id sid tid token lemma pos ks65h993556 1 1 zeolite zeolite NOUN ks65h993556 1 2 is be AUX ks65h993556 1 3 a a DET ks65h993556 1 4 fascinating fascinating ADJ ks65h993556 1 5 porous porous ADJ ks65h993556 1 6 material material NOUN ks65h993556 1 7 made make VERB ks65h993556 1 8 up up ADP ks65h993556 1 9 of of ADP ks65h993556 1 10 many many ADJ ks65h993556 1 11 chemical chemical NOUN ks65h993556 1 12 building building NOUN ks65h993556 1 13 blocks block NOUN ks65h993556 1 14 . . PUNCT ks65h993556 2 1 the the DET ks65h993556 2 2 use use NOUN ks65h993556 2 3 of of ADP ks65h993556 2 4 zeolite zeolite NOUN ks65h993556 2 5 is be AUX ks65h993556 2 6 prevalent prevalent ADJ ks65h993556 2 7 in in ADP ks65h993556 2 8 modern modern ADJ ks65h993556 2 9 days day NOUN ks65h993556 2 10 applications application NOUN ks65h993556 2 11 . . PUNCT ks65h993556 3 1 its its PRON ks65h993556 3 2 usage usage NOUN ks65h993556 3 3 can can AUX ks65h993556 3 4 be be AUX ks65h993556 3 5 widely widely ADV ks65h993556 3 6 seen see VERB ks65h993556 3 7 in in ADP ks65h993556 3 8 agriculture agriculture NOUN ks65h993556 3 9 , , PUNCT ks65h993556 3 10 cement cement NOUN ks65h993556 3 11 making making NOUN ks65h993556 3 12 , , PUNCT ks65h993556 3 13 wastewater wastewater NOUN ks65h993556 3 14 treatment treatment NOUN ks65h993556 3 15 , , PUNCT ks65h993556 3 16 environment environment NOUN ks65h993556 3 17 protection protection NOUN ks65h993556 3 18 , , PUNCT ks65h993556 3 19 and and CCONJ ks65h993556 3 20 numerous numerous ADJ ks65h993556 3 21 small small ADJ ks65h993556 3 22 - - PUNCT ks65h993556 3 23 scale scale NOUN ks65h993556 3 24 and and CCONJ ks65h993556 3 25 micro micro NOUN ks65h993556 3 26 - - NOUN ks65h993556 3 27 scale scale NOUN ks65h993556 3 28 applications.1–5 applications.1–5 PUNCT ks65h993556 3 29 zeolite zeolite NOUN ks65h993556 3 30 is be AUX ks65h993556 3 31 built build VERB ks65h993556 3 32 up up ADP ks65h993556 3 33 by by ADP ks65h993556 3 34 its its PRON ks65h993556 3 35 tetrahedral tetrahedral ADJ ks65h993556 3 36 sites site NOUN ks65h993556 3 37 ( ( PUNCT ks65h993556 3 38 t t PROPN ks65h993556 3 39 - - PUNCT ks65h993556 3 40 site site NOUN ks65h993556 3 41 ) ) PUNCT ks65h993556 3 42 such such ADJ ks65h993556 3 43 as as ADP ks65h993556 3 44 silicon silicon NOUN ks65h993556 3 45 ( ( PUNCT ks65h993556 3 46 si4 si4 NOUN ks65h993556 3 47 + + NUM ks65h993556 3 48 ) ) PUNCT ks65h993556 3 49 and and CCONJ ks65h993556 3 50 aluminum aluminum NOUN ks65h993556 3 51 ( ( PUNCT ks65h993556 3 52 al3 al3 PROPN ks65h993556 3 53 + + NUM ks65h993556 3 54 ) ) PUNCT ks65h993556 3 55 t t NOUN ks65h993556 3 56 - - PUNCT ks65h993556 3 57 sites site NOUN ks65h993556 3 58 that that PRON ks65h993556 3 59 are be AUX ks65h993556 3 60 bridged bridge VERB ks65h993556 3 61 together together ADV ks65h993556 3 62 by by ADP ks65h993556 3 63 oxygen oxygen NOUN ks65h993556 3 64 atoms.6 atoms.6 DET ks65h993556 3 65 an an DET ks65h993556 3 66 incumbent incumbent NOUN ks65h993556 3 67 si4 si4 NOUN ks65h993556 3 68 + + SYM ks65h993556 3 69 type type NOUN ks65h993556 3 70 tetrahedra tetrahedron NOUN ks65h993556 3 71 which which PRON ks65h993556 3 72 is be AUX ks65h993556 3 73 replaced replace VERB ks65h993556 3 74 by by ADP ks65h993556 3 75 al3 al3 PROPN ks65h993556 3 76 + + CCONJ ks65h993556 3 77 leads lead VERB ks65h993556 3 78 to to ADP ks65h993556 3 79 the the DET ks65h993556 3 80 creation creation NOUN ks65h993556 3 81 of of ADP ks65h993556 3 82 a a DET ks65h993556 3 83 -1 -1 ADJ ks65h993556 3 84 charge charge NOUN ks65h993556 3 85 on on ADP ks65h993556 3 86 its its PRON ks65h993556 3 87 connected connected ADJ ks65h993556 3 88 oxygen oxygen NOUN ks65h993556 3 89 . . PUNCT ks65h993556 4 1 within within ADP ks65h993556 4 2 that that DET ks65h993556 4 3 al3 al3 NOUN ks65h993556 4 4 + + SYM ks65h993556 4 5 inclusive inclusive ADJ ks65h993556 4 6 zeolite zeolite NOUN ks65h993556 4 7 ring ring NOUN ks65h993556 4 8 , , PUNCT ks65h993556 4 9 such such ADJ ks65h993556 4 10 as as ADP ks65h993556 4 11 the the DET ks65h993556 4 12 six six NUM ks65h993556 4 13 - - PUNCT ks65h993556 4 14 membered membered NOUN ks65h993556 4 15 - - PUNCT ks65h993556 4 16 ring ring NOUN ks65h993556 4 17 ( ( PUNCT ks65h993556 4 18 6mr 6mr PROPN ks65h993556 4 19 ) ) PUNCT ks65h993556 4 20 and and CCONJ ks65h993556 4 21 the the DET ks65h993556 4 22 eight eight NUM ks65h993556 4 23 - - PUNCT ks65h993556 4 24 membered membered NOUN ks65h993556 4 25 - - PUNCT ks65h993556 4 26 ring ring NOUN ks65h993556 4 27 ( ( PUNCT ks65h993556 4 28 8mr 8mr PROPN ks65h993556 4 29 ) ) PUNCT ks65h993556 4 30 , , PUNCT ks65h993556 4 31 there there PRON ks65h993556 4 32 can can AUX ks65h993556 4 33 be be AUX ks65h993556 4 34 another another DET ks65h993556 4 35 al3 al3 NOUN ks65h993556 4 36 + + SYM ks65h993556 4 37 substituted substituted ADJ ks65h993556 4 38 site site NOUN ks65h993556 4 39 that that PRON ks65h993556 4 40 gives give VERB ks65h993556 4 41 another another DET ks65h993556 4 42 -1 -1 ADJ ks65h993556 4 43 charge charge NOUN ks65h993556 4 44 in in ADP ks65h993556 4 45 the the DET ks65h993556 4 46 ring ring NOUN ks65h993556 4 47 . . PUNCT ks65h993556 5 1 these these DET ks65h993556 5 2 two two NUM ks65h993556 5 3 al3 al3 NOUN ks65h993556 5 4 + + CCONJ ks65h993556 5 5 form form VERB ks65h993556 5 6 a a DET ks65h993556 5 7 -2 -2 NOUN ks65h993556 5 8 charge charge NOUN ks65h993556 5 9 al al PROPN ks65h993556 5 10 pair pair NOUN ks65h993556 5 11 in in ADP ks65h993556 5 12 the the DET ks65h993556 5 13 ring ring NOUN ks65h993556 5 14 . . PUNCT ks65h993556 6 1 altogether altogether ADV ks65h993556 6 2 , , PUNCT ks65h993556 6 3 these these DET ks65h993556 6 4 negative negative ADJ ks65h993556 6 5 charges charge NOUN ks65h993556 6 6 can can AUX ks65h993556 6 7 be be AUX ks65h993556 6 8 compensated compensate VERB ks65h993556 6 9 by by ADP ks65h993556 6 10 many many ADJ ks65h993556 6 11 types type NOUN ks65h993556 6 12 of of ADP ks65h993556 6 13 cations cation NOUN ks65h993556 6 14 , , PUNCT ks65h993556 6 15 such such ADJ ks65h993556 6 16 as as ADP ks65h993556 6 17 bronsted bronsted ADJ ks65h993556 6 18 acids acid NOUN ks65h993556 6 19 ( ( PUNCT ks65h993556 6 20 h+ h+ PROPN ks65h993556 6 21 ) ) PUNCT ks65h993556 6 22 , , PUNCT ks65h993556 6 23 metal metal NOUN ks65h993556 6 24 cations cation NOUN ks65h993556 6 25 ( ( PUNCT ks65h993556 6 26 cu2 cu2 NOUN ks65h993556 6 27 + + NOUN ks65h993556 6 28 , , PUNCT ks65h993556 6 29 fe3 fe3 PROPN ks65h993556 6 30 + + NUM ks65h993556 6 31 ) ) PUNCT ks65h993556 6 32 , , PUNCT ks65h993556 6 33 or or CCONJ ks65h993556 6 34 metal metal NOUN ks65h993556 6 35 combinations combination NOUN ks65h993556 6 36 with with ADP ks65h993556 6 37 oxygen oxygen NOUN ks65h993556 6 38 and and CCONJ ks65h993556 6 39 hydrogen hydrogen NOUN ks65h993556 6 40 ( ( PUNCT ks65h993556 6 41 cuoh+ cuoh+ PROPN ks65h993556 6 42 , , PUNCT ks65h993556 6 43 fe(oh)2+).7,8 fe(oh)2+).7,8 VERB ks65h993556 6 44 copper copper NOUN ks65h993556 6 45 is be AUX ks65h993556 6 46 a a DET ks65h993556 6 47 common common ADJ ks65h993556 6 48 species specie NOUN ks65h993556 6 49 in in ADP ks65h993556 6 50 ssz-13 ssz-13 PROPN ks65h993556 6 51 due due ADP ks65h993556 6 52 to to ADP ks65h993556 6 53 its its PRON ks65h993556 6 54 excellent excellent ADJ ks65h993556 6 55 catalytic catalytic ADJ ks65h993556 6 56 properties property NOUN ks65h993556 6 57 in in ADP ks65h993556 6 58 scr scr NOUN ks65h993556 6 59 and and CCONJ ks65h993556 6 60 partial partial ADJ ks65h993556 6 61 methane methane NOUN ks65h993556 6 62 oxidation oxidation NOUN ks65h993556 6 63 ( ( PUNCT ks65h993556 6 64 pmo).10,18,19 pmo).10,18,19 PROPN ks65h993556 6 65 in in ADP ks65h993556 6 66 copper copper NOUN ks65h993556 6 67 exchange exchange PROPN ks65h993556 6 68 , , PUNCT ks65h993556 6 69 copper copper NOUN ks65h993556 6 70 prefers prefer VERB ks65h993556 6 71 to to PART ks65h993556 6 72 be be AUX ks65h993556 6 73 located locate VERB ks65h993556 6 74 either either CCONJ ks65h993556 6 75 in in ADP ks65h993556 6 76 the the DET ks65h993556 6 77 6mr 6mr NOUN ks65h993556 6 78 as as ADP ks65h993556 6 79 cu2 cu2 SPACE ks65h993556 6 80 + + NUM ks65h993556 6 81 or or CCONJ ks65h993556 6 82 the the DET ks65h993556 6 83 8mr 8mr NOUN ks65h993556 6 84 as as SCONJ ks65h993556 6 85 cuoh+.20,21 cuoh+.20,21 ADP ks65h993556 6 86 the the DET ks65h993556 6 87 siting siting NOUN ks65h993556 6 88 of of ADP ks65h993556 6 89 copper copper NOUN ks65h993556 6 90 species specie NOUN ks65h993556 6 91 strongly strongly ADV ks65h993556 6 92 depends depend VERB ks65h993556 6 93 on on ADP ks65h993556 6 94 the the DET ks65h993556 6 95 availability availability NOUN ks65h993556 6 96 of of ADP ks65h993556 6 97 the the DET ks65h993556 6 98 ' ' PUNCT ks65h993556 6 99 low low ADJ ks65h993556 6 100 energy energy NOUN ks65h993556 6 101 ' ' PART ks65h993556 6 102 sites site NOUN ks65h993556 6 103 present present ADJ ks65h993556 6 104 in in ADP ks65h993556 6 105 these these DET ks65h993556 6 106 membered membered NOUN ks65h993556 6 107 - - PUNCT ks65h993556 6 108 rings ring NOUN ks65h993556 6 109 . . PUNCT ks65h993556 7 1 thus thus ADV ks65h993556 7 2 , , PUNCT ks65h993556 7 3 researchers researcher NOUN ks65h993556 7 4 have have AUX ks65h993556 7 5 formulated formulate VERB ks65h993556 7 6 a a DET ks65h993556 7 7 way way NOUN ks65h993556 7 8 to to PART ks65h993556 7 9 estimate estimate VERB ks65h993556 7 10 the the DET ks65h993556 7 11 number number NOUN ks65h993556 7 12 of of ADP ks65h993556 7 13 these these DET ks65h993556 7 14 preferred preferred ADJ ks65h993556 7 15 sites site NOUN ks65h993556 7 16 using use VERB ks65h993556 7 17 composition composition NOUN ks65h993556 7 18 parameters parameter NOUN ks65h993556 7 19 such such ADJ ks65h993556 7 20 as as ADP ks65h993556 7 21 si si PROPN ks65h993556 7 22 / / SYM ks65h993556 7 23 al al PROPN ks65h993556 7 24 and and CCONJ ks65h993556 7 25 cu cu PROPN ks65h993556 7 26 / / SYM ks65h993556 7 27 al al PROPN ks65h993556 7 28 ratios.22–24 ratios.22–24 PROPN ks65h993556 7 29 in in ADP ks65h993556 7 30 fact fact NOUN ks65h993556 7 31 , , PUNCT ks65h993556 7 32 quantification quantification NOUN ks65h993556 7 33 of of ADP ks65h993556 7 34 copper copper NOUN ks65h993556 7 35 in in ADP ks65h993556 7 36 zeolite zeolite NOUN ks65h993556 7 37 has have AUX ks65h993556 7 38 long long ADV ks65h993556 7 39 been be AUX ks65h993556 7 40 an an DET ks65h993556 7 41 interest interest NOUN ks65h993556 7 42 to to ADP ks65h993556 7 43 the the DET ks65h993556 7 44 catalyst catalyst NOUN ks65h993556 7 45 community community NOUN ks65h993556 7 46 . . PUNCT ks65h993556 8 1 in in ADP ks65h993556 8 2 literature literature NOUN ks65h993556 8 3 , , PUNCT ks65h993556 8 4 several several ADJ ks65h993556 8 5 spectroscopic spectroscopic ADJ ks65h993556 8 6 and and CCONJ ks65h993556 8 7 molecular molecular ADJ ks65h993556 8 8 adsorption adsorption NOUN ks65h993556 8 9 methods method NOUN ks65h993556 8 10 have have AUX ks65h993556 8 11 been be AUX ks65h993556 8 12 proposed propose VERB ks65h993556 8 13 and and CCONJ ks65h993556 8 14 studied study VERB ks65h993556 8 15 . . PUNCT ks65h993556 9 1 in in ADP ks65h993556 9 2 one one NUM ks65h993556 9 3 of of ADP ks65h993556 9 4 those those DET ks65h993556 9 5 works work NOUN ks65h993556 9 6 , , PUNCT ks65h993556 9 7 paolucci paolucci PROPN ks65h993556 9 8 et et PROPN ks65h993556 9 9 al al PROPN ks65h993556 9 10 . . PROPN ks65h993556 9 11 measured measure VERB ks65h993556 9 12 the the DET ks65h993556 9 13 proportion proportion NOUN ks65h993556 9 14 of of ADP ks65h993556 9 15 cu2 cu2 SPACE ks65h993556 9 16 + + NOUN ks65h993556 9 17 and and CCONJ ks65h993556 9 18 cuoh+ cuoh+ PROPN ks65h993556 9 19 by by ADP ks65h993556 9 20 reducing reduce VERB ks65h993556 9 21 the the DET ks65h993556 9 22 copper copper NOUN ks65h993556 9 23 species specie NOUN ks65h993556 9 24 with with ADP ks65h993556 9 25 no+nh3 no+nh3 NOUN ks65h993556 9 26 reduction reduction NOUN ks65h993556 9 27 and and CCONJ ks65h993556 9 28 ammonia ammonia NOUN ks65h993556 9 29 temperature temperature NOUN ks65h993556 9 30 programmed program VERB ks65h993556 9 31 desorption desorption NOUN ks65h993556 9 32 ( ( PUNCT ks65h993556 9 33 nh3 nh3 NOUN ks65h993556 9 34 - - NOUN ks65h993556 9 35 tpd).28–30 tpd).28–30 X ks65h993556 9 36 the the DET ks65h993556 9 37 presence presence NOUN ks65h993556 9 38 of of ADP ks65h993556 9 39 no no PRON ks65h993556 9 40 and and CCONJ ks65h993556 9 41 nh3 nh3 PRON ks65h993556 9 42 reduces reduce VERB ks65h993556 9 43 cu2 cu2 SPACE ks65h993556 9 44 + + NUM ks65h993556 9 45 into into ADP ks65h993556 9 46 cu+ cu+ PROPN ks65h993556 9 47 and and CCONJ ks65h993556 9 48 h+ h+ PROPN ks65h993556 9 49 while while SCONJ ks65h993556 9 50 it it PRON ks65h993556 9 51 reduces reduce VERB ks65h993556 9 52 cuoh+ cuoh+ PROPN ks65h993556 9 53 into into ADP ks65h993556 9 54 cu+.31,32 cu+.31,32 PROPN ks65h993556 9 55 when when SCONJ ks65h993556 9 56 nh3 nh3 PRON ks65h993556 9 57 is be AUX ks65h993556 9 58 introduced introduce VERB ks65h993556 9 59 to to ADP ks65h993556 9 60 the the DET ks65h993556 9 61 species specie NOUN ks65h993556 9 62 after after ADP ks65h993556 9 63 reduction reduction NOUN ks65h993556 9 64 , , PUNCT ks65h993556 9 65 it it PRON ks65h993556 9 66 adsorbs adsorb VERB ks65h993556 9 67 on on ADP ks65h993556 9 68 both both DET ks65h993556 9 69 cu+ cu+ PROPN ks65h993556 9 70 and and CCONJ ks65h993556 9 71 h+ h+ PROPN ks65h993556 9 72 sites.33,34 sites.33,34 PROPN ks65h993556 9 73 when when SCONJ ks65h993556 9 74 temperature temperature NOUN ks65h993556 9 75 ramps ramp VERB ks65h993556 9 76 up up ADV ks65h993556 9 77 , , PUNCT ks65h993556 9 78 the the DET ks65h993556 9 79 temperature temperature NOUN ks65h993556 9 80 which which PRON ks65h993556 9 81 nh3 nh3 DET ks65h993556 9 82 desorbs desorb NOUN ks65h993556 9 83 will will AUX ks65h993556 9 84 tell tell VERB ks65h993556 9 85 the the DET ks65h993556 9 86 number number NOUN ks65h993556 9 87 of of ADP ks65h993556 9 88 cu+ cu+ PROPN ks65h993556 9 89 and and CCONJ ks65h993556 9 90 h+ h+ PROPN ks65h993556 9 91 sites site NOUN ks65h993556 9 92 available available ADJ ks65h993556 9 93 in in ADP ks65h993556 9 94 the the DET ks65h993556 9 95 zeolite zeolite NOUN ks65h993556 9 96 . . PUNCT ks65h993556 10 1 comparing compare VERB ks65h993556 10 2 with with ADP ks65h993556 10 3 a a DET ks65h993556 10 4 nh3 nh3 ADJ ks65h993556 10 5 - - PUNCT ks65h993556 10 6 tpd tpd NOUN ks65h993556 10 7 conducted conduct VERB ks65h993556 10 8 before before ADP ks65h993556 10 9 the the DET ks65h993556 10 10 reduction reduction NOUN ks65h993556 10 11 step step NOUN ks65h993556 10 12 , , PUNCT ks65h993556 10 13 the the DET ks65h993556 10 14 quantity quantity NOUN ks65h993556 10 15 of of ADP ks65h993556 10 16 cu2 cu2 SPACE ks65h993556 10 17 + + NOUN ks65h993556 10 18 and and CCONJ ks65h993556 10 19 cuoh+ cuoh+ PROPN ks65h993556 10 20 can can AUX ks65h993556 10 21 then then ADV ks65h993556 10 22 be be AUX ks65h993556 10 23 counted count VERB ks65h993556 10 24 . . PUNCT ks65h993556 11 1 though though SCONJ ks65h993556 11 2 nh3 nh3 ADJ ks65h993556 11 3 - - PUNCT ks65h993556 11 4 tpd tpd PROPN ks65h993556 11 5 works work VERB ks65h993556 11 6 satisfactorily satisfactorily ADV ks65h993556 11 7 in in ADP ks65h993556 11 8 the the DET ks65h993556 11 9 study study NOUN ks65h993556 11 10 , , PUNCT ks65h993556 11 11 it it PRON ks65h993556 11 12 rarely rarely ADV ks65h993556 11 13 serves serve VERB ks65h993556 11 14 as as ADP ks65h993556 11 15 a a DET ks65h993556 11 16 final final ADJ ks65h993556 11 17 step step NOUN ks65h993556 11 18 to to PART ks65h993556 11 19 quantify quantify VERB ks65h993556 11 20 cu2 cu2 SPACE ks65h993556 11 21 + + NUM ks65h993556 11 22 and and CCONJ ks65h993556 11 23 cuoh+ cuoh+ PROPN ks65h993556 11 24 . . PUNCT ks65h993556 12 1 thus thus ADV ks65h993556 12 2 , , PUNCT ks65h993556 12 3 several several ADJ ks65h993556 12 4 interrogation interrogation NOUN ks65h993556 12 5 methods method NOUN ks65h993556 12 6 are be AUX ks65h993556 12 7 used use VERB ks65h993556 12 8 to to PART ks65h993556 12 9 complement complement VERB ks65h993556 12 10 each each PRON ks65h993556 12 11 other.24,33,35,36hydrogen other.24,33,35,36hydrogen ADP ks65h993556 12 12 temperature temperature NOUN ks65h993556 12 13 programmed program VERB ks65h993556 12 14 reduction reduction NOUN ks65h993556 12 15 ( ( PUNCT ks65h993556 12 16 h2 h2 NOUN ks65h993556 12 17 - - PUNCT ks65h993556 12 18 tpr tpr PROPN ks65h993556 12 19 ) ) PUNCT ks65h993556 12 20 is be AUX ks65h993556 12 21 an an DET ks65h993556 12 22 easy easy ADJ ks65h993556 12 23 and and CCONJ ks65h993556 12 24 direct direct ADJ ks65h993556 12 25 method method NOUN ks65h993556 12 26 to to PART ks65h993556 12 27 quantify quantify VERB ks65h993556 12 28 cu2 cu2 SPACE ks65h993556 12 29 + + NUM ks65h993556 12 30 and and CCONJ ks65h993556 12 31 cuoh+ cuoh+ PROPN ks65h993556 12 32 . . PUNCT ks65h993556 13 1 h2 h2 PROPN ks65h993556 13 2 is be AUX ks65h993556 13 3 a a DET ks65h993556 13 4 simple simple ADJ ks65h993556 13 5 molecule molecule NOUN ks65h993556 13 6 compared compare VERB ks65h993556 13 7 to to ADP ks65h993556 13 8 nh3 nh3 PROPN ks65h993556 13 9 . . PROPN ks65h993556 14 1 it it PRON ks65h993556 14 2 adsorbs adsorb VERB ks65h993556 14 3 directly directly ADV ks65h993556 14 4 onto onto ADP ks65h993556 14 5 cu2 cu2 SPACE ks65h993556 14 6 + + NOUN ks65h993556 14 7 and and CCONJ ks65h993556 14 8 cuoh+ cuoh+ PROPN ks65h993556 14 9 instead instead ADV ks65h993556 14 10 of of ADP ks65h993556 14 11 using use VERB ks65h993556 14 12 cu+ cu+ PROPN ks65h993556 14 13 and and CCONJ ks65h993556 14 14 h+ h+ PROPN ks65h993556 14 15 as as ADP ks65h993556 14 16 surrogates surrogate NOUN ks65h993556 14 17 as as ADP ks65h993556 14 18 in in ADP ks65h993556 14 19 nh3 nh3 NOUN ks65h993556 14 20 - - NOUN ks65h993556 14 21 tpd tpd PROPN ks65h993556 14 22 . . PROPN ks65h993556 15 1 however however ADV ks65h993556 15 2 , , PUNCT ks65h993556 15 3 it it PRON ks65h993556 15 4 also also ADV ks65h993556 15 5 shares share VERB ks65h993556 15 6 a a DET ks65h993556 15 7 similar similar ADJ ks65h993556 15 8 shortcoming shortcoming NOUN ks65h993556 15 9 with with ADP ks65h993556 15 10 nh3 nh3 NOUN ks65h993556 15 11 - - NOUN ks65h993556 15 12 tpd tpd NOUN ks65h993556 15 13 , , PUNCT ks65h993556 15 14 among among ADP ks65h993556 15 15 others other NOUN ks65h993556 15 16 . . PUNCT ks65h993556 16 1 in in ADP ks65h993556 16 2 its its PRON ks65h993556 16 3 case case NOUN ks65h993556 16 4 , , PUNCT ks65h993556 16 5 the the DET ks65h993556 16 6 type type NOUN ks65h993556 16 7 of of ADP ks65h993556 16 8 intermediary intermediary ADJ ks65h993556 16 9 species specie NOUN ks65h993556 16 10 and and CCONJ ks65h993556 16 11 their their PRON ks65h993556 16 12 formation formation NOUN ks65h993556 16 13 steps step NOUN ks65h993556 16 14 in in ADP ks65h993556 16 15 h2 h2 NOUN ks65h993556 16 16 reduction reduction NOUN ks65h993556 16 17 of of ADP ks65h993556 16 18 cu2 cu2 SPACE ks65h993556 16 19 + + NOUN ks65h993556 16 20 and and CCONJ ks65h993556 16 21 cuoh+ cuoh+ PROPN ks65h993556 16 22 have have AUX ks65h993556 16 23 yet yet ADV ks65h993556 16 24 been be AUX ks65h993556 16 25 understood understand VERB ks65h993556 16 26 . . PUNCT ks65h993556 17 1 in in ADP ks65h993556 17 2 a a DET ks65h993556 17 3 big big ADJ ks65h993556 17 4 picture picture NOUN ks65h993556 17 5 , , PUNCT ks65h993556 17 6 the the DET ks65h993556 17 7 elementary elementary ADJ ks65h993556 17 8 steps step NOUN ks65h993556 17 9 of of ADP ks65h993556 17 10 getting get VERB ks65h993556 17 11 from from ADP ks65h993556 17 12 the the DET ks65h993556 17 13 reactants reactant NOUN ks65h993556 17 14 ( ( PUNCT ks65h993556 17 15 h2 h2 PROPN ks65h993556 17 16 , , PUNCT ks65h993556 17 17 cu2 cu2 SPACE ks65h993556 17 18 + + NUM ks65h993556 17 19 , , PUNCT ks65h993556 17 20 and and CCONJ ks65h993556 17 21 cuoh+ cuoh+ PROPN ks65h993556 17 22 ) ) PUNCT ks65h993556 17 23 to to ADP ks65h993556 17 24 the the DET ks65h993556 17 25 products product NOUN ks65h993556 17 26 ( ( PUNCT ks65h993556 17 27 h2 h2 PROPN ks65h993556 17 28 , , PUNCT ks65h993556 17 29 h2o h2o PROPN ks65h993556 17 30 , , PUNCT ks65h993556 17 31 cu+ cu+ PROPN ks65h993556 17 32 , , PUNCT ks65h993556 17 33 and and CCONJ ks65h993556 17 34 cu+/h+ cu+/h+ PROPN ks65h993556 17 35 ) ) PUNCT ks65h993556 17 36 are be AUX ks65h993556 17 37 not not PART ks65h993556 17 38 yet yet ADV ks65h993556 17 39 understood understand VERB ks65h993556 17 40 . . PUNCT ks65h993556 18 1 therefore therefore ADV ks65h993556 18 2 , , PUNCT ks65h993556 18 3 this this DET ks65h993556 18 4 work work NOUN ks65h993556 18 5 will will AUX ks65h993556 18 6 investigate investigate VERB ks65h993556 18 7 their their PRON ks65h993556 18 8 reduction reduction NOUN ks65h993556 18 9 mechanisms mechanism NOUN ks65h993556 18 10 in in ADP ks65h993556 18 11 ssz-13 ssz-13 PROPN ks65h993556 18 12 zeolite zeolite NOUN ks65h993556 18 13 through through ADP ks65h993556 18 14 making make VERB ks65h993556 18 15 and and CCONJ ks65h993556 18 16 validating validate VERB ks65h993556 18 17 hypothesis hypothesis NOUN ks65h993556 18 18 on on ADP ks65h993556 18 19 their their PRON ks65h993556 18 20 reaction reaction NOUN ks65h993556 18 21 mechanisms mechanism NOUN ks65h993556 18 22 . . PUNCT ks65h993556 19 1 the the DET ks65h993556 19 2 understanding understanding NOUN ks65h993556 19 3 of of ADP ks65h993556 19 4 this this DET ks65h993556 19 5 copper copper NOUN ks65h993556 19 6 reduction reduction NOUN ks65h993556 19 7 mechanism mechanism NOUN ks65h993556 19 8 has have VERB ks65h993556 19 9 an an DET ks65h993556 19 10 impact impact NOUN ks65h993556 19 11 in in ADP ks65h993556 19 12 the the DET ks65h993556 19 13 understanding understanding NOUN ks65h993556 19 14 of of ADP ks65h993556 19 15 copper copper NOUN ks65h993556 19 16 reduction reduction NOUN ks65h993556 19 17 pathway pathway NOUN ks65h993556 19 18 , , PUNCT ks65h993556 19 19 the the DET ks65h993556 19 20 types type NOUN ks65h993556 19 21 of of ADP ks65h993556 19 22 intermediate intermediate ADJ ks65h993556 19 23 species specie NOUN ks65h993556 19 24 , , PUNCT ks65h993556 19 25 and and CCONJ ks65h993556 19 26 possibly possibly ADV ks65h993556 19 27 the the DET ks65h993556 19 28 effects effect NOUN ks65h993556 19 29 of of ADP ks65h993556 19 30 water water NOUN ks65h993556 19 31 solvation solvation NOUN ks65h993556 19 32 on on ADP ks65h993556 19 33 copper copper NOUN ks65h993556 19 34 reduction reduction NOUN ks65h993556 19 35 rate rate NOUN ks65h993556 19 36 . . PUNCT