id	sid	tid	token	lemma	pos
gm80ht27s6q	1	1	many	many	ADJ
gm80ht27s6q	1	2	fundamental	fundamental	ADJ
gm80ht27s6q	1	3	processes	process	NOUN
gm80ht27s6q	1	4	in	in	ADP
gm80ht27s6q	1	5	nature	nature	NOUN
gm80ht27s6q	1	6	and	and	CCONJ
gm80ht27s6q	1	7	technology	technology	NOUN
gm80ht27s6q	1	8	,	,	PUNCT
gm80ht27s6q	1	9	from	from	ADP
gm80ht27s6q	1	10	the	the	DET
gm80ht27s6q	1	11	electronic	electronic	ADJ
gm80ht27s6q	1	12	energy	energy	NOUN
gm80ht27s6q	1	13	transfer	transfer	NOUN
gm80ht27s6q	1	14	in	in	ADP
gm80ht27s6q	1	15	biological	biological	ADJ
gm80ht27s6q	1	16	photosynthetic	photosynthetic	ADJ
gm80ht27s6q	1	17	complexes	complex	NOUN
gm80ht27s6q	1	18	to	to	ADP
gm80ht27s6q	1	19	the	the	DET
gm80ht27s6q	1	20	charge	charge	NOUN
gm80ht27s6q	1	21	mobility	mobility	NOUN
gm80ht27s6q	1	22	in	in	ADP
gm80ht27s6q	1	23	solid	solid	ADJ
gm80ht27s6q	1	24	-	-	PUNCT
gm80ht27s6q	1	25	state	state	NOUN
gm80ht27s6q	1	26	photovoltaic	photovoltaic	ADJ
gm80ht27s6q	1	27	devices	device	NOUN
gm80ht27s6q	1	28	,	,	PUNCT
gm80ht27s6q	1	29	involve	involve	VERB
gm80ht27s6q	1	30	the	the	DET
gm80ht27s6q	1	31	dynamics	dynamic	NOUN
gm80ht27s6q	1	32	of	of	ADP
gm80ht27s6q	1	33	electrons	electron	NOUN
gm80ht27s6q	1	34	in	in	ADP
gm80ht27s6q	1	35	complex	complex	ADJ
gm80ht27s6q	1	36	molecular	molecular	ADJ
gm80ht27s6q	1	37	systems	system	NOUN
gm80ht27s6q	1	38	and	and	CCONJ
gm80ht27s6q	1	39	nanostructures	nanostructure	NOUN
gm80ht27s6q	1	40	.	.	PUNCT
gm80ht27s6q	2	1	therefore	therefore	ADV
gm80ht27s6q	2	2	,	,	PUNCT
gm80ht27s6q	2	3	understanding	understand	VERB
gm80ht27s6q	2	4	the	the	DET
gm80ht27s6q	2	5	dynamical	dynamical	ADJ
gm80ht27s6q	2	6	characteristics	characteristic	NOUN
gm80ht27s6q	2	7	of	of	ADP
gm80ht27s6q	2	8	electronic	electronic	ADJ
gm80ht27s6q	2	9	states	state	NOUN
gm80ht27s6q	2	10	is	be	AUX
gm80ht27s6q	2	11	crucial	crucial	ADJ
gm80ht27s6q	2	12	for	for	ADP
gm80ht27s6q	2	13	rational	rational	ADJ
gm80ht27s6q	2	14	designs	design	NOUN
gm80ht27s6q	2	15	of	of	ADP
gm80ht27s6q	2	16	functional	functional	ADJ
gm80ht27s6q	2	17	materials	material	NOUN
gm80ht27s6q	2	18	.	.	PUNCT
gm80ht27s6q	3	1	to	to	PART
gm80ht27s6q	3	2	make	make	VERB
gm80ht27s6q	3	3	progresses	progress	NOUN
gm80ht27s6q	3	4	toward	toward	ADP
gm80ht27s6q	3	5	this	this	DET
gm80ht27s6q	3	6	goal	goal	NOUN
gm80ht27s6q	3	7	,	,	PUNCT
gm80ht27s6q	3	8	we	we	PRON
gm80ht27s6q	3	9	have	have	AUX
gm80ht27s6q	3	10	developed	develop	VERB
gm80ht27s6q	3	11	time	time	NOUN
gm80ht27s6q	3	12	-	-	PUNCT
gm80ht27s6q	3	13	dependent	dependent	ADJ
gm80ht27s6q	3	14	open	open	ADJ
gm80ht27s6q	3	15	-	-	PUNCT
gm80ht27s6q	3	16	system	system	NOUN
gm80ht27s6q	3	17	self	self	NOUN
gm80ht27s6q	3	18	-	-	PUNCT
gm80ht27s6q	3	19	consistent	consistent	ADJ
gm80ht27s6q	3	20	field	field	NOUN
gm80ht27s6q	3	21	at	at	ADP
gm80ht27s6q	3	22	second	second	ADJ
gm80ht27s6q	3	23	order	order	NOUN
gm80ht27s6q	3	24	(	(	PUNCT
gm80ht27s6q	3	25	oscf2	oscf2	NOUN
gm80ht27s6q	3	26	)	)	PUNCT
gm80ht27s6q	3	27	,	,	PUNCT
gm80ht27s6q	3	28	a	a	DET
gm80ht27s6q	3	29	real	real	ADJ
gm80ht27s6q	3	30	-	-	PUNCT
gm80ht27s6q	3	31	time	time	NOUN
gm80ht27s6q	3	32	time	time	NOUN
gm80ht27s6q	3	33	-	-	PUNCT
gm80ht27s6q	3	34	dependent	dependent	ADJ
gm80ht27s6q	3	35	functional	functional	ADJ
gm80ht27s6q	3	36	theory	theory	NOUN
gm80ht27s6q	3	37	method	method	NOUN
gm80ht27s6q	3	38	incorporated	incorporate	VERB
gm80ht27s6q	3	39	with	with	ADP
gm80ht27s6q	3	40	open	open	ADJ
gm80ht27s6q	3	41	quantum	quantum	NOUN
gm80ht27s6q	3	42	systems	system	NOUN
gm80ht27s6q	3	43	theory	theory	NOUN
gm80ht27s6q	3	44	.	.	PUNCT
gm80ht27s6q	4	1	this	this	DET
gm80ht27s6q	4	2	dissertation	dissertation	NOUN
gm80ht27s6q	4	3	focuses	focus	VERB
gm80ht27s6q	4	4	on	on	ADP
gm80ht27s6q	4	5	the	the	DET
gm80ht27s6q	4	6	derivation	derivation	NOUN
gm80ht27s6q	4	7	and	and	CCONJ
gm80ht27s6q	4	8	implementation	implementation	NOUN
gm80ht27s6q	4	9	of	of	ADP
gm80ht27s6q	4	10	oscf2	oscf2	NOUN
gm80ht27s6q	4	11	,	,	PUNCT
gm80ht27s6q	4	12	and	and	CCONJ
gm80ht27s6q	4	13	explores	explore	VERB
gm80ht27s6q	4	14	its	its	PRON
gm80ht27s6q	4	15	applicability	applicability	NOUN
gm80ht27s6q	4	16	in	in	ADP
gm80ht27s6q	4	17	realistic	realistic	ADJ
gm80ht27s6q	4	18	,	,	PUNCT
gm80ht27s6q	4	19	chemically	chemically	ADV
gm80ht27s6q	4	20	relevant	relevant	ADJ
gm80ht27s6q	4	21	molecular	molecular	ADJ
gm80ht27s6q	4	22	systems	system	NOUN
gm80ht27s6q	4	23	.	.	PUNCT
gm80ht27s6q	5	1	the	the	DET
gm80ht27s6q	5	2	contribution	contribution	NOUN
gm80ht27s6q	5	3	of	of	ADP
gm80ht27s6q	5	4	the	the	DET
gm80ht27s6q	5	5	present	present	ADJ
gm80ht27s6q	5	6	work	work	NOUN
gm80ht27s6q	5	7	is	be	AUX
gm80ht27s6q	5	8	three	three	NUM
gm80ht27s6q	5	9	-	-	ADJ
gm80ht27s6q	5	10	fold	fold	ADJ
gm80ht27s6q	5	11	.	.	PUNCT
gm80ht27s6q	6	1	first	first	ADV
gm80ht27s6q	6	2	,	,	PUNCT
gm80ht27s6q	6	3	we	we	PRON
gm80ht27s6q	6	4	derive	derive	VERB
gm80ht27s6q	6	5	a	a	DET
gm80ht27s6q	6	6	new	new	ADJ
gm80ht27s6q	6	7	dissipative	dissipative	ADJ
gm80ht27s6q	6	8	theory	theory	NOUN
gm80ht27s6q	6	9	for	for	ADP
gm80ht27s6q	6	10	electrons	electron	NOUN
gm80ht27s6q	6	11	in	in	ADP
gm80ht27s6q	6	12	energetic	energetic	ADJ
gm80ht27s6q	6	13	contact	contact	NOUN
gm80ht27s6q	6	14	with	with	ADP
gm80ht27s6q	6	15	the	the	DET
gm80ht27s6q	6	16	environment	environment	NOUN
gm80ht27s6q	6	17	that	that	PRON
gm80ht27s6q	6	18	causes	cause	VERB
gm80ht27s6q	6	19	the	the	DET
gm80ht27s6q	6	20	electronic	electronic	ADJ
gm80ht27s6q	6	21	populations	population	NOUN
gm80ht27s6q	6	22	to	to	PART
gm80ht27s6q	6	23	naturally	naturally	ADV
gm80ht27s6q	6	24	relax	relax	VERB
gm80ht27s6q	6	25	to	to	ADP
gm80ht27s6q	6	26	a	a	DET
gm80ht27s6q	6	27	fermi	fermi	NOUN
gm80ht27s6q	6	28	-	-	PUNCT
gm80ht27s6q	6	29	dirac	dirac	NOUN
gm80ht27s6q	6	30	thermal	thermal	ADJ
gm80ht27s6q	6	31	equilibrium	equilibrium	NOUN
gm80ht27s6q	6	32	statistics	statistic	NOUN
gm80ht27s6q	6	33	limit	limit	NOUN
gm80ht27s6q	6	34	.	.	PUNCT
gm80ht27s6q	7	1	second	second	ADV
gm80ht27s6q	7	2	,	,	PUNCT
gm80ht27s6q	7	3	we	we	PRON
gm80ht27s6q	7	4	present	present	VERB
gm80ht27s6q	7	5	a	a	DET
gm80ht27s6q	7	6	complete	complete	ADJ
gm80ht27s6q	7	7	implementation	implementation	NOUN
gm80ht27s6q	7	8	of	of	ADP
gm80ht27s6q	7	9	oscf2	oscf2	NOUN
gm80ht27s6q	7	10	for	for	ADP
gm80ht27s6q	7	11	real	real	ADJ
gm80ht27s6q	7	12	-	-	PUNCT
gm80ht27s6q	7	13	time	time	NOUN
gm80ht27s6q	7	14	simulations	simulation	NOUN
gm80ht27s6q	7	15	of	of	ADP
gm80ht27s6q	7	16	chemical	chemical	NOUN
gm80ht27s6q	7	17	systems	system	NOUN
gm80ht27s6q	7	18	including	include	VERB
gm80ht27s6q	7	19	the	the	DET
gm80ht27s6q	7	20	treatment	treatment	NOUN
gm80ht27s6q	7	21	of	of	ADP
gm80ht27s6q	7	22	energy	energy	NOUN
gm80ht27s6q	7	23	dissipation	dissipation	NOUN
gm80ht27s6q	7	24	.	.	PUNCT
gm80ht27s6q	8	1	the	the	DET
gm80ht27s6q	8	2	cubic	cubic	ADJ
gm80ht27s6q	8	3	scaling	scaling	NOUN
gm80ht27s6q	8	4	achieved	achieve	VERB
gm80ht27s6q	8	5	through	through	ADP
gm80ht27s6q	8	6	highly	highly	ADV
gm80ht27s6q	8	7	efficient	efficient	ADJ
gm80ht27s6q	8	8	algorithms	algorithm	NOUN
gm80ht27s6q	8	9	means	mean	VERB
gm80ht27s6q	8	10	oscf2	oscf2	ADJ
gm80ht27s6q	8	11	is	be	AUX
gm80ht27s6q	8	12	computationally	computationally	ADV
gm80ht27s6q	8	13	inexpensive	inexpensive	ADJ
gm80ht27s6q	8	14	compared	compare	VERB
gm80ht27s6q	8	15	to	to	ADP
gm80ht27s6q	8	16	existing	exist	VERB
gm80ht27s6q	8	17	real	real	ADJ
gm80ht27s6q	8	18	-	-	PUNCT
gm80ht27s6q	8	19	time	time	NOUN
gm80ht27s6q	8	20	dynamics	dynamic	NOUN
gm80ht27s6q	8	21	codes	code	NOUN
gm80ht27s6q	8	22	.	.	PUNCT
gm80ht27s6q	9	1	we	we	PRON
gm80ht27s6q	9	2	critically	critically	ADV
gm80ht27s6q	9	3	assess	assess	VERB
gm80ht27s6q	9	4	the	the	DET
gm80ht27s6q	9	5	validity	validity	NOUN
gm80ht27s6q	9	6	in	in	ADP
gm80ht27s6q	9	7	numerous	numerous	ADJ
gm80ht27s6q	9	8	simulation	simulation	NOUN
gm80ht27s6q	9	9	studies	study	NOUN
gm80ht27s6q	9	10	and	and	CCONJ
gm80ht27s6q	9	11	demonstrate	demonstrate	VERB
gm80ht27s6q	9	12	that	that	PRON
gm80ht27s6q	9	13	oscf2	oscf2	ADJ
gm80ht27s6q	9	14	consistently	consistently	ADV
gm80ht27s6q	9	15	produces	produce	VERB
gm80ht27s6q	9	16	absorption	absorption	NOUN
gm80ht27s6q	9	17	spectra	spectra	ADJ
gm80ht27s6q	9	18	and	and	CCONJ
gm80ht27s6q	9	19	non	non	ADJ
gm80ht27s6q	9	20	-	-	ADJ
gm80ht27s6q	9	21	radiative	radiative	ADJ
gm80ht27s6q	9	22	relaxation	relaxation	NOUN
gm80ht27s6q	9	23	rates	rate	NOUN
gm80ht27s6q	9	24	which	which	PRON
gm80ht27s6q	9	25	are	be	AUX
gm80ht27s6q	9	26	in	in	ADP
gm80ht27s6q	9	27	good	good	ADJ
gm80ht27s6q	9	28	agreement	agreement	NOUN
gm80ht27s6q	9	29	with	with	ADP
gm80ht27s6q	9	30	experimental	experimental	ADJ
gm80ht27s6q	9	31	results	result	NOUN
gm80ht27s6q	9	32	.	.	PUNCT
gm80ht27s6q	10	1	finally	finally	ADV
gm80ht27s6q	10	2	,	,	PUNCT
gm80ht27s6q	10	3	we	we	PRON
gm80ht27s6q	10	4	present	present	VERB
gm80ht27s6q	10	5	the	the	DET
gm80ht27s6q	10	6	first	first	ADJ
gm80ht27s6q	10	7	ab	ab	PROPN
gm80ht27s6q	10	8	initio	initio	NOUN
gm80ht27s6q	10	9	simulations	simulation	NOUN
gm80ht27s6q	10	10	of	of	ADP
gm80ht27s6q	10	11	transient	transient	ADJ
gm80ht27s6q	10	12	absorption	absorption	NOUN
gm80ht27s6q	10	13	spectra	spectra	NOUN
gm80ht27s6q	10	14	spectroscopy	spectroscopy	NOUN
gm80ht27s6q	10	15	.	.	PUNCT
gm80ht27s6q	11	1	in	in	ADP
gm80ht27s6q	11	2	particular	particular	ADJ
gm80ht27s6q	11	3	,	,	PUNCT
gm80ht27s6q	11	4	the	the	DET
gm80ht27s6q	11	5	transient	transient	ADJ
gm80ht27s6q	11	6	spectrum	spectrum	NOUN
gm80ht27s6q	11	7	and	and	CCONJ
gm80ht27s6q	11	8	relaxation	relaxation	NOUN
gm80ht27s6q	11	9	dynamics	dynamic	NOUN
gm80ht27s6q	11	10	of	of	ADP
gm80ht27s6q	11	11	methylammonium	methylammonium	PROPN
gm80ht27s6q	11	12	lead	lead	PROPN
gm80ht27s6q	11	13	triiodide	triiodide	PROPN
gm80ht27s6q	11	14	perovskite	perovskite	PROPN
gm80ht27s6q	11	15	is	be	AUX
gm80ht27s6q	11	16	investigated	investigate	VERB
gm80ht27s6q	11	17	,	,	PUNCT
gm80ht27s6q	11	18	substantiating	substantiate	VERB
gm80ht27s6q	11	19	the	the	DET
gm80ht27s6q	11	20	assignment	assignment	NOUN
gm80ht27s6q	11	21	of	of	ADP
gm80ht27s6q	11	22	induced	induce	VERB
gm80ht27s6q	11	23	bleach	bleach	NOUN
gm80ht27s6q	11	24	and	and	CCONJ
gm80ht27s6q	11	25	absorption	absorption	NOUN
gm80ht27s6q	11	26	signals	signal	NOUN
gm80ht27s6q	11	27	.	.	PUNCT