id	sid	tid	token	lemma	pos
nz805x2515r	1	1	the	the	DET
nz805x2515r	1	2	actinides	actinide	NOUN
nz805x2515r	1	3	are	be	AUX
nz805x2515r	1	4	a	a	DET
nz805x2515r	1	5	series	series	NOUN
nz805x2515r	1	6	of	of	ADP
nz805x2515r	1	7	f	f	PROPN
nz805x2515r	1	8	-	-	PUNCT
nz805x2515r	1	9	block	block	NOUN
nz805x2515r	1	10	inner	inner	ADJ
nz805x2515r	1	11	transition	transition	NOUN
nz805x2515r	1	12	metals	metal	NOUN
nz805x2515r	1	13	,	,	PUNCT
nz805x2515r	1	14	and	and	CCONJ
nz805x2515r	1	15	are	be	AUX
nz805x2515r	1	16	primarily	primarily	ADV
nz805x2515r	1	17	used	use	VERB
nz805x2515r	1	18	in	in	ADP
nz805x2515r	1	19	the	the	DET
nz805x2515r	1	20	production	production	NOUN
nz805x2515r	1	21	of	of	ADP
nz805x2515r	1	22	nuclear	nuclear	ADJ
nz805x2515r	1	23	power	power	NOUN
nz805x2515r	1	24	.	.	PUNCT
nz805x2515r	2	1	nuclear	nuclear	ADJ
nz805x2515r	2	2	power	power	NOUN
nz805x2515r	2	3	is	be	AUX
nz805x2515r	2	4	plentiful	plentiful	ADJ
nz805x2515r	2	5	,	,	PUNCT
nz805x2515r	2	6	safe	safe	ADJ
nz805x2515r	2	7	,	,	PUNCT
nz805x2515r	2	8	and	and	CCONJ
nz805x2515r	2	9	does	do	AUX
nz805x2515r	2	10	not	not	PART
nz805x2515r	2	11	involve	involve	VERB
nz805x2515r	2	12	the	the	DET
nz805x2515r	2	13	emission	emission	NOUN
nz805x2515r	2	14	of	of	ADP
nz805x2515r	2	15	toxic	toxic	ADJ
nz805x2515r	2	16	greenhouse	greenhouse	NOUN
nz805x2515r	2	17	gases	gas	NOUN
nz805x2515r	2	18	.	.	PUNCT
nz805x2515r	3	1	therefore	therefore	ADV
nz805x2515r	3	2	,	,	PUNCT
nz805x2515r	3	3	it	it	PRON
nz805x2515r	3	4	has	have	VERB
nz805x2515r	3	5	the	the	DET
nz805x2515r	3	6	potential	potential	NOUN
nz805x2515r	3	7	to	to	PART
nz805x2515r	3	8	be	be	AUX
nz805x2515r	3	9	a	a	DET
nz805x2515r	3	10	transitionary	transitionary	ADJ
nz805x2515r	3	11	fuel	fuel	NOUN
nz805x2515r	3	12	as	as	SCONJ
nz805x2515r	3	13	society	society	NOUN
nz805x2515r	3	14	moves	move	VERB
nz805x2515r	3	15	away	away	ADV
nz805x2515r	3	16	from	from	ADP
nz805x2515r	3	17	the	the	DET
nz805x2515r	3	18	use	use	NOUN
nz805x2515r	3	19	of	of	ADP
nz805x2515r	3	20	nonrenewable	nonrenewable	ADJ
nz805x2515r	3	21	sources	source	NOUN
nz805x2515r	3	22	of	of	ADP
nz805x2515r	3	23	energy	energy	NOUN
nz805x2515r	3	24	.	.	PUNCT
nz805x2515r	4	1	however	however	ADV
nz805x2515r	4	2	,	,	PUNCT
nz805x2515r	4	3	the	the	DET
nz805x2515r	4	4	long	long	ADJ
nz805x2515r	4	5	-	-	PUNCT
nz805x2515r	4	6	term	term	NOUN
nz805x2515r	4	7	fate	fate	NOUN
nz805x2515r	4	8	of	of	ADP
nz805x2515r	4	9	nuclear	nuclear	ADJ
nz805x2515r	4	10	waste	waste	NOUN
nz805x2515r	4	11	is	be	AUX
nz805x2515r	4	12	a	a	DET
nz805x2515r	4	13	major	major	ADJ
nz805x2515r	4	14	concern	concern	NOUN
nz805x2515r	4	15	.	.	PUNCT
nz805x2515r	5	1	knowledge	knowledge	NOUN
nz805x2515r	5	2	of	of	ADP
nz805x2515r	5	3	the	the	DET
nz805x2515r	5	4	solution	solution	NOUN
nz805x2515r	5	5	-	-	PUNCT
nz805x2515r	5	6	phase	phase	NOUN
nz805x2515r	5	7	thermodynamic	thermodynamic	ADJ
nz805x2515r	5	8	behavior	behavior	NOUN
nz805x2515r	5	9	of	of	ADP
nz805x2515r	5	10	actinides	actinide	NOUN
nz805x2515r	5	11	is	be	AUX
nz805x2515r	5	12	essential	essential	ADJ
nz805x2515r	5	13	for	for	ADP
nz805x2515r	5	14	the	the	DET
nz805x2515r	5	15	design	design	NOUN
nz805x2515r	5	16	of	of	ADP
nz805x2515r	5	17	advanced	advanced	ADJ
nz805x2515r	5	18	separation	separation	NOUN
nz805x2515r	5	19	processes	process	NOUN
nz805x2515r	5	20	used	use	VERB
nz805x2515r	5	21	to	to	PART
nz805x2515r	5	22	recycle	recycle	VERB
nz805x2515r	5	23	the	the	DET
nz805x2515r	5	24	fuel	fuel	NOUN
nz805x2515r	5	25	.	.	PUNCT
nz805x2515r	6	1	therefore	therefore	ADV
nz805x2515r	6	2	,	,	PUNCT
nz805x2515r	6	3	it	it	PRON
nz805x2515r	6	4	is	be	AUX
nz805x2515r	6	5	important	important	ADJ
nz805x2515r	6	6	to	to	PART
nz805x2515r	6	7	understand	understand	VERB
nz805x2515r	6	8	and	and	CCONJ
nz805x2515r	6	9	be	be	AUX
nz805x2515r	6	10	able	able	ADJ
nz805x2515r	6	11	to	to	PART
nz805x2515r	6	12	control	control	VERB
nz805x2515r	6	13	actinides	actinide	NOUN
nz805x2515r	6	14	at	at	ADP
nz805x2515r	6	15	the	the	DET
nz805x2515r	6	16	nanoscale.the	nanoscale.the	DET
nz805x2515r	6	17	actinides	actinide	NOUN
nz805x2515r	6	18	are	be	AUX
nz805x2515r	6	19	particularly	particularly	ADV
nz805x2515r	6	20	well	well	ADV
nz805x2515r	6	21	-	-	PUNCT
nz805x2515r	6	22	suited	suited	ADJ
nz805x2515r	6	23	for	for	ADP
nz805x2515r	6	24	molecular	molecular	ADJ
nz805x2515r	6	25	simulation	simulation	NOUN
nz805x2515r	6	26	studies	study	NOUN
nz805x2515r	6	27	.	.	PUNCT
nz805x2515r	7	1	due	due	ADP
nz805x2515r	7	2	to	to	ADP
nz805x2515r	7	3	their	their	PRON
nz805x2515r	7	4	radioactivity	radioactivity	NOUN
nz805x2515r	7	5	,	,	PUNCT
nz805x2515r	7	6	actinides	actinide	NOUN
nz805x2515r	7	7	present	present	VERB
nz805x2515r	7	8	an	an	DET
nz805x2515r	7	9	significant	significant	ADJ
nz805x2515r	7	10	experimental	experimental	ADJ
nz805x2515r	7	11	hazard	hazard	NOUN
nz805x2515r	7	12	.	.	PUNCT
nz805x2515r	8	1	in	in	ADP
nz805x2515r	8	2	addition	addition	NOUN
nz805x2515r	8	3	,	,	PUNCT
nz805x2515r	8	4	thermodynamic	thermodynamic	ADJ
nz805x2515r	8	5	properties	property	NOUN
nz805x2515r	8	6	of	of	ADP
nz805x2515r	8	7	important	important	ADJ
nz805x2515r	8	8	transuranic	transuranic	ADJ
nz805x2515r	8	9	compounds	compound	NOUN
nz805x2515r	8	10	like	like	ADP
nz805x2515r	8	11	neptunium	neptunium	NOUN
nz805x2515r	8	12	and	and	CCONJ
nz805x2515r	8	13	plutonium	plutonium	NOUN
nz805x2515r	8	14	are	be	AUX
nz805x2515r	8	15	relatively	relatively	ADV
nz805x2515r	8	16	scarce	scarce	ADJ
nz805x2515r	8	17	.	.	PUNCT
nz805x2515r	9	1	molecular	molecular	ADJ
nz805x2515r	9	2	simulation	simulation	NOUN
nz805x2515r	9	3	can	can	AUX
nz805x2515r	9	4	help	help	VERB
nz805x2515r	9	5	fill	fill	VERB
nz805x2515r	9	6	in	in	ADP
nz805x2515r	9	7	this	this	DET
nz805x2515r	9	8	data	data	NOUN
nz805x2515r	9	9	gap	gap	NOUN
nz805x2515r	9	10	.	.	PUNCT
nz805x2515r	10	1	finally	finally	ADV
nz805x2515r	10	2	,	,	PUNCT
nz805x2515r	10	3	molecular	molecular	ADJ
nz805x2515r	10	4	simulation	simulation	NOUN
nz805x2515r	10	5	can	can	AUX
nz805x2515r	10	6	provide	provide	VERB
nz805x2515r	10	7	an	an	DET
nz805x2515r	10	8	atomic	atomic	ADJ
nz805x2515r	10	9	-	-	PUNCT
nz805x2515r	10	10	scale	scale	NOUN
nz805x2515r	10	11	understanding	understanding	NOUN
nz805x2515r	10	12	of	of	ADP
nz805x2515r	10	13	a	a	DET
nz805x2515r	10	14	chemical	chemical	NOUN
nz805x2515r	10	15	process	process	NOUN
nz805x2515r	10	16	that	that	PRON
nz805x2515r	10	17	would	would	AUX
nz805x2515r	10	18	difficult	difficult	ADJ
nz805x2515r	10	19	or	or	CCONJ
nz805x2515r	10	20	impossible	impossible	ADJ
nz805x2515r	10	21	to	to	PART
nz805x2515r	10	22	observe	observe	VERB
nz805x2515r	10	23	experimentally	experimentally	ADV
nz805x2515r	10	24	.	.	PUNCT
nz805x2515r	11	1	thermophysical	thermophysical	ADJ
nz805x2515r	11	2	properties	property	NOUN
nz805x2515r	11	3	like	like	ADP
nz805x2515r	11	4	free	free	ADJ
nz805x2515r	11	5	energies	energy	NOUN
nz805x2515r	11	6	,	,	PUNCT
nz805x2515r	11	7	stability	stability	NOUN
nz805x2515r	11	8	constants	constant	NOUN
nz805x2515r	11	9	,	,	PUNCT
nz805x2515r	11	10	and	and	CCONJ
nz805x2515r	11	11	diffusivities	diffusivitie	NOUN
nz805x2515r	11	12	can	can	AUX
nz805x2515r	11	13	be	be	AUX
nz805x2515r	11	14	determined	determine	VERB
nz805x2515r	11	15	from	from	ADP
nz805x2515r	11	16	the	the	DET
nz805x2515r	11	17	simulations.since	simulations.since	NOUN
nz805x2515r	11	18	uo2	uo2	PROPN
nz805x2515r	11	19	and	and	CCONJ
nz805x2515r	11	20	npo2	npo2	PROPN
nz805x2515r	11	21	are	be	AUX
nz805x2515r	11	22	commonly	commonly	ADV
nz805x2515r	11	23	found	find	VERB
nz805x2515r	11	24	species	specie	NOUN
nz805x2515r	11	25	in	in	ADP
nz805x2515r	11	26	the	the	DET
nz805x2515r	11	27	nuclear	nuclear	ADJ
nz805x2515r	11	28	fuel	fuel	NOUN
nz805x2515r	11	29	cycle	cycle	NOUN
nz805x2515r	11	30	,	,	PUNCT
nz805x2515r	11	31	we	we	PRON
nz805x2515r	11	32	first	first	ADV
nz805x2515r	11	33	studied	study	VERB
nz805x2515r	11	34	the	the	DET
nz805x2515r	11	35	complexation	complexation	NOUN
nz805x2515r	11	36	of	of	ADP
nz805x2515r	11	37	these	these	DET
nz805x2515r	11	38	ions	ion	NOUN
nz805x2515r	11	39	with	with	ADP
nz805x2515r	11	40	a	a	DET
nz805x2515r	11	41	variety	variety	NOUN
nz805x2515r	11	42	of	of	ADP
nz805x2515r	11	43	ionic	ionic	ADJ
nz805x2515r	11	44	ligands	ligand	NOUN
nz805x2515r	11	45	.	.	PUNCT
nz805x2515r	12	1	in	in	ADP
nz805x2515r	12	2	the	the	DET
nz805x2515r	12	3	event	event	NOUN
nz805x2515r	12	4	that	that	PRON
nz805x2515r	12	5	nuclear	nuclear	ADJ
nz805x2515r	12	6	waste	waste	NOUN
nz805x2515r	12	7	is	be	AUX
nz805x2515r	12	8	accidentally	accidentally	ADV
nz805x2515r	12	9	discharged	discharge	VERB
nz805x2515r	12	10	into	into	ADP
nz805x2515r	12	11	an	an	DET
nz805x2515r	12	12	aquifer	aquifer	NOUN
nz805x2515r	12	13	,	,	PUNCT
nz805x2515r	12	14	knowledge	knowledge	NOUN
nz805x2515r	12	15	of	of	ADP
nz805x2515r	12	16	the	the	DET
nz805x2515r	12	17	stability	stability	NOUN
nz805x2515r	12	18	of	of	ADP
nz805x2515r	12	19	actinyl	actinyl	PROPN
nz805x2515r	12	20	-	-	PUNCT
nz805x2515r	12	21	ligand	ligand	NOUN
nz805x2515r	12	22	complexes	complex	NOUN
nz805x2515r	12	23	would	would	AUX
nz805x2515r	12	24	be	be	AUX
nz805x2515r	12	25	crucial	crucial	ADJ
nz805x2515r	12	26	.	.	PUNCT
nz805x2515r	13	1	therefore	therefore	ADV
nz805x2515r	13	2	,	,	PUNCT
nz805x2515r	13	3	we	we	PRON
nz805x2515r	13	4	first	first	ADV
nz805x2515r	13	5	used	use	VERB
nz805x2515r	13	6	molecular	molecular	ADJ
nz805x2515r	13	7	dynamics	dynamic	NOUN
nz805x2515r	13	8	simulations	simulation	NOUN
nz805x2515r	13	9	to	to	PART
nz805x2515r	13	10	calculate	calculate	VERB
nz805x2515r	13	11	the	the	DET
nz805x2515r	13	12	potential	potential	NOUN
nz805x2515r	13	13	of	of	ADP
nz805x2515r	13	14	mean	mean	ADJ
nz805x2515r	13	15	force	force	NOUN
nz805x2515r	13	16	between	between	ADP
nz805x2515r	13	17	two	two	NUM
nz805x2515r	13	18	actinyl	actinyl	NOUN
nz805x2515r	13	19	ions	ion	NOUN
nz805x2515r	13	20	(	(	PUNCT
nz805x2515r	13	21	uo2(2	uo2(2	ADV
nz805x2515r	13	22	+	+	PROPN
nz805x2515r	13	23	)	)	PUNCT
nz805x2515r	13	24	and	and	CCONJ
nz805x2515r	13	25	npo2(+	npo2(+	PROPN
nz805x2515r	13	26	)	)	PUNCT
nz805x2515r	13	27	)	)	PUNCT
nz805x2515r	13	28	and	and	CCONJ
nz805x2515r	13	29	various	various	ADJ
nz805x2515r	13	30	ligands	ligand	NOUN
nz805x2515r	13	31	(	(	PUNCT
nz805x2515r	13	32	f-	f-	X
nz805x2515r	13	33	,	,	PUNCT
nz805x2515r	13	34	cl-	cl-	SPACE
nz805x2515r	13	35	,	,	PUNCT
nz805x2515r	13	36	oh-	oh-	SPACE
nz805x2515r	13	37	,	,	PUNCT
nz805x2515r	13	38	no3-	no3-	PROPN
nz805x2515r	13	39	,	,	PUNCT
nz805x2515r	13	40	so4(2-	so4(2-	PROPN
nz805x2515r	13	41	)	)	PUNCT
nz805x2515r	13	42	,	,	PUNCT
nz805x2515r	13	43	co3(2-	co3(2-	PROPN
nz805x2515r	13	44	)	)	PUNCT
nz805x2515r	13	45	,	,	PUNCT
nz805x2515r	13	46	na+	na+	NOUN
nz805x2515r	13	47	,	,	PUNCT
nz805x2515r	13	48	and	and	CCONJ
nz805x2515r	13	49	h2o	h2o	NOUN
nz805x2515r	13	50	)	)	PUNCT
nz805x2515r	13	51	in	in	ADP
nz805x2515r	13	52	explicitly	explicitly	ADV
nz805x2515r	13	53	-	-	PUNCT
nz805x2515r	13	54	modeled	model	VERB
nz805x2515r	13	55	aqueous	aqueous	ADJ
nz805x2515r	13	56	solution	solution	NOUN
nz805x2515r	13	57	.	.	PUNCT
nz805x2515r	14	1	equilibrium	equilibrium	NOUN
nz805x2515r	14	2	constants	constant	NOUN
nz805x2515r	14	3	were	be	AUX
nz805x2515r	14	4	calculated	calculate	VERB
nz805x2515r	14	5	,	,	PUNCT
nz805x2515r	14	6	and	and	CCONJ
nz805x2515r	14	7	are	be	AUX
nz805x2515r	14	8	consistent	consistent	ADJ
nz805x2515r	14	9	with	with	ADP
nz805x2515r	14	10	experimental	experimental	ADJ
nz805x2515r	14	11	trends	trend	NOUN
nz805x2515r	14	12	.	.	PUNCT
nz805x2515r	15	1	dication	dication	NOUN
nz805x2515r	15	2	actinyls	actinyls	ADV
nz805x2515r	15	3	show	show	VERB
nz805x2515r	15	4	stronger	strong	ADJ
nz805x2515r	15	5	affinity	affinity	NOUN
nz805x2515r	15	6	for	for	ADP
nz805x2515r	15	7	anions	anion	NOUN
nz805x2515r	15	8	compared	compare	VERB
nz805x2515r	15	9	to	to	ADP
nz805x2515r	15	10	monocation	monocation	NOUN
nz805x2515r	15	11	actinyls	actinyls	ADV
nz805x2515r	15	12	,	,	PUNCT
nz805x2515r	15	13	whereas	whereas	SCONJ
nz805x2515r	15	14	the	the	DET
nz805x2515r	15	15	opposite	opposite	NOUN
nz805x2515r	15	16	is	be	AUX
nz805x2515r	15	17	true	true	ADJ
nz805x2515r	15	18	for	for	ADP
nz805x2515r	15	19	cation	cation	NOUN
nz805x2515r	15	20	-	-	PUNCT
nz805x2515r	15	21	cation	cation	NOUN
nz805x2515r	15	22	interactions	interaction	NOUN
nz805x2515r	15	23	between	between	ADP
nz805x2515r	15	24	actinyls	actinyls	PROPN
nz805x2515r	15	25	.	.	PUNCT
nz805x2515r	16	1	finally	finally	ADV
nz805x2515r	16	2	,	,	PUNCT
nz805x2515r	16	3	the	the	DET
nz805x2515r	16	4	dynamics	dynamic	NOUN
nz805x2515r	16	5	of	of	ADP
nz805x2515r	16	6	actinyl	actinyl	PROPN
nz805x2515r	16	7	-	-	PUNCT
nz805x2515r	16	8	ligand	ligand	NOUN
nz805x2515r	16	9	contact	contact	NOUN
nz805x2515r	16	10	ion	ion	NOUN
nz805x2515r	16	11	pair	pair	NOUN
nz805x2515r	16	12	dissociation	dissociation	NOUN
nz805x2515r	16	13	were	be	AUX
nz805x2515r	16	14	characterized	characterize	VERB
nz805x2515r	16	15	by	by	ADP
nz805x2515r	16	16	calculating	calculate	VERB
nz805x2515r	16	17	rate	rate	NOUN
nz805x2515r	16	18	constants	constant	NOUN
nz805x2515r	16	19	from	from	ADP
nz805x2515r	16	20	transition	transition	NOUN
nz805x2515r	16	21	state	state	NOUN
nz805x2515r	16	22	theory	theory	NOUN
nz805x2515r	16	23	.	.	PUNCT
nz805x2515r	17	1	the	the	DET
nz805x2515r	17	2	transmission	transmission	NOUN
nz805x2515r	17	3	coefficient	coefficient	NOUN
nz805x2515r	17	4	,	,	PUNCT
nz805x2515r	17	5	a	a	DET
nz805x2515r	17	6	dynamical	dynamical	ADJ
nz805x2515r	17	7	correction	correction	NOUN
nz805x2515r	17	8	factor	factor	NOUN
nz805x2515r	17	9	used	use	VERB
nz805x2515r	17	10	to	to	PART
nz805x2515r	17	11	correct	correct	VERB
nz805x2515r	17	12	for	for	ADP
nz805x2515r	17	13	reaction	reaction	NOUN
nz805x2515r	17	14	barrier	barrier	NOUN
nz805x2515r	17	15	recrossing	recrossing	NOUN
nz805x2515r	17	16	,	,	PUNCT
nz805x2515r	17	17	was	be	AUX
nz805x2515r	17	18	calculated	calculate	VERB
nz805x2515r	17	19	for	for	ADP
nz805x2515r	17	20	each	each	DET
nz805x2515r	17	21	actinyl	actinyl	PROPN
nz805x2515r	17	22	-	-	PUNCT
nz805x2515r	17	23	ligand	ligand	NOUN
nz805x2515r	17	24	dissociation	dissociation	NOUN
nz805x2515r	17	25	event.simple	event.simple	NOUN
nz805x2515r	17	26	actinyl	actinyl	PROPN
nz805x2515r	17	27	ions	ion	NOUN
nz805x2515r	17	28	can	can	AUX
nz805x2515r	17	29	self	self	NOUN
nz805x2515r	17	30	-	-	PUNCT
nz805x2515r	17	31	assemble	assemble	VERB
nz805x2515r	17	32	in	in	ADP
nz805x2515r	17	33	water	water	NOUN
nz805x2515r	17	34	to	to	PART
nz805x2515r	17	35	form	form	VERB
nz805x2515r	17	36	nanoclusters	nanocluster	NOUN
nz805x2515r	17	37	.	.	PUNCT
nz805x2515r	18	1	the	the	DET
nz805x2515r	18	2	nanoclusters	nanocluster	NOUN
nz805x2515r	18	3	are	be	AUX
nz805x2515r	18	4	formed	form	VERB
nz805x2515r	18	5	from	from	ADP
nz805x2515r	18	6	the	the	DET
nz805x2515r	18	7	self	self	NOUN
nz805x2515r	18	8	-	-	PUNCT
nz805x2515r	18	9	assembly	assembly	NOUN
nz805x2515r	18	10	of	of	ADP
nz805x2515r	18	11	uranyl	uranyl	ADJ
nz805x2515r	18	12	ions	ion	NOUN
nz805x2515r	18	13	in	in	ADP
nz805x2515r	18	14	aqueous	aqueous	ADJ
nz805x2515r	18	15	solution	solution	NOUN
nz805x2515r	18	16	and	and	CCONJ
nz805x2515r	18	17	consist	consist	NOUN
nz805x2515r	18	18	of	of	ADP
nz805x2515r	18	19	20	20	NUM
nz805x2515r	18	20	-	-	SYM
nz805x2515r	18	21	124	124	NUM
nz805x2515r	18	22	uranium	uranium	NOUN
nz805x2515r	18	23	polyhedra	polyhedron	NOUN
nz805x2515r	18	24	,	,	PUNCT
nz805x2515r	18	25	with	with	ADP
nz805x2515r	18	26	diameters	diameter	NOUN
nz805x2515r	18	27	ranging	range	VERB
nz805x2515r	18	28	from	from	ADP
nz805x2515r	18	29	1.5	1.5	NUM
nz805x2515r	18	30	to	to	ADP
nz805x2515r	18	31	4.0	4.0	NUM
nz805x2515r	18	32	nm	nm	NOUN
nz805x2515r	18	33	.	.	PUNCT
nz805x2515r	19	1	the	the	DET
nz805x2515r	19	2	nanoclusters	nanocluster	NOUN
nz805x2515r	19	3	carry	carry	VERB
nz805x2515r	19	4	an	an	DET
nz805x2515r	19	5	overall	overall	ADJ
nz805x2515r	19	6	negative	negative	ADJ
nz805x2515r	19	7	charge	charge	NOUN
nz805x2515r	19	8	ranging	range	VERB
nz805x2515r	19	9	from	from	ADP
nz805x2515r	19	10	-20	-20	PROPN
nz805x2515r	19	11	to	to	ADP
nz805x2515r	19	12	-60	-60	NUM
nz805x2515r	19	13	,	,	PUNCT
nz805x2515r	19	14	which	which	PRON
nz805x2515r	19	15	is	be	AUX
nz805x2515r	19	16	balanced	balance	VERB
nz805x2515r	19	17	by	by	ADP
nz805x2515r	19	18	cations	cation	NOUN
nz805x2515r	19	19	in	in	ADP
nz805x2515r	19	20	solution	solution	NOUN
nz805x2515r	19	21	.	.	PUNCT
nz805x2515r	20	1	nanoclusters	nanocluster	NOUN
nz805x2515r	20	2	have	have	VERB
nz805x2515r	20	3	a	a	DET
nz805x2515r	20	4	promising	promising	ADJ
nz805x2515r	20	5	future	future	NOUN
nz805x2515r	20	6	in	in	ADP
nz805x2515r	20	7	designing	design	VERB
nz805x2515r	20	8	advanced	advanced	ADJ
nz805x2515r	20	9	nuclear	nuclear	ADJ
nz805x2515r	20	10	cycles	cycle	NOUN
nz805x2515r	20	11	,	,	PUNCT
nz805x2515r	20	12	where	where	SCONJ
nz805x2515r	20	13	they	they	PRON
nz805x2515r	20	14	can	can	AUX
nz805x2515r	20	15	be	be	AUX
nz805x2515r	20	16	filtered	filter	VERB
nz805x2515r	20	17	out	out	ADP
nz805x2515r	20	18	due	due	ADP
nz805x2515r	20	19	to	to	ADP
nz805x2515r	20	20	their	their	PRON
nz805x2515r	20	21	size	size	NOUN
nz805x2515r	20	22	,	,	PUNCT
nz805x2515r	20	23	thus	thus	ADV
nz805x2515r	20	24	avoiding	avoid	VERB
nz805x2515r	20	25	the	the	DET
nz805x2515r	20	26	usage	usage	NOUN
nz805x2515r	20	27	of	of	ADP
nz805x2515r	20	28	any	any	DET
nz805x2515r	20	29	liquid	liquid	NOUN
nz805x2515r	20	30	-	-	PUNCT
nz805x2515r	20	31	liquid	liquid	ADJ
nz805x2515r	20	32	extraction	extraction	NOUN
nz805x2515r	20	33	processes	process	NOUN
nz805x2515r	20	34	.	.	PUNCT
nz805x2515r	21	1	this	this	DET
nz805x2515r	21	2	technology	technology	NOUN
nz805x2515r	21	3	could	could	AUX
nz805x2515r	21	4	considerably	considerably	ADV
nz805x2515r	21	5	reduce	reduce	VERB
nz805x2515r	21	6	the	the	DET
nz805x2515r	21	7	amount	amount	NOUN
nz805x2515r	21	8	of	of	ADP
nz805x2515r	21	9	nuclear	nuclear	ADJ
nz805x2515r	21	10	waste	waste	NOUN
nz805x2515r	21	11	for	for	ADP
nz805x2515r	21	12	final	final	ADJ
nz805x2515r	21	13	disposal.the	disposal.the	DET
nz805x2515r	21	14	nanoclusters	nanocluster	NOUN
nz805x2515r	21	15	can	can	AUX
nz805x2515r	21	16	further	far	ADV
nz805x2515r	21	17	assemble	assemble	VERB
nz805x2515r	21	18	into	into	ADP
nz805x2515r	21	19	tertiary	tertiary	ADJ
nz805x2515r	21	20	structures	structure	NOUN
nz805x2515r	21	21	.	.	PUNCT
nz805x2515r	22	1	it	it	PRON
nz805x2515r	22	2	was	be	AUX
nz805x2515r	22	3	recently	recently	ADV
nz805x2515r	22	4	discovered	discover	VERB
nz805x2515r	22	5	by	by	ADP
nz805x2515r	22	6	burns	burn	NOUN
nz805x2515r	22	7	et	et	PROPN
nz805x2515r	22	8	al	al	PROPN
nz805x2515r	22	9	.	.	PUNCT
nz805x2515r	23	1	that	that	SCONJ
nz805x2515r	23	2	the	the	DET
nz805x2515r	23	3	type	type	NOUN
nz805x2515r	23	4	of	of	ADP
nz805x2515r	23	5	tertiary	tertiary	ADJ
nz805x2515r	23	6	structure	structure	NOUN
nz805x2515r	23	7	formed	form	VERB
nz805x2515r	23	8	depends	depend	VERB
nz805x2515r	23	9	upon	upon	SCONJ
nz805x2515r	23	10	the	the	DET
nz805x2515r	23	11	valency	valency	NOUN
nz805x2515r	23	12	of	of	ADP
nz805x2515r	23	13	the	the	DET
nz805x2515r	23	14	charge	charge	NOUN
nz805x2515r	23	15	-	-	PUNCT
nz805x2515r	23	16	balancing	balance	VERB
nz805x2515r	23	17	cations	cation	NOUN
nz805x2515r	23	18	.	.	PUNCT
nz805x2515r	24	1	when	when	SCONJ
nz805x2515r	24	2	neutralized	neutralize	VERB
nz805x2515r	24	3	with	with	ADP
nz805x2515r	24	4	divalent	divalent	ADJ
nz805x2515r	24	5	cations	cation	NOUN
nz805x2515r	24	6	(	(	PUNCT
nz805x2515r	24	7	ca(2	ca(2	PROPN
nz805x2515r	24	8	+	+	NUM
nz805x2515r	24	9	)	)	PUNCT
nz805x2515r	24	10	)	)	PUNCT
nz805x2515r	24	11	,	,	PUNCT
nz805x2515r	24	12	the	the	DET
nz805x2515r	24	13	nanoclusters	nanocluster	NOUN
nz805x2515r	24	14	aggregate	aggregate	VERB
nz805x2515r	24	15	into	into	ADP
nz805x2515r	24	16	spherical	spherical	ADJ
nz805x2515r	24	17	macroassemblies	macroassemblie	NOUN
nz805x2515r	24	18	known	know	VERB
nz805x2515r	24	19	as	as	ADP
nz805x2515r	24	20	`	`	PUNCT
nz805x2515r	24	21	`	`	PUNCT
nz805x2515r	24	22	blackberries	blackberry	NOUN
nz805x2515r	24	23	"	"	PUNCT
nz805x2515r	24	24	,	,	PUNCT
nz805x2515r	24	25	consisting	consist	VERB
nz805x2515r	24	26	of	of	ADP
nz805x2515r	24	27	hundreds	hundred	NOUN
nz805x2515r	24	28	of	of	ADP
nz805x2515r	24	29	individual	individual	ADJ
nz805x2515r	24	30	nanoclusters	nanocluster	NOUN
nz805x2515r	24	31	.	.	PUNCT
nz805x2515r	25	1	however	however	ADV
nz805x2515r	25	2	,	,	PUNCT
nz805x2515r	25	3	in	in	ADP
nz805x2515r	25	4	the	the	DET
nz805x2515r	25	5	presence	presence	NOUN
nz805x2515r	25	6	of	of	ADP
nz805x2515r	25	7	monovalent	monovalent	NOUN
nz805x2515r	25	8	salt	salt	NOUN
nz805x2515r	25	9	(	(	PUNCT
nz805x2515r	25	10	k+	k+	NOUN
nz805x2515r	25	11	)	)	PUNCT
nz805x2515r	25	12	,	,	PUNCT
nz805x2515r	25	13	the	the	DET
nz805x2515r	25	14	nanoclusters	nanocluster	NOUN
nz805x2515r	25	15	form	form	VERB
nz805x2515r	25	16	elongated	elongate	VERB
nz805x2515r	25	17	structures	structure	NOUN
nz805x2515r	25	18	.	.	PUNCT
nz805x2515r	26	1	the	the	DET
nz805x2515r	26	2	exact	exact	ADJ
nz805x2515r	26	3	role	role	NOUN
nz805x2515r	26	4	of	of	ADP
nz805x2515r	26	5	the	the	DET
nz805x2515r	26	6	cations	cation	NOUN
nz805x2515r	26	7	in	in	ADP
nz805x2515r	26	8	this	this	DET
nz805x2515r	26	9	process	process	NOUN
nz805x2515r	26	10	is	be	AUX
nz805x2515r	26	11	not	not	PART
nz805x2515r	26	12	well	well	ADV
nz805x2515r	26	13	understood	understand	VERB
nz805x2515r	26	14	experimentally.we	experimentally.we	NUM
nz805x2515r	26	15	sought	seek	VERB
nz805x2515r	26	16	to	to	PART
nz805x2515r	26	17	accurately	accurately	ADV
nz805x2515r	26	18	determine	determine	VERB
nz805x2515r	26	19	the	the	DET
nz805x2515r	26	20	binding	bind	VERB
nz805x2515r	26	21	sites	site	NOUN
nz805x2515r	26	22	of	of	ADP
nz805x2515r	26	23	water	water	NOUN
nz805x2515r	26	24	and	and	CCONJ
nz805x2515r	26	25	various	various	ADJ
nz805x2515r	26	26	cations	cation	NOUN
nz805x2515r	26	27	(	(	PUNCT
nz805x2515r	26	28	li+	li+	PROPN
nz805x2515r	26	29	,	,	PUNCT
nz805x2515r	26	30	na+	na+	NOUN
nz805x2515r	26	31	,	,	PUNCT
nz805x2515r	26	32	k+	k+	ADV
nz805x2515r	26	33	,	,	PUNCT
nz805x2515r	26	34	rb+	rb+	PROPN
nz805x2515r	26	35	,	,	PUNCT
nz805x2515r	26	36	cs+	cs+	ADJ
nz805x2515r	26	37	,	,	PUNCT
nz805x2515r	26	38	and	and	CCONJ
nz805x2515r	26	39	ca(2	ca(2	PROPN
nz805x2515r	26	40	+	+	NUM
nz805x2515r	26	41	)	)	PUNCT
nz805x2515r	26	42	)	)	PUNCT
nz805x2515r	26	43	to	to	ADP
nz805x2515r	26	44	the	the	DET
nz805x2515r	26	45	u20	u20	NUM
nz805x2515r	26	46	nanocluster	nanocluster	NOUN
nz805x2515r	26	47	,	,	PUNCT
nz805x2515r	26	48	and	and	CCONJ
nz805x2515r	26	49	to	to	PART
nz805x2515r	26	50	better	well	ADV
nz805x2515r	26	51	understand	understand	VERB
nz805x2515r	26	52	how	how	SCONJ
nz805x2515r	26	53	the	the	DET
nz805x2515r	26	54	identity	identity	NOUN
nz805x2515r	26	55	of	of	ADP
nz805x2515r	26	56	the	the	DET
nz805x2515r	26	57	cation	cation	NOUN
nz805x2515r	26	58	affects	affect	VERB
nz805x2515r	26	59	nanocluster	nanocluster	PROPN
nz805x2515r	26	60	aggregation	aggregation	NOUN
nz805x2515r	26	61	.	.	PUNCT
nz805x2515r	27	1	we	we	PRON
nz805x2515r	27	2	first	first	ADV
nz805x2515r	27	3	developed	develop	VERB
nz805x2515r	27	4	a	a	DET
nz805x2515r	27	5	new	new	ADJ
nz805x2515r	27	6	classical	classical	ADJ
nz805x2515r	27	7	force	force	NOUN
nz805x2515r	27	8	field	field	NOUN
nz805x2515r	27	9	for	for	ADP
nz805x2515r	27	10	the	the	DET
nz805x2515r	27	11	simulation	simulation	NOUN
nz805x2515r	27	12	of	of	ADP
nz805x2515r	27	13	u20	u20	NUM
nz805x2515r	27	14	nanoclusters	nanocluster	NOUN
nz805x2515r	27	15	in	in	ADP
nz805x2515r	27	16	explicitly	explicitly	ADV
nz805x2515r	27	17	-	-	PUNCT
nz805x2515r	27	18	modeled	model	VERB
nz805x2515r	27	19	water	water	NOUN
nz805x2515r	27	20	using	use	VERB
nz805x2515r	27	21	a	a	DET
nz805x2515r	27	22	combination	combination	NOUN
nz805x2515r	27	23	of	of	ADP
nz805x2515r	27	24	lennard	lennard	PROPN
nz805x2515r	27	25	-	-	PUNCT
nz805x2515r	27	26	jones	jones	PROPN
nz805x2515r	27	27	and	and	CCONJ
nz805x2515r	27	28	coloumb	coloumb	PROPN
nz805x2515r	27	29	potentials	potential	NOUN
nz805x2515r	27	30	.	.	PUNCT
nz805x2515r	28	1	molecular	molecular	ADJ
nz805x2515r	28	2	dynamics	dynamic	NOUN
nz805x2515r	28	3	was	be	AUX
nz805x2515r	28	4	used	use	VERB
nz805x2515r	28	5	to	to	PART
nz805x2515r	28	6	determine	determine	VERB
nz805x2515r	28	7	the	the	DET
nz805x2515r	28	8	preferred	preferred	ADJ
nz805x2515r	28	9	binding	bind	VERB
nz805x2515r	28	10	sites	site	NOUN
nz805x2515r	28	11	of	of	ADP
nz805x2515r	28	12	the	the	DET
nz805x2515r	28	13	cations	cation	NOUN
nz805x2515r	28	14	.	.	PUNCT
nz805x2515r	29	1	replica	replica	PROPN
nz805x2515r	29	2	exchange	exchange	PROPN
nz805x2515r	29	3	molecular	molecular	ADJ
nz805x2515r	29	4	dynamics	dynamic	NOUN
nz805x2515r	29	5	was	be	AUX
nz805x2515r	29	6	used	use	VERB
nz805x2515r	29	7	to	to	PART
nz805x2515r	29	8	ensure	ensure	VERB
nz805x2515r	29	9	equilibration	equilibration	NOUN
nz805x2515r	29	10	and	and	CCONJ
nz805x2515r	29	11	ultimately	ultimately	ADV
nz805x2515r	29	12	determine	determine	VERB
nz805x2515r	29	13	the	the	DET
nz805x2515r	29	14	equilibrium	equilibrium	NOUN
nz805x2515r	29	15	distribution	distribution	NOUN
nz805x2515r	29	16	of	of	ADP
nz805x2515r	29	17	cations	cation	NOUN
nz805x2515r	29	18	and	and	CCONJ
nz805x2515r	29	19	water	water	NOUN
nz805x2515r	29	20	around	around	ADP
nz805x2515r	29	21	the	the	DET
nz805x2515r	29	22	nanocluster	nanocluster	NOUN
nz805x2515r	29	23	.	.	PUNCT
nz805x2515r	30	1	in	in	ADP
nz805x2515r	30	2	addition	addition	NOUN
nz805x2515r	30	3	,	,	PUNCT
nz805x2515r	30	4	the	the	DET
nz805x2515r	30	5	free	free	ADJ
nz805x2515r	30	6	energy	energy	NOUN
nz805x2515r	30	7	barrier	barrier	NOUN
nz805x2515r	30	8	associated	associate	VERB
nz805x2515r	30	9	with	with	ADP
nz805x2515r	30	10	a	a	DET
nz805x2515r	30	11	cation	cation	NOUN
nz805x2515r	30	12	entering	enter	VERB
nz805x2515r	30	13	the	the	DET
nz805x2515r	30	14	nanocluster	nanocluster	NOUN
nz805x2515r	30	15	was	be	AUX
nz805x2515r	30	16	computed	compute	VERB
nz805x2515r	30	17	.	.	PUNCT
nz805x2515r	31	1	finally	finally	ADV
nz805x2515r	31	2	,	,	PUNCT
nz805x2515r	31	3	the	the	DET
nz805x2515r	31	4	association	association	NOUN
nz805x2515r	31	5	of	of	ADP
nz805x2515r	31	6	two	two	NUM
nz805x2515r	31	7	u20	u20	NUM
nz805x2515r	31	8	nanoclusters	nanocluster	NOUN
nz805x2515r	31	9	was	be	AUX
nz805x2515r	31	10	explored	explore	VERB
nz805x2515r	31	11	by	by	ADP
nz805x2515r	31	12	free	free	ADJ
nz805x2515r	31	13	energy	energy	NOUN
nz805x2515r	31	14	calculations	calculation	NOUN
nz805x2515r	31	15	.	.	PUNCT
nz805x2515r	32	1	the	the	DET
nz805x2515r	32	2	free	free	ADJ
nz805x2515r	32	3	energy	energy	NOUN
nz805x2515r	32	4	of	of	ADP
nz805x2515r	32	5	association	association	NOUN
nz805x2515r	32	6	was	be	AUX
nz805x2515r	32	7	found	find	VERB
nz805x2515r	32	8	to	to	PART
nz805x2515r	32	9	vary	vary	VERB
nz805x2515r	32	10	greatly	greatly	ADV
nz805x2515r	32	11	with	with	ADP
nz805x2515r	32	12	the	the	DET
nz805x2515r	32	13	valency	valency	NOUN
nz805x2515r	32	14	of	of	ADP
nz805x2515r	32	15	the	the	DET
nz805x2515r	32	16	charge	charge	NOUN
nz805x2515r	32	17	balancing	balance	VERB
nz805x2515r	32	18	cations.in	cations.in	NUM
nz805x2515r	32	19	this	this	DET
nz805x2515r	32	20	dissertation	dissertation	NOUN
nz805x2515r	32	21	,	,	PUNCT
nz805x2515r	32	22	solutions	solution	NOUN
nz805x2515r	32	23	of	of	ADP
nz805x2515r	32	24	actinyl	actinyl	PROPN
nz805x2515r	32	25	ions	ion	NOUN
nz805x2515r	32	26	and	and	CCONJ
nz805x2515r	32	27	nanoclusters	nanocluster	NOUN
nz805x2515r	32	28	are	be	AUX
nz805x2515r	32	29	studied	study	VERB
nz805x2515r	32	30	using	use	VERB
nz805x2515r	32	31	classical	classical	ADJ
nz805x2515r	32	32	molecular	molecular	ADJ
nz805x2515r	32	33	simulation	simulation	NOUN
nz805x2515r	32	34	techniques	technique	NOUN
nz805x2515r	32	35	.	.	PUNCT
nz805x2515r	33	1	thermodynamic	thermodynamic	ADJ
nz805x2515r	33	2	properties	property	NOUN
nz805x2515r	33	3	of	of	ADP
nz805x2515r	33	4	actinyl	actinyl	PROPN
nz805x2515r	33	5	solutions	solution	NOUN
nz805x2515r	33	6	were	be	AUX
nz805x2515r	33	7	computed	compute	VERB
nz805x2515r	33	8	and	and	CCONJ
nz805x2515r	33	9	corroborate	corroborate	VERB
nz805x2515r	33	10	experiments	experiment	NOUN
nz805x2515r	33	11	,	,	PUNCT
nz805x2515r	33	12	and	and	CCONJ
nz805x2515r	33	13	predictions	prediction	NOUN
nz805x2515r	33	14	are	be	AUX
nz805x2515r	33	15	made	make	VERB
nz805x2515r	33	16	where	where	SCONJ
nz805x2515r	33	17	experimental	experimental	ADJ
nz805x2515r	33	18	data	datum	NOUN
nz805x2515r	33	19	is	be	AUX
nz805x2515r	33	20	lacking	lack	VERB
nz805x2515r	33	21	.	.	PUNCT
nz805x2515r	34	1	these	these	DET
nz805x2515r	34	2	studies	study	NOUN
nz805x2515r	34	3	support	support	VERB
nz805x2515r	34	4	the	the	DET
nz805x2515r	34	5	goal	goal	NOUN
nz805x2515r	34	6	of	of	ADP
nz805x2515r	34	7	obtaining	obtain	VERB
nz805x2515r	34	8	nanoscale	nanoscale	NOUN
nz805x2515r	34	9	control	control	NOUN
nz805x2515r	34	10	of	of	ADP
nz805x2515r	34	11	the	the	DET
nz805x2515r	34	12	actinides	actinide	NOUN
nz805x2515r	34	13	,	,	PUNCT
nz805x2515r	34	14	which	which	PRON
nz805x2515r	34	15	is	be	AUX
nz805x2515r	34	16	crucial	crucial	ADJ
nz805x2515r	34	17	for	for	ADP
nz805x2515r	34	18	the	the	DET
nz805x2515r	34	19	advancement	advancement	NOUN
nz805x2515r	34	20	of	of	ADP
nz805x2515r	34	21	nuclear	nuclear	ADJ
nz805x2515r	34	22	power	power	NOUN
nz805x2515r	34	23	generation	generation	NOUN
nz805x2515r	34	24	,	,	PUNCT
nz805x2515r	34	25	human	human	ADJ
nz805x2515r	34	26	health	health	NOUN
nz805x2515r	34	27	,	,	PUNCT
nz805x2515r	34	28	and	and	CCONJ
nz805x2515r	34	29	the	the	DET
nz805x2515r	34	30	environment	environment	NOUN
nz805x2515r	34	31	.	.	PUNCT