id	sid	tid	token	lemma	pos
d504rj4556c	1	1	the	the	DET
d504rj4556c	1	2	burgeoning	burgeon	VERB
d504rj4556c	1	3	class	class	NOUN
d504rj4556c	1	4	of	of	ADP
d504rj4556c	1	5	metal	metal	NOUN
d504rj4556c	1	6	halide	halide	NOUN
d504rj4556c	1	7	perovskites	perovskite	NOUN
d504rj4556c	1	8	constitutes	constitute	VERB
d504rj4556c	1	9	a	a	DET
d504rj4556c	1	10	paradigm	paradigm	NOUN
d504rj4556c	1	11	shift	shift	NOUN
d504rj4556c	1	12	in	in	ADP
d504rj4556c	1	13	the	the	DET
d504rj4556c	1	14	study	study	NOUN
d504rj4556c	1	15	and	and	CCONJ
d504rj4556c	1	16	application	application	NOUN
d504rj4556c	1	17	of	of	ADP
d504rj4556c	1	18	solution	solution	NOUN
d504rj4556c	1	19	-	-	PUNCT
d504rj4556c	1	20	processed	process	VERB
d504rj4556c	1	21	semiconductors	semiconductor	NOUN
d504rj4556c	1	22	.	.	PUNCT
d504rj4556c	2	1	advancements	advancement	NOUN
d504rj4556c	2	2	in	in	ADP
d504rj4556c	2	3	thin	thin	ADJ
d504rj4556c	2	4	film	film	NOUN
d504rj4556c	2	5	processing	processing	NOUN
d504rj4556c	2	6	and	and	CCONJ
d504rj4556c	2	7	our	our	PRON
d504rj4556c	2	8	understanding	understanding	NOUN
d504rj4556c	2	9	of	of	ADP
d504rj4556c	2	10	the	the	DET
d504rj4556c	2	11	underlying	underlie	VERB
d504rj4556c	2	12	structural	structural	ADJ
d504rj4556c	2	13	,	,	PUNCT
d504rj4556c	2	14	photophysical	photophysical	ADJ
d504rj4556c	2	15	,	,	PUNCT
d504rj4556c	2	16	and	and	CCONJ
d504rj4556c	2	17	electronic	electronic	ADJ
d504rj4556c	2	18	properties	property	NOUN
d504rj4556c	2	19	of	of	ADP
d504rj4556c	2	20	these	these	DET
d504rj4556c	2	21	materials	material	NOUN
d504rj4556c	2	22	over	over	ADP
d504rj4556c	2	23	the	the	DET
d504rj4556c	2	24	past	past	ADJ
d504rj4556c	2	25	several	several	ADJ
d504rj4556c	2	26	years	year	NOUN
d504rj4556c	2	27	have	have	AUX
d504rj4556c	2	28	led	lead	VERB
d504rj4556c	2	29	to	to	ADP
d504rj4556c	2	30	development	development	NOUN
d504rj4556c	2	31	of	of	ADP
d504rj4556c	2	32	perovskite	perovskite	ADJ
d504rj4556c	2	33	solar	solar	ADJ
d504rj4556c	2	34	cells	cell	NOUN
d504rj4556c	2	35	with	with	ADP
d504rj4556c	2	36	power	power	NOUN
d504rj4556c	2	37	conversion	conversion	NOUN
d504rj4556c	2	38	efficiencies	efficiency	NOUN
d504rj4556c	2	39	that	that	PRON
d504rj4556c	2	40	rival	rival	VERB
d504rj4556c	2	41	much	much	ADV
d504rj4556c	2	42	more	more	ADV
d504rj4556c	2	43	mature	mature	ADJ
d504rj4556c	2	44	firstand	firstand	ADJ
d504rj4556c	2	45	second	second	ADJ
d504rj4556c	2	46	-	-	PUNCT
d504rj4556c	2	47	generation	generation	NOUN
d504rj4556c	2	48	technologies	technology	NOUN
d504rj4556c	2	49	.	.	PUNCT
d504rj4556c	3	1	characterizing	characterize	VERB
d504rj4556c	3	2	the	the	DET
d504rj4556c	3	3	behavior	behavior	NOUN
d504rj4556c	3	4	of	of	ADP
d504rj4556c	3	5	photogenerated	photogenerate	VERB
d504rj4556c	3	6	charges	charge	NOUN
d504rj4556c	3	7	in	in	ADP
d504rj4556c	3	8	metal	metal	NOUN
d504rj4556c	3	9	halide	halide	NOUN
d504rj4556c	3	10	perovskites	perovskite	NOUN
d504rj4556c	3	11	is	be	AUX
d504rj4556c	3	12	integral	integral	ADJ
d504rj4556c	3	13	for	for	ADP
d504rj4556c	3	14	understanding	understand	VERB
d504rj4556c	3	15	the	the	DET
d504rj4556c	3	16	operating	operate	VERB
d504rj4556c	3	17	principles	principle	NOUN
d504rj4556c	3	18	and	and	CCONJ
d504rj4556c	3	19	fundamental	fundamental	ADJ
d504rj4556c	3	20	limitations	limitation	NOUN
d504rj4556c	3	21	of	of	ADP
d504rj4556c	3	22	perovskite	perovskite	ADJ
d504rj4556c	3	23	optoelectronics	optoelectronic	NOUN
d504rj4556c	3	24	.	.	PUNCT
d504rj4556c	4	1	the	the	DET
d504rj4556c	4	2	majority	majority	NOUN
d504rj4556c	4	3	of	of	ADP
d504rj4556c	4	4	studies	study	NOUN
d504rj4556c	4	5	outlined	outline	VERB
d504rj4556c	4	6	in	in	ADP
d504rj4556c	4	7	this	this	DET
d504rj4556c	4	8	dissertation	dissertation	NOUN
d504rj4556c	4	9	involve	involve	VERB
d504rj4556c	4	10	fundamental	fundamental	ADJ
d504rj4556c	4	11	study	study	NOUN
d504rj4556c	4	12	of	of	ADP
d504rj4556c	4	13	the	the	DET
d504rj4556c	4	14	prototypical	prototypical	ADJ
d504rj4556c	4	15	organic	organic	ADJ
d504rj4556c	4	16	-	-	PUNCT
d504rj4556c	4	17	inorganic	inorganic	ADJ
d504rj4556c	4	18	compound	compound	NOUN
d504rj4556c	4	19	methylammonium	methylammonium	PROPN
d504rj4556c	4	20	lead	lead	PROPN
d504rj4556c	4	21	iodide	iodide	PROPN
d504rj4556c	4	22	(	(	PUNCT
d504rj4556c	4	23	ch3nh3pbi3	ch3nh3pbi3	NOUN
d504rj4556c	4	24	)	)	PUNCT
d504rj4556c	4	25	.	.	PUNCT
d504rj4556c	5	1	time	time	NOUN
d504rj4556c	5	2	-	-	PUNCT
d504rj4556c	5	3	resolved	resolve	VERB
d504rj4556c	5	4	pump	pump	NOUN
d504rj4556c	5	5	-	-	PUNCT
d504rj4556c	5	6	probe	probe	NOUN
d504rj4556c	5	7	spectroscopy	spectroscopy	NOUN
d504rj4556c	5	8	serves	serve	VERB
d504rj4556c	5	9	as	as	ADP
d504rj4556c	5	10	a	a	DET
d504rj4556c	5	11	principle	principle	ADJ
d504rj4556c	5	12	tool	tool	NOUN
d504rj4556c	5	13	in	in	ADP
d504rj4556c	5	14	these	these	DET
d504rj4556c	5	15	investigations	investigation	NOUN
d504rj4556c	5	16	to	to	PART
d504rj4556c	5	17	analyze	analyze	VERB
d504rj4556c	5	18	excited	excited	ADJ
d504rj4556c	5	19	state	state	NOUN
d504rj4556c	5	20	decay	decay	NOUN
d504rj4556c	5	21	kinetics	kinetic	NOUN
d504rj4556c	5	22	and	and	CCONJ
d504rj4556c	5	23	optical	optical	ADJ
d504rj4556c	5	24	nonlinearities	nonlinearitie	NOUN
d504rj4556c	5	25	in	in	ADP
d504rj4556c	5	26	perovskite	perovskite	NOUN
d504rj4556c	5	27	thin	thin	ADJ
d504rj4556c	5	28	films.it	films.it	NUM
d504rj4556c	5	29	is	be	AUX
d504rj4556c	5	30	demonstrated	demonstrate	VERB
d504rj4556c	5	31	herein	herein	ADV
d504rj4556c	5	32	that	that	SCONJ
d504rj4556c	5	33	nonresonant	nonresonant	ADJ
d504rj4556c	5	34	photoexcitation	photoexcitation	NOUN
d504rj4556c	5	35	of	of	ADP
d504rj4556c	5	36	ch3nh3pbi3	ch3nh3pbi3	ADJ
d504rj4556c	5	37	yields	yield	NOUN
d504rj4556c	5	38	a	a	DET
d504rj4556c	5	39	large	large	ADJ
d504rj4556c	5	40	fraction	fraction	NOUN
d504rj4556c	5	41	of	of	ADP
d504rj4556c	5	42	free	free	ADJ
d504rj4556c	5	43	carriers	carrier	NOUN
d504rj4556c	5	44	on	on	ADP
d504rj4556c	5	45	a	a	DET
d504rj4556c	5	46	sub	sub	ADJ
d504rj4556c	5	47	-	-	ADJ
d504rj4556c	5	48	picosecond	picosecond	ADJ
d504rj4556c	5	49	time	time	NOUN
d504rj4556c	5	50	scale	scale	NOUN
d504rj4556c	5	51	.	.	PUNCT
d504rj4556c	6	1	in	in	ADP
d504rj4556c	6	2	practical	practical	ADJ
d504rj4556c	6	3	optoelectronic	optoelectronic	NOUN
d504rj4556c	6	4	applications	application	NOUN
d504rj4556c	6	5	,	,	PUNCT
d504rj4556c	6	6	these	these	DET
d504rj4556c	6	7	photogenerated	photogenerate	VERB
d504rj4556c	6	8	carriers	carrier	NOUN
d504rj4556c	6	9	must	must	AUX
d504rj4556c	6	10	travel	travel	VERB
d504rj4556c	6	11	large	large	ADJ
d504rj4556c	6	12	distances	distance	NOUN
d504rj4556c	6	13	across	across	ADP
d504rj4556c	6	14	the	the	DET
d504rj4556c	6	15	thickness	thickness	NOUN
d504rj4556c	6	16	of	of	ADP
d504rj4556c	6	17	the	the	DET
d504rj4556c	6	18	material	material	NOUN
d504rj4556c	6	19	to	to	PART
d504rj4556c	6	20	realize	realize	VERB
d504rj4556c	6	21	large	large	ADJ
d504rj4556c	6	22	external	external	ADJ
d504rj4556c	6	23	quantum	quantum	NOUN
d504rj4556c	6	24	efficiencies	efficiency	NOUN
d504rj4556c	6	25	and	and	CCONJ
d504rj4556c	6	26	efficient	efficient	ADJ
d504rj4556c	6	27	charge	charge	NOUN
d504rj4556c	6	28	extraction	extraction	NOUN
d504rj4556c	6	29	.	.	PUNCT
d504rj4556c	7	1	using	use	VERB
d504rj4556c	7	2	a	a	DET
d504rj4556c	7	3	powerful	powerful	ADJ
d504rj4556c	7	4	technique	technique	NOUN
d504rj4556c	7	5	known	know	VERB
d504rj4556c	7	6	as	as	ADP
d504rj4556c	7	7	transient	transient	ADJ
d504rj4556c	7	8	absorption	absorption	NOUN
d504rj4556c	7	9	microscopy	microscopy	NOUN
d504rj4556c	7	10	,	,	PUNCT
d504rj4556c	7	11	long	long	ADJ
d504rj4556c	7	12	-	-	PUNCT
d504rj4556c	7	13	range	range	NOUN
d504rj4556c	7	14	carrier	carrier	NOUN
d504rj4556c	7	15	diffusion	diffusion	NOUN
d504rj4556c	7	16	in	in	ADP
d504rj4556c	7	17	a	a	DET
d504rj4556c	7	18	ch3nh3pbi3	ch3nh3pbi3	ADJ
d504rj4556c	7	19	thin	thin	ADJ
d504rj4556c	7	20	film	film	NOUN
d504rj4556c	7	21	is	be	AUX
d504rj4556c	7	22	directly	directly	ADV
d504rj4556c	7	23	imaged	image	VERB
d504rj4556c	7	24	.	.	PUNCT
d504rj4556c	8	1	charges	charge	NOUN
d504rj4556c	8	2	are	be	AUX
d504rj4556c	8	3	unambiguously	unambiguously	ADV
d504rj4556c	8	4	shown	show	VERB
d504rj4556c	8	5	to	to	PART
d504rj4556c	8	6	travel	travel	VERB
d504rj4556c	8	7	220	220	NUM
d504rj4556c	8	8	nm	nm	NOUN
d504rj4556c	8	9	over	over	ADP
d504rj4556c	8	10	the	the	DET
d504rj4556c	8	11	course	course	NOUN
d504rj4556c	8	12	of	of	ADP
d504rj4556c	8	13	2	2	NUM
d504rj4556c	8	14	ns	n	NOUN
d504rj4556c	8	15	after	after	ADP
d504rj4556c	8	16	photoexcitation	photoexcitation	NOUN
d504rj4556c	8	17	,	,	PUNCT
d504rj4556c	8	18	with	with	ADP
d504rj4556c	8	19	an	an	DET
d504rj4556c	8	20	extrapolated	extrapolate	VERB
d504rj4556c	8	21	diffusion	diffusion	NOUN
d504rj4556c	8	22	length	length	NOUN
d504rj4556c	8	23	greater	great	ADJ
d504rj4556c	8	24	than	than	ADP
d504rj4556c	8	25	one	one	NUM
d504rj4556c	8	26	micrometer	micrometer	NOUN
d504rj4556c	8	27	over	over	ADP
d504rj4556c	8	28	the	the	DET
d504rj4556c	8	29	full	full	ADJ
d504rj4556c	8	30	excited	excited	ADJ
d504rj4556c	8	31	state	state	NOUN
d504rj4556c	8	32	lifetime	lifetime	NOUN
d504rj4556c	8	33	.	.	PUNCT
d504rj4556c	9	1	furthermore	furthermore	ADV
d504rj4556c	9	2	,	,	PUNCT
d504rj4556c	9	3	through	through	ADP
d504rj4556c	9	4	structural	structural	ADJ
d504rj4556c	9	5	and	and	CCONJ
d504rj4556c	9	6	steady	steady	ADJ
d504rj4556c	9	7	-	-	PUNCT
d504rj4556c	9	8	state	state	NOUN
d504rj4556c	9	9	and	and	CCONJ
d504rj4556c	9	10	time	time	NOUN
d504rj4556c	9	11	-	-	PUNCT
d504rj4556c	9	12	resolved	resolve	VERB
d504rj4556c	9	13	absorption	absorption	NOUN
d504rj4556c	9	14	studies	study	NOUN
d504rj4556c	9	15	,	,	PUNCT
d504rj4556c	9	16	the	the	DET
d504rj4556c	9	17	important	important	ADJ
d504rj4556c	9	18	link	link	NOUN
d504rj4556c	9	19	between	between	ADP
d504rj4556c	9	20	the	the	DET
d504rj4556c	9	21	excited	excited	ADJ
d504rj4556c	9	22	state	state	NOUN
d504rj4556c	9	23	properties	property	NOUN
d504rj4556c	9	24	of	of	ADP
d504rj4556c	9	25	perovskite	perovskite	ADJ
d504rj4556c	9	26	precursor	precursor	NOUN
d504rj4556c	9	27	components	component	NOUN
d504rj4556c	9	28	,	,	PUNCT
d504rj4556c	9	29	composed	compose	VERB
d504rj4556c	9	30	of	of	ADP
d504rj4556c	9	31	solvated	solvated	ADJ
d504rj4556c	9	32	and	and	CCONJ
d504rj4556c	9	33	solid	solid	ADJ
d504rj4556c	9	34	-	-	PUNCT
d504rj4556c	9	35	state	state	NOUN
d504rj4556c	9	36	halometallate	halometallate	NOUN
d504rj4556c	9	37	complexes	complex	NOUN
d504rj4556c	9	38	,	,	PUNCT
d504rj4556c	9	39	and	and	CCONJ
d504rj4556c	9	40	ch3nh3pbi3	ch3nh3pbi3	PROPN
d504rj4556c	9	41	is	be	AUX
d504rj4556c	9	42	evinced	evince	VERB
d504rj4556c	9	43	.	.	PUNCT
d504rj4556c	10	1	this	this	DET
d504rj4556c	10	2	connection	connection	NOUN
d504rj4556c	10	3	provides	provide	VERB
d504rj4556c	10	4	insight	insight	NOUN
d504rj4556c	10	5	into	into	ADP
d504rj4556c	10	6	optical	optical	ADJ
d504rj4556c	10	7	nonlinearities	nonlinearitie	NOUN
d504rj4556c	10	8	and	and	CCONJ
d504rj4556c	10	9	electronic	electronic	ADJ
d504rj4556c	10	10	properties	property	NOUN
d504rj4556c	10	11	of	of	ADP
d504rj4556c	10	12	the	the	DET
d504rj4556c	10	13	perovskite	perovskite	ADJ
d504rj4556c	10	14	phase	phase	NOUN
d504rj4556c	10	15	.	.	PUNCT
d504rj4556c	11	1	in	in	ADP
d504rj4556c	11	2	the	the	DET
d504rj4556c	11	3	final	final	ADJ
d504rj4556c	11	4	chapter	chapter	NOUN
d504rj4556c	11	5	,	,	PUNCT
d504rj4556c	11	6	the	the	DET
d504rj4556c	11	7	operation	operation	NOUN
d504rj4556c	11	8	of	of	ADP
d504rj4556c	11	9	ch3nh3pbi3	ch3nh3pbi3	ADJ
d504rj4556c	11	10	solar	solar	ADJ
d504rj4556c	11	11	cells	cell	NOUN
d504rj4556c	11	12	in	in	ADP
d504rj4556c	11	13	a	a	DET
d504rj4556c	11	14	tandem	tandem	NOUN
d504rj4556c	11	15	architecture	architecture	NOUN
d504rj4556c	11	16	is	be	AUX
d504rj4556c	11	17	presented	present	VERB
d504rj4556c	11	18	.	.	PUNCT
d504rj4556c	12	1	utilizing	utilize	VERB
d504rj4556c	12	2	an	an	DET
d504rj4556c	12	3	all	all	DET
d504rj4556c	12	4	solution	solution	NOUN
d504rj4556c	12	5	-	-	PUNCT
d504rj4556c	12	6	processed	process	VERB
d504rj4556c	12	7	tandem	tandem	NOUN
d504rj4556c	12	8	water	water	NOUN
d504rj4556c	12	9	splitting	splitting	NOUN
d504rj4556c	12	10	assembly	assembly	NOUN
d504rj4556c	12	11	composed	compose	VERB
d504rj4556c	12	12	of	of	ADP
d504rj4556c	12	13	a	a	DET
d504rj4556c	12	14	bivo4	bivo4	ADJ
d504rj4556c	12	15	photoanode	photoanode	NOUN
d504rj4556c	12	16	and	and	CCONJ
d504rj4556c	12	17	a	a	DET
d504rj4556c	12	18	single	single	ADJ
d504rj4556c	12	19	-	-	PUNCT
d504rj4556c	12	20	junction	junction	NOUN
d504rj4556c	12	21	ch3nh3pbi3	ch3nh3pbi3	PROPN
d504rj4556c	12	22	hybrid	hybrid	ADJ
d504rj4556c	12	23	perovskite	perovskite	NOUN
d504rj4556c	12	24	solar	solar	ADJ
d504rj4556c	12	25	cell	cell	NOUN
d504rj4556c	12	26	,	,	PUNCT
d504rj4556c	12	27	hydrogen	hydrogen	NOUN
d504rj4556c	12	28	is	be	AUX
d504rj4556c	12	29	generated	generate	VERB
d504rj4556c	12	30	from	from	ADP
d504rj4556c	12	31	pure	pure	ADJ
d504rj4556c	12	32	water	water	NOUN
d504rj4556c	12	33	at	at	ADP
d504rj4556c	12	34	neutral	neutral	ADJ
d504rj4556c	12	35	ph	ph	NOUN
d504rj4556c	12	36	at	at	ADP
d504rj4556c	12	37	an	an	DET
d504rj4556c	12	38	efficiency	efficiency	NOUN
d504rj4556c	12	39	of	of	ADP
d504rj4556c	12	40	2.5	2.5	NUM
d504rj4556c	12	41	%	%	NOUN
d504rj4556c	12	42	without	without	ADP
d504rj4556c	12	43	external	external	ADJ
d504rj4556c	12	44	bias	bias	NOUN
d504rj4556c	12	45	.	.	PUNCT
d504rj4556c	13	1	the	the	DET
d504rj4556c	13	2	design	design	NOUN
d504rj4556c	13	3	of	of	ADP
d504rj4556c	13	4	low	low	ADJ
d504rj4556c	13	5	-	-	PUNCT
d504rj4556c	13	6	cost	cost	NOUN
d504rj4556c	13	7	tandem	tandem	NOUN
d504rj4556c	13	8	water	water	NOUN
d504rj4556c	13	9	splitting	splitting	NOUN
d504rj4556c	13	10	assemblies	assembly	NOUN
d504rj4556c	13	11	employing	employ	VERB
d504rj4556c	13	12	single	single	ADJ
d504rj4556c	13	13	-	-	PUNCT
d504rj4556c	13	14	junction	junction	NOUN
d504rj4556c	13	15	hybrid	hybrid	NOUN
d504rj4556c	13	16	perovskite	perovskite	NOUN
d504rj4556c	13	17	materials	material	NOUN
d504rj4556c	13	18	establishes	establish	VERB
d504rj4556c	13	19	a	a	DET
d504rj4556c	13	20	potentially	potentially	ADV
d504rj4556c	13	21	promising	promising	ADJ
d504rj4556c	13	22	new	new	ADJ
d504rj4556c	13	23	frontier	frontier	NOUN
d504rj4556c	13	24	for	for	ADP
d504rj4556c	13	25	solar	solar	ADJ
d504rj4556c	13	26	water	water	NOUN
d504rj4556c	13	27	splitting	splitting	NOUN
d504rj4556c	13	28	research	research	NOUN
d504rj4556c	13	29	.	.	PUNCT