q	15	12	uranyl	uranyl	ADJ
xk81jh37c5q	15	13	peroxide	peroxide	NOUN
xk81jh37c5q	15	14	cluster	cluster	NOUN
xk81jh37c5q	15	15	crystals	crystal	NOUN
xk81jh37c5q	15	16	are	be	AUX
xk81jh37c5q	15	17	largely	largely	ADV
xk81jh37c5q	15	18	driven	drive	VERB
xk81jh37c5q	15	19	by	by	ADP
xk81jh37c5q	15	20	the	the	DET
xk81jh37c5q	15	21	alkali	alkali	ADJ
xk81jh37c5q	15	22	cation	cation	NOUN
xk81jh37c5q	15	23	oxide	oxide	NOUN
xk81jh37c5q	15	24	thermodynamics	thermodynamic	NOUN
xk81jh37c5q	15	25	,	,	PUNCT
xk81jh37c5q	15	26	rather	rather	ADV
xk81jh37c5q	15	27	than	than	ADP
xk81jh37c5q	15	28	negatively	negatively	ADV
xk81jh37c5q	15	29	charged	charge	VERB
xk81jh37c5q	15	30	uranyl	uranyl	NOUN
xk81jh37c5q	15	31	cages.the	cages.the	DET
xk81jh37c5q	15	32	data	datum	NOUN
xk81jh37c5q	15	33	obtained	obtain	VERB
xk81jh37c5q	15	34	from	from	ADP
xk81jh37c5q	15	35	this	this	DET
xk81jh37c5q	15	36	work	work	NOUN
xk81jh37c5q	15	37	proposes	propose	VERB
xk81jh37c5q	15	38	trends	trend	NOUN
xk81jh37c5q	15	39	between	between	ADP
xk81jh37c5q	15	40	enthalpies	enthalpy	NOUN
xk81jh37c5q	15	41	of	of	ADP
xk81jh37c5q	15	42	formation	formation	NOUN
xk81jh37c5q	15	43	of	of	ADP
xk81jh37c5q	15	44	select	select	ADJ
xk81jh37c5q	15	45	uranyl	uranyl	NOUN
xk81jh37c5q	15	46	phases	phase	NOUN
xk81jh37c5q	15	47	and	and	CCONJ
xk81jh37c5q	15	48	their	their	PRON
xk81jh37c5q	15	49	chemical	chemical	NOUN
xk81jh37c5q	15	50	properties	property	NOUN
xk81jh37c5q	15	51	related	relate	VERB
xk81jh37c5q	15	52	to	to	ADP
xk81jh37c5q	15	53	their	their	PRON
xk81jh37c5q	15	54	crystal	crystal	NOUN
xk81jh37c5q	15	55	structure	structure	NOUN
xk81jh37c5q	15	56	.	.	PUNCT
xk81jh37c5q	16	1	the	the	DET
xk81jh37c5q	16	2	findings	finding	NOUN
xk81jh37c5q	16	3	may	may	AUX
xk81jh37c5q	16	4	be	be	AUX
xk81jh37c5q	16	5	used	use	VERB
xk81jh37c5q	16	6	to	to	PART
xk81jh37c5q	16	7	predict	predict	VERB
xk81jh37c5q	16	8	the	the	DET
xk81jh37c5q	16	9	energetics	energetic	NOUN
xk81jh37c5q	16	10	of	of	ADP
xk81jh37c5q	16	11	other	other	ADJ
xk81jh37c5q	16	12	members	member	NOUN
xk81jh37c5q	16	13	of	of	ADP
xk81jh37c5q	16	14	that	that	DET
xk81jh37c5q	16	15	family	family	NOUN
xk81jh37c5q	16	16	,	,	PUNCT
xk81jh37c5q	16	17	or	or	CCONJ
xk81jh37c5q	16	18	on	on	ADP
xk81jh37c5q	16	19	a	a	DET
xk81jh37c5q	16	20	larger	large	ADJ
xk81jh37c5q	16	21	scale	scale	NOUN
xk81jh37c5q	16	22	to	to	PART
xk81jh37c5q	16	23	better	well	ADV
xk81jh37c5q	16	24	understand	understand	VERB
xk81jh37c5q	16	25	and	and	CCONJ
xk81jh37c5q	16	26	improve	improve	VERB
xk81jh37c5q	16	27	the	the	DET
xk81jh37c5q	16	28	nuclear	nuclear	ADJ
xk81jh37c5q	16	29	fuel	fuel	NOUN
xk81jh37c5q	16	30	cycle	cycle	NOUN
xk81jh37c5q	16	31	.	.	PUNCT