id	sid	tid	token	lemma	pos
nc580k24p3c	1	1	c	c	X
nc580k24p3c	1	2	-	-	PUNCT
nc580k24p3c	1	3	c	c	NOUN
nc580k24p3c	1	4	coupling	coupling	NOUN
nc580k24p3c	1	5	reactions	reaction	NOUN
nc580k24p3c	1	6	are	be	AUX
nc580k24p3c	1	7	of	of	ADP
nc580k24p3c	1	8	high	high	ADJ
nc580k24p3c	1	9	interest	interest	NOUN
nc580k24p3c	1	10	to	to	ADP
nc580k24p3c	1	11	synthetic	synthetic	ADJ
nc580k24p3c	1	12	chemists	chemist	NOUN
nc580k24p3c	1	13	due	due	ADP
nc580k24p3c	1	14	to	to	ADP
nc580k24p3c	1	15	their	their	PRON
nc580k24p3c	1	16	ability	ability	NOUN
nc580k24p3c	1	17	to	to	PART
nc580k24p3c	1	18	accomplish	accomplish	VERB
nc580k24p3c	1	19	chemical	chemical	NOUN
nc580k24p3c	1	20	transformations	transformation	NOUN
nc580k24p3c	1	21	often	often	ADV
nc580k24p3c	1	22	involving	involve	VERB
nc580k24p3c	1	23	value	value	NOUN
nc580k24p3c	1	24	addition	addition	NOUN
nc580k24p3c	1	25	to	to	ADP
nc580k24p3c	1	26	the	the	DET
nc580k24p3c	1	27	substrates	substrate	NOUN
nc580k24p3c	1	28	.	.	PUNCT
nc580k24p3c	2	1	the	the	DET
nc580k24p3c	2	2	high	high	ADJ
nc580k24p3c	2	3	impact	impact	NOUN
nc580k24p3c	2	4	of	of	ADP
nc580k24p3c	2	5	the	the	DET
nc580k24p3c	2	6	research	research	NOUN
nc580k24p3c	2	7	in	in	ADP
nc580k24p3c	2	8	this	this	DET
nc580k24p3c	2	9	area	area	NOUN
nc580k24p3c	2	10	is	be	AUX
nc580k24p3c	2	11	evident	evident	ADJ
nc580k24p3c	2	12	by	by	ADP
nc580k24p3c	2	13	a	a	DET
nc580k24p3c	2	14	nobel	nobel	PROPN
nc580k24p3c	2	15	prize	prize	PROPN
nc580k24p3c	2	16	awarded	award	VERB
nc580k24p3c	2	17	to	to	ADP
nc580k24p3c	2	18	richard	richard	PROPN
nc580k24p3c	2	19	f.	f.	PROPN
nc580k24p3c	2	20	heck	heck	PROPN
nc580k24p3c	2	21	,	,	PUNCT
nc580k24p3c	2	22	ei	ei	PROPN
nc580k24p3c	2	23	-	-	PUNCT
nc580k24p3c	2	24	ichi	ichi	PROPN
nc580k24p3c	2	25	negishi	negishi	PROPN
nc580k24p3c	2	26	,	,	PUNCT
nc580k24p3c	2	27	and	and	CCONJ
nc580k24p3c	2	28	akira	akira	PROPN
nc580k24p3c	2	29	suzuki	suzuki	NOUN
nc580k24p3c	2	30	in	in	ADP
nc580k24p3c	2	31	the	the	DET
nc580k24p3c	2	32	year	year	NOUN
nc580k24p3c	2	33	2010	2010	NUM
nc580k24p3c	2	34	.	.	PUNCT
nc580k24p3c	3	1	this	this	DET
nc580k24p3c	3	2	thesis	thesis	NOUN
nc580k24p3c	3	3	outlines	outline	VERB
nc580k24p3c	3	4	a	a	DET
nc580k24p3c	3	5	research	research	NOUN
nc580k24p3c	3	6	project	project	NOUN
nc580k24p3c	3	7	in	in	ADP
nc580k24p3c	3	8	the	the	DET
nc580k24p3c	3	9	area	area	NOUN
nc580k24p3c	3	10	of	of	ADP
nc580k24p3c	3	11	c	c	PROPN
nc580k24p3c	3	12	-	-	PUNCT
nc580k24p3c	3	13	c	c	NOUN
nc580k24p3c	3	14	coupling	coupling	NOUN
nc580k24p3c	3	15	reactions	reaction	NOUN
nc580k24p3c	3	16	to	to	PART
nc580k24p3c	3	17	synthesize	synthesize	VERB
nc580k24p3c	3	18	industrially	industrially	ADV
nc580k24p3c	3	19	relevant	relevant	ADJ
nc580k24p3c	3	20	products	product	NOUN
nc580k24p3c	3	21	using	use	VERB
nc580k24p3c	3	22	substrate	substrate	NOUN
nc580k24p3c	3	23	molecules	molecule	NOUN
nc580k24p3c	3	24	typically	typically	ADV
nc580k24p3c	3	25	small	small	ADJ
nc580k24p3c	3	26	oxygenates	oxygenate	NOUN
nc580k24p3c	3	27	,	,	PUNCT
nc580k24p3c	3	28	such	such	ADJ
nc580k24p3c	3	29	as	as	ADP
nc580k24p3c	3	30	,	,	PUNCT
nc580k24p3c	3	31	acetic	acetic	ADJ
nc580k24p3c	3	32	acid	acid	NOUN
nc580k24p3c	3	33	,	,	PUNCT
nc580k24p3c	3	34	and	and	CCONJ
nc580k24p3c	3	35	c2	c2	PROPN
nc580k24p3c	3	36	-	-	PUNCT
nc580k24p3c	3	37	c3	c3	NOUN
nc580k24p3c	3	38	aldehydes	aldehyde	NOUN
nc580k24p3c	3	39	.	.	PUNCT
nc580k24p3c	4	1	the	the	DET
nc580k24p3c	4	2	focus	focus	NOUN
nc580k24p3c	4	3	is	be	AUX
nc580k24p3c	4	4	on	on	ADP
nc580k24p3c	4	5	the	the	DET
nc580k24p3c	4	6	development	development	NOUN
nc580k24p3c	4	7	of	of	ADP
nc580k24p3c	4	8	suitable	suitable	ADJ
nc580k24p3c	4	9	catalysts	catalyst	NOUN
nc580k24p3c	4	10	to	to	PART
nc580k24p3c	4	11	accomplish	accomplish	VERB
nc580k24p3c	4	12	these	these	DET
nc580k24p3c	4	13	transformations	transformation	NOUN
nc580k24p3c	4	14	efficiently	efficiently	ADV
nc580k24p3c	4	15	.	.	PUNCT
nc580k24p3c	5	1	self	self	NOUN
nc580k24p3c	5	2	c	c	X
nc580k24p3c	5	3	-	-	PUNCT
nc580k24p3c	5	4	c	c	NOUN
nc580k24p3c	5	5	coupling	coupling	NOUN
nc580k24p3c	5	6	of	of	ADP
nc580k24p3c	5	7	acetic	acetic	ADJ
nc580k24p3c	5	8	acid	acid	NOUN
nc580k24p3c	5	9	,	,	PUNCT
nc580k24p3c	5	10	and	and	CCONJ
nc580k24p3c	5	11	propionaldehyde	propionaldehyde	PROPN
nc580k24p3c	5	12	via	via	ADP
nc580k24p3c	5	13	ketonization	ketonization	NOUN
nc580k24p3c	5	14	and	and	CCONJ
nc580k24p3c	5	15	aldol	aldol	ADJ
nc580k24p3c	5	16	condensation	condensation	NOUN
nc580k24p3c	5	17	,	,	PUNCT
nc580k24p3c	5	18	respectively	respectively	ADV
nc580k24p3c	5	19	,	,	PUNCT
nc580k24p3c	5	20	are	be	AUX
nc580k24p3c	5	21	the	the	DET
nc580k24p3c	5	22	reactions	reaction	NOUN
nc580k24p3c	5	23	under	under	ADP
nc580k24p3c	5	24	investigation	investigation	NOUN
nc580k24p3c	5	25	during	during	ADP
nc580k24p3c	5	26	the	the	DET
nc580k24p3c	5	27	course	course	NOUN
nc580k24p3c	5	28	of	of	ADP
nc580k24p3c	5	29	this	this	DET
nc580k24p3c	5	30	thesis	thesis	NOUN
nc580k24p3c	5	31	project	project	NOUN
nc580k24p3c	5	32	.	.	PUNCT
nc580k24p3c	6	1	acetone	acetone	NOUN
nc580k24p3c	6	2	,	,	PUNCT
nc580k24p3c	6	3	and	and	CCONJ
nc580k24p3c	6	4	2	2	NUM
nc580k24p3c	6	5	-	-	PUNCT
nc580k24p3c	6	6	methyl-2	methyl-2	NUM
nc580k24p3c	6	7	-	-	PUNCT
nc580k24p3c	6	8	pentenal	pentenal	PROPN
nc580k24p3c	6	9	are	be	AUX
nc580k24p3c	6	10	the	the	DET
nc580k24p3c	6	11	desired	desire	VERB
nc580k24p3c	6	12	products	product	NOUN
nc580k24p3c	6	13	,	,	PUNCT
nc580k24p3c	6	14	which	which	PRON
nc580k24p3c	6	15	have	have	VERB
nc580k24p3c	6	16	a	a	DET
nc580k24p3c	6	17	wide	wide	ADJ
nc580k24p3c	6	18	range	range	NOUN
nc580k24p3c	6	19	of	of	ADP
nc580k24p3c	6	20	industrial	industrial	ADJ
nc580k24p3c	6	21	applications	application	NOUN
nc580k24p3c	6	22	.	.	PUNCT
nc580k24p3c	7	1	however	however	ADV
nc580k24p3c	7	2	,	,	PUNCT
nc580k24p3c	7	3	tendency	tendency	NOUN
nc580k24p3c	7	4	of	of	ADP
nc580k24p3c	7	5	these	these	DET
nc580k24p3c	7	6	molecules	molecule	NOUN
nc580k24p3c	7	7	to	to	PART
nc580k24p3c	7	8	form	form	VERB
nc580k24p3c	7	9	longer	long	ADJ
nc580k24p3c	7	10	carbon	carbon	NOUN
nc580k24p3c	7	11	chains	chain	NOUN
nc580k24p3c	7	12	via	via	ADP
nc580k24p3c	7	13	continuous	continuous	ADJ
nc580k24p3c	7	14	coupling	coupling	NOUN
nc580k24p3c	7	15	is	be	AUX
nc580k24p3c	7	16	a	a	DET
nc580k24p3c	7	17	major	major	ADJ
nc580k24p3c	7	18	drawback	drawback	NOUN
nc580k24p3c	7	19	during	during	ADP
nc580k24p3c	7	20	these	these	DET
nc580k24p3c	7	21	reactions	reaction	NOUN
nc580k24p3c	7	22	.	.	PUNCT
nc580k24p3c	8	1	therefore	therefore	ADV
nc580k24p3c	8	2	,	,	PUNCT
nc580k24p3c	8	3	a	a	DET
nc580k24p3c	8	4	catalyst	catalyst	NOUN
nc580k24p3c	8	5	that	that	PRON
nc580k24p3c	8	6	is	be	AUX
nc580k24p3c	8	7	highly	highly	ADV
nc580k24p3c	8	8	selective	selective	ADJ
nc580k24p3c	8	9	to	to	ADP
nc580k24p3c	8	10	the	the	DET
nc580k24p3c	8	11	desired	desire	VERB
nc580k24p3c	8	12	products	product	NOUN
nc580k24p3c	8	13	and	and	CCONJ
nc580k24p3c	8	14	that	that	PRON
nc580k24p3c	8	15	can	can	AUX
nc580k24p3c	8	16	deliver	deliver	VERB
nc580k24p3c	8	17	competitive	competitive	ADJ
nc580k24p3c	8	18	yields	yield	NOUN
nc580k24p3c	8	19	is	be	AUX
nc580k24p3c	8	20	needed	need	VERB
nc580k24p3c	8	21	.	.	PUNCT
nc580k24p3c	9	1	with	with	ADP
nc580k24p3c	9	2	this	this	DET
nc580k24p3c	9	3	regard	regard	NOUN
nc580k24p3c	9	4	,	,	PUNCT
nc580k24p3c	9	5	novel	novel	ADJ
nc580k24p3c	9	6	materials	material	NOUN
nc580k24p3c	9	7	containing	contain	VERB
nc580k24p3c	9	8	cerium	cerium	NOUN
nc580k24p3c	9	9	and/or	and/or	CCONJ
nc580k24p3c	9	10	manganese	manganese	NOUN
nc580k24p3c	9	11	heteroatoms	heteroatom	NOUN
nc580k24p3c	9	12	incorporated	incorporate	VERB
nc580k24p3c	9	13	in	in	ADP
nc580k24p3c	9	14	the	the	DET
nc580k24p3c	9	15	zeolite	zeolite	NOUN
nc580k24p3c	9	16	frameworks	framework	NOUN
nc580k24p3c	9	17	are	be	AUX
nc580k24p3c	9	18	tested	test	VERB
nc580k24p3c	9	19	as	as	ADP
nc580k24p3c	9	20	catalysts	catalyst	NOUN
nc580k24p3c	9	21	.	.	PUNCT
nc580k24p3c	10	1	the	the	DET
nc580k24p3c	10	2	data	datum	NOUN
nc580k24p3c	10	3	show	show	VERB
nc580k24p3c	10	4	the	the	DET
nc580k24p3c	10	5	presence	presence	NOUN
nc580k24p3c	10	6	of	of	ADP
nc580k24p3c	10	7	ce3	ce3	SPACE
nc580k24p3c	10	8	+	+	NOUN
nc580k24p3c	10	9	,	,	PUNCT
nc580k24p3c	10	10	and	and	CCONJ
nc580k24p3c	10	11	mn3	mn3	PROPN
nc580k24p3c	10	12	+	+	PROPN
nc580k24p3c	10	13	heteroatom	heteroatom	NOUN
nc580k24p3c	10	14	species	specie	NOUN
nc580k24p3c	10	15	in	in	ADP
nc580k24p3c	10	16	the	the	DET
nc580k24p3c	10	17	crystalline	crystalline	ADJ
nc580k24p3c	10	18	zeolite	zeolite	NOUN
nc580k24p3c	10	19	framework	framework	NOUN
nc580k24p3c	10	20	,	,	PUNCT
nc580k24p3c	10	21	and	and	CCONJ
nc580k24p3c	10	22	these	these	DET
nc580k24p3c	10	23	catalysts	catalyst	NOUN
nc580k24p3c	10	24	are	be	AUX
nc580k24p3c	10	25	active	active	ADJ
nc580k24p3c	10	26	at	at	ADP
nc580k24p3c	10	27	low	low	ADJ
nc580k24p3c	10	28	temperature	temperature	NOUN
nc580k24p3c	10	29	during	during	ADP
nc580k24p3c	10	30	self	self	NOUN
nc580k24p3c	10	31	-	-	PUNCT
nc580k24p3c	10	32	aldol	aldol	NOUN
nc580k24p3c	10	33	condensation	condensation	NOUN
nc580k24p3c	10	34	reaction	reaction	NOUN
nc580k24p3c	10	35	as	as	ADV
nc580k24p3c	10	36	well	well	ADV
nc580k24p3c	10	37	as	as	ADP
nc580k24p3c	10	38	can	can	AUX
nc580k24p3c	10	39	deliver	deliver	VERB
nc580k24p3c	10	40	higher	high	ADJ
nc580k24p3c	10	41	rates	rate	NOUN
nc580k24p3c	10	42	to	to	ADP
nc580k24p3c	10	43	the	the	DET
nc580k24p3c	10	44	desired	desire	VERB
nc580k24p3c	10	45	products	product	NOUN
nc580k24p3c	10	46	during	during	ADP
nc580k24p3c	10	47	the	the	DET
nc580k24p3c	10	48	c	c	PROPN
nc580k24p3c	10	49	-	-	PUNCT
nc580k24p3c	10	50	c	c	NOUN
nc580k24p3c	10	51	coupling	coupling	NOUN
nc580k24p3c	10	52	reactions	reaction	NOUN
nc580k24p3c	10	53	of	of	ADP
nc580k24p3c	10	54	small	small	ADJ
nc580k24p3c	10	55	oxygenates	oxygenate	NOUN
nc580k24p3c	10	56	tested	test	VERB
nc580k24p3c	10	57	.	.	PUNCT