id	sid	tid	token	lemma	pos
c821gh95n7n	1	1	the	the	DET
c821gh95n7n	1	2	properties	property	NOUN
c821gh95n7n	1	3	of	of	ADP
c821gh95n7n	1	4	a	a	DET
c821gh95n7n	1	5	material	material	NOUN
c821gh95n7n	1	6	are	be	AUX
c821gh95n7n	1	7	governed	govern	VERB
c821gh95n7n	1	8	by	by	ADP
c821gh95n7n	1	9	its	its	PRON
c821gh95n7n	1	10	microscopic	microscopic	ADJ
c821gh95n7n	1	11	structure	structure	NOUN
c821gh95n7n	1	12	,	,	PUNCT
c821gh95n7n	1	13	and	and	CCONJ
c821gh95n7n	1	14	the	the	DET
c821gh95n7n	1	15	investigation	investigation	NOUN
c821gh95n7n	1	16	of	of	ADP
c821gh95n7n	1	17	structure	structure	NOUN
c821gh95n7n	1	18	-	-	PUNCT
c821gh95n7n	1	19	property	property	NOUN
c821gh95n7n	1	20	relationships	relationship	NOUN
c821gh95n7n	1	21	has	have	AUX
c821gh95n7n	1	22	been	be	AUX
c821gh95n7n	1	23	the	the	DET
c821gh95n7n	1	24	focus	focus	NOUN
c821gh95n7n	1	25	of	of	ADP
c821gh95n7n	1	26	material	material	ADJ
c821gh95n7n	1	27	science	science	NOUN
c821gh95n7n	1	28	.	.	PUNCT
c821gh95n7n	2	1	group	group	PROPN
c821gh95n7n	2	2	iii	iii	PROPN
c821gh95n7n	2	3	-	-	PUNCT
c821gh95n7n	2	4	v	v	NOUN
c821gh95n7n	2	5	compound	compound	NOUN
c821gh95n7n	2	6	semiconductors	semiconductor	NOUN
c821gh95n7n	2	7	have	have	AUX
c821gh95n7n	2	8	been	be	AUX
c821gh95n7n	2	9	demonstrated	demonstrate	VERB
c821gh95n7n	2	10	to	to	PART
c821gh95n7n	2	11	be	be	AUX
c821gh95n7n	2	12	promising	promise	VERB
c821gh95n7n	2	13	candidates	candidate	NOUN
c821gh95n7n	2	14	for	for	ADP
c821gh95n7n	2	15	incorporating	incorporate	VERB
c821gh95n7n	2	16	into	into	ADP
c821gh95n7n	2	17	devices	device	NOUN
c821gh95n7n	2	18	for	for	ADP
c821gh95n7n	2	19	solar	solar	ADJ
c821gh95n7n	2	20	cell	cell	NOUN
c821gh95n7n	2	21	,	,	PUNCT
c821gh95n7n	2	22	photoelectrochemical	photoelectrochemical	ADJ
c821gh95n7n	2	23	water	water	NOUN
c821gh95n7n	2	24	splitting	splitting	NOUN
c821gh95n7n	2	25	and	and	CCONJ
c821gh95n7n	2	26	co2	co2	NOUN
c821gh95n7n	2	27	reduction	reduction	NOUN
c821gh95n7n	2	28	applications	application	NOUN
c821gh95n7n	2	29	.	.	PUNCT
c821gh95n7n	3	1	the	the	DET
c821gh95n7n	3	2	surface	surface	NOUN
c821gh95n7n	3	3	structural	structural	ADJ
c821gh95n7n	3	4	properties	property	NOUN
c821gh95n7n	3	5	of	of	ADP
c821gh95n7n	3	6	iii	iii	NUM
c821gh95n7n	3	7	-	-	PUNCT
c821gh95n7n	3	8	v	v	NOUN
c821gh95n7n	3	9	semiconductors	semiconductor	NOUN
c821gh95n7n	3	10	are	be	AUX
c821gh95n7n	3	11	often	often	ADV
c821gh95n7n	3	12	affected	affect	VERB
c821gh95n7n	3	13	by	by	ADP
c821gh95n7n	3	14	their	their	PRON
c821gh95n7n	3	15	interactions	interaction	NOUN
c821gh95n7n	3	16	with	with	ADP
c821gh95n7n	3	17	their	their	PRON
c821gh95n7n	3	18	environment	environment	NOUN
c821gh95n7n	3	19	,	,	PUNCT
c821gh95n7n	3	20	such	such	ADJ
c821gh95n7n	3	21	as	as	ADP
c821gh95n7n	3	22	the	the	DET
c821gh95n7n	3	23	surrounding	surround	VERB
c821gh95n7n	3	24	electrolyte	electrolyte	NOUN
c821gh95n7n	3	25	,	,	PUNCT
c821gh95n7n	3	26	which	which	PRON
c821gh95n7n	3	27	is	be	AUX
c821gh95n7n	3	28	usually	usually	ADV
c821gh95n7n	3	29	an	an	DET
c821gh95n7n	3	30	aqueous	aqueous	ADJ
c821gh95n7n	3	31	solution	solution	NOUN
c821gh95n7n	3	32	exposed	expose	VERB
c821gh95n7n	3	33	to	to	ADP
c821gh95n7n	3	34	an	an	DET
c821gh95n7n	3	35	ambient	ambient	ADJ
c821gh95n7n	3	36	environment	environment	NOUN
c821gh95n7n	3	37	.	.	PUNCT
c821gh95n7n	4	1	for	for	ADP
c821gh95n7n	4	2	controllable	controllable	ADJ
c821gh95n7n	4	3	design	design	NOUN
c821gh95n7n	4	4	and	and	CCONJ
c821gh95n7n	4	5	fabrication	fabrication	NOUN
c821gh95n7n	4	6	of	of	ADP
c821gh95n7n	4	7	high	high	ADJ
c821gh95n7n	4	8	-	-	PUNCT
c821gh95n7n	4	9	quality	quality	NOUN
c821gh95n7n	4	10	iii	iii	NUM
c821gh95n7n	4	11	-	-	PUNCT
c821gh95n7n	4	12	v	v	NOUN
c821gh95n7n	4	13	semiconductor	semiconductor	NOUN
c821gh95n7n	4	14	-	-	PUNCT
c821gh95n7n	4	15	based	base	VERB
c821gh95n7n	4	16	devices	device	NOUN
c821gh95n7n	4	17	,	,	PUNCT
c821gh95n7n	4	18	knowledge	knowledge	NOUN
c821gh95n7n	4	19	of	of	ADP
c821gh95n7n	4	20	environmental	environmental	ADJ
c821gh95n7n	4	21	molecule	molecule	NOUN
c821gh95n7n	4	22	/	/	SYM
c821gh95n7n	4	23	iii	iii	NUM
c821gh95n7n	4	24	-	-	PUNCT
c821gh95n7n	4	25	v	v	NOUN
c821gh95n7n	4	26	semiconductor	semiconductor	NOUN
c821gh95n7n	4	27	interfacial	interfacial	PROPN
c821gh95n7n	4	28	chemical	chemical	NOUN
c821gh95n7n	4	29	and	and	CCONJ
c821gh95n7n	4	30	electronic	electronic	ADJ
c821gh95n7n	4	31	properties	property	NOUN
c821gh95n7n	4	32	is	be	AUX
c821gh95n7n	4	33	highly	highly	ADV
c821gh95n7n	4	34	desirable	desirable	ADJ
c821gh95n7n	4	35	,	,	PUNCT
c821gh95n7n	4	36	especially	especially	ADV
c821gh95n7n	4	37	that	that	PRON
c821gh95n7n	4	38	gained	gain	VERB
c821gh95n7n	4	39	from	from	ADP
c821gh95n7n	4	40	studies	study	NOUN
c821gh95n7n	4	41	performed	perform	VERB
c821gh95n7n	4	42	under	under	ADP
c821gh95n7n	4	43	close	close	ADV
c821gh95n7n	4	44	to	to	ADP
c821gh95n7n	4	45	practical	practical	ADJ
c821gh95n7n	4	46	operational	operational	ADJ
c821gh95n7n	4	47	conditions	condition	NOUN
c821gh95n7n	4	48	.	.	PUNCT
c821gh95n7n	5	1	however	however	ADV
c821gh95n7n	5	2	,	,	PUNCT
c821gh95n7n	5	3	previous	previous	ADJ
c821gh95n7n	5	4	studies	study	NOUN
c821gh95n7n	5	5	have	have	AUX
c821gh95n7n	5	6	been	be	AUX
c821gh95n7n	5	7	limited	limit	VERB
c821gh95n7n	5	8	by	by	ADP
c821gh95n7n	5	9	the	the	DET
c821gh95n7n	5	10	complexity	complexity	NOUN
c821gh95n7n	5	11	of	of	ADP
c821gh95n7n	5	12	the	the	DET
c821gh95n7n	5	13	system	system	NOUN
c821gh95n7n	5	14	or	or	CCONJ
c821gh95n7n	5	15	the	the	DET
c821gh95n7n	5	16	availability	availability	NOUN
c821gh95n7n	5	17	of	of	ADP
c821gh95n7n	5	18	suitable	suitable	ADJ
c821gh95n7n	5	19	instrumentation	instrumentation	NOUN
c821gh95n7n	5	20	,	,	PUNCT
c821gh95n7n	5	21	and	and	CCONJ
c821gh95n7n	5	22	all	all	DET
c821gh95n7n	5	23	the	the	DET
c821gh95n7n	5	24	experimental	experimental	ADJ
c821gh95n7n	5	25	data	datum	NOUN
c821gh95n7n	5	26	in	in	ADP
c821gh95n7n	5	27	literature	literature	NOUN
c821gh95n7n	5	28	are	be	AUX
c821gh95n7n	5	29	performed	perform	VERB
c821gh95n7n	5	30	under	under	ADP
c821gh95n7n	5	31	ex	ex	NOUN
c821gh95n7n	5	32	-	-	ADJ
c821gh95n7n	5	33	situ	situ	ADJ
c821gh95n7n	5	34	and	and	CCONJ
c821gh95n7n	5	35	ultra	ultra	ADJ
c821gh95n7n	5	36	-	-	ADJ
c821gh95n7n	5	37	high	high	ADJ
c821gh95n7n	5	38	vacuum	vacuum	NOUN
c821gh95n7n	5	39	conditions.in	conditions.in	NUM
c821gh95n7n	5	40	the	the	DET
c821gh95n7n	5	41	frame	frame	NOUN
c821gh95n7n	5	42	of	of	ADP
c821gh95n7n	5	43	my	my	PRON
c821gh95n7n	5	44	phd	phd	NOUN
c821gh95n7n	5	45	thesis	thesis	NOUN
c821gh95n7n	5	46	,	,	PUNCT
c821gh95n7n	5	47	i	i	PRON
c821gh95n7n	5	48	aim	aim	VERB
c821gh95n7n	5	49	to	to	PART
c821gh95n7n	5	50	investigate	investigate	VERB
c821gh95n7n	5	51	the	the	DET
c821gh95n7n	5	52	chemical	chemical	ADJ
c821gh95n7n	5	53	and	and	CCONJ
c821gh95n7n	5	54	electronic	electronic	ADJ
c821gh95n7n	5	55	properties	property	NOUN
c821gh95n7n	5	56	at	at	ADP
c821gh95n7n	5	57	the	the	DET
c821gh95n7n	5	58	environmental	environmental	ADJ
c821gh95n7n	5	59	molecule	molecule	NOUN
c821gh95n7n	5	60	(	(	PUNCT
c821gh95n7n	5	61	h2o	h2o	PROPN
c821gh95n7n	5	62	and	and	CCONJ
c821gh95n7n	5	63	o2)/iii	o2)/iii	ADJ
c821gh95n7n	5	64	-	-	PUNCT
c821gh95n7n	5	65	v	v	NOUN
c821gh95n7n	5	66	semiconductor	semiconductor	NOUN
c821gh95n7n	5	67	interface	interface	NOUN
c821gh95n7n	5	68	under	under	ADP
c821gh95n7n	5	69	in	in	ADP
c821gh95n7n	5	70	-	-	PUNCT
c821gh95n7n	5	71	situ	situ	NOUN
c821gh95n7n	5	72	or	or	CCONJ
c821gh95n7n	5	73	operando	operando	NOUN
c821gh95n7n	5	74	conditions	condition	NOUN
c821gh95n7n	5	75	using	use	VERB
c821gh95n7n	5	76	ambient	ambient	ADJ
c821gh95n7n	5	77	pressure	pressure	NOUN
c821gh95n7n	5	78	x	x	NOUN
c821gh95n7n	5	79	-	-	NOUN
c821gh95n7n	5	80	ray	ray	NOUN
c821gh95n7n	5	81	photoelectron	photoelectron	NOUN
c821gh95n7n	5	82	spectroscopy	spectroscopy	NOUN
c821gh95n7n	5	83	(	(	PUNCT
c821gh95n7n	5	84	ap	ap	PROPN
c821gh95n7n	5	85	-	-	PUNCT
c821gh95n7n	5	86	xps	xps	PROPN
c821gh95n7n	5	87	)	)	PUNCT
c821gh95n7n	5	88	.	.	PUNCT
c821gh95n7n	6	1	chapter	chapter	NOUN
c821gh95n7n	6	2	1	1	NUM
c821gh95n7n	6	3	introduces	introduce	VERB
c821gh95n7n	6	4	background	background	NOUN
c821gh95n7n	6	5	information	information	NOUN
c821gh95n7n	6	6	for	for	ADP
c821gh95n7n	6	7	solar	solar	ADJ
c821gh95n7n	6	8	water	water	NOUN
c821gh95n7n	6	9	splitting	splitting	NOUN
c821gh95n7n	6	10	,	,	PUNCT
c821gh95n7n	6	11	the	the	DET
c821gh95n7n	6	12	motivations	motivation	NOUN
c821gh95n7n	6	13	of	of	ADP
c821gh95n7n	6	14	the	the	DET
c821gh95n7n	6	15	thesis	thesis	NOUN
c821gh95n7n	6	16	,	,	PUNCT
c821gh95n7n	6	17	the	the	DET
c821gh95n7n	6	18	details	detail	NOUN
c821gh95n7n	6	19	of	of	ADP
c821gh95n7n	6	20	the	the	DET
c821gh95n7n	6	21	major	major	ADJ
c821gh95n7n	6	22	instrumentation	instrumentation	NOUN
c821gh95n7n	6	23	(	(	PUNCT
c821gh95n7n	6	24	ap	ap	PROPN
c821gh95n7n	6	25	-	-	PUNCT
c821gh95n7n	6	26	xps	xps	PROPN
c821gh95n7n	6	27	)	)	PUNCT
c821gh95n7n	6	28	and	and	CCONJ
c821gh95n7n	6	29	the	the	DET
c821gh95n7n	6	30	overall	overall	ADJ
c821gh95n7n	6	31	goal	goal	NOUN
c821gh95n7n	6	32	of	of	ADP
c821gh95n7n	6	33	the	the	DET
c821gh95n7n	6	34	thesis	thesis	NOUN
c821gh95n7n	6	35	;	;	PUNCT
c821gh95n7n	6	36	chapter	chapter	NOUN
c821gh95n7n	6	37	2	2	NUM
c821gh95n7n	6	38	and	and	CCONJ
c821gh95n7n	6	39	3	3	NUM
c821gh95n7n	6	40	present	present	VERB
c821gh95n7n	6	41	the	the	DET
c821gh95n7n	6	42	studies	study	NOUN
c821gh95n7n	6	43	of	of	ADP
c821gh95n7n	6	44	the	the	DET
c821gh95n7n	6	45	interfacial	interfacial	ADJ
c821gh95n7n	6	46	chemistry	chemistry	NOUN
c821gh95n7n	6	47	of	of	ADP
c821gh95n7n	6	48	o2	o2	PROPN
c821gh95n7n	6	49	and	and	CCONJ
c821gh95n7n	6	50	h2o	h2o	PROPN
c821gh95n7n	6	51	/	/	SYM
c821gh95n7n	6	52	iii	iii	NUM
c821gh95n7n	6	53	-	-	PUNCT
c821gh95n7n	6	54	v	v	NOUN
c821gh95n7n	6	55	semiconductors	semiconductor	NOUN
c821gh95n7n	6	56	,	,	PUNCT
c821gh95n7n	6	57	respectively	respectively	ADV
c821gh95n7n	6	58	;	;	PUNCT
c821gh95n7n	6	59	chapter	chapter	NOUN
c821gh95n7n	6	60	4	4	NUM
c821gh95n7n	6	61	focuses	focus	VERB
c821gh95n7n	6	62	on	on	ADP
c821gh95n7n	6	63	the	the	DET
c821gh95n7n	6	64	investigation	investigation	NOUN
c821gh95n7n	6	65	of	of	ADP
c821gh95n7n	6	66	the	the	DET
c821gh95n7n	6	67	interfacial	interfacial	ADJ
c821gh95n7n	6	68	chemical	chemical	NOUN
c821gh95n7n	6	69	and	and	CCONJ
c821gh95n7n	6	70	electronic	electronic	ADJ
c821gh95n7n	6	71	property	property	NOUN
c821gh95n7n	6	72	relationship	relationship	NOUN
c821gh95n7n	6	73	in	in	ADP
c821gh95n7n	6	74	a	a	DET
c821gh95n7n	6	75	iii	iii	NUM
c821gh95n7n	6	76	-	-	PUNCT
c821gh95n7n	6	77	v	v	NOUN
c821gh95n7n	6	78	based	base	VERB
c821gh95n7n	6	79	photoelectrode	photoelectrode	NOUN
c821gh95n7n	6	80	;	;	PUNCT
c821gh95n7n	6	81	chapter	chapter	NOUN
c821gh95n7n	6	82	5	5	NUM
c821gh95n7n	6	83	is	be	AUX
c821gh95n7n	6	84	an	an	DET
c821gh95n7n	6	85	extension	extension	NOUN
c821gh95n7n	6	86	of	of	ADP
c821gh95n7n	6	87	the	the	DET
c821gh95n7n	6	88	previous	previous	ADJ
c821gh95n7n	6	89	three	three	NUM
c821gh95n7n	6	90	chapters	chapter	NOUN
c821gh95n7n	6	91	,	,	PUNCT
c821gh95n7n	6	92	where	where	SCONJ
c821gh95n7n	6	93	a	a	DET
c821gh95n7n	6	94	real	real	ADJ
c821gh95n7n	6	95	electrochemical	electrochemical	ADJ
c821gh95n7n	6	96	device	device	NOUN
c821gh95n7n	6	97	for	for	ADP
c821gh95n7n	6	98	water	water	NOUN
c821gh95n7n	6	99	splitting	splitting	NOUN
c821gh95n7n	6	100	is	be	AUX
c821gh95n7n	6	101	designed	design	VERB
c821gh95n7n	6	102	,	,	PUNCT
c821gh95n7n	6	103	fabricated	fabricate	VERB
c821gh95n7n	6	104	and	and	CCONJ
c821gh95n7n	6	105	incorporated	incorporate	VERB
c821gh95n7n	6	106	into	into	ADP
c821gh95n7n	6	107	the	the	DET
c821gh95n7n	6	108	ap	ap	PROPN
c821gh95n7n	6	109	-	-	PUNCT
c821gh95n7n	6	110	xps	xps	PROPN
c821gh95n7n	6	111	system	system	NOUN
c821gh95n7n	6	112	,	,	PUNCT
c821gh95n7n	6	113	and	and	CCONJ
c821gh95n7n	6	114	properties	property	NOUN
c821gh95n7n	6	115	including	include	VERB
c821gh95n7n	6	116	the	the	DET
c821gh95n7n	6	117	h2o	h2o	NOUN
c821gh95n7n	6	118	/	/	SYM
c821gh95n7n	6	119	device	device	NOUN
c821gh95n7n	6	120	interfacial	interfacial	ADJ
c821gh95n7n	6	121	chemical	chemical	NOUN
c821gh95n7n	6	122	,	,	PUNCT
c821gh95n7n	6	123	electrical	electrical	ADJ
c821gh95n7n	6	124	and	and	CCONJ
c821gh95n7n	6	125	catalytic	catalytic	ADJ
c821gh95n7n	6	126	features	feature	NOUN
c821gh95n7n	6	127	are	be	AUX
c821gh95n7n	6	128	investigated	investigate	VERB
c821gh95n7n	6	129	under	under	ADP
c821gh95n7n	6	130	operational	operational	ADJ
c821gh95n7n	6	131	conditions	condition	NOUN
c821gh95n7n	6	132	.	.	PUNCT
c821gh95n7n	7	1	the	the	DET
c821gh95n7n	7	2	present	present	ADJ
c821gh95n7n	7	3	study	study	NOUN
c821gh95n7n	7	4	has	have	VERB
c821gh95n7n	7	5	important	important	ADJ
c821gh95n7n	7	6	implications	implication	NOUN
c821gh95n7n	7	7	for	for	ADP
c821gh95n7n	7	8	the	the	DET
c821gh95n7n	7	9	fundamental	fundamental	ADJ
c821gh95n7n	7	10	understanding	understanding	NOUN
c821gh95n7n	7	11	of	of	ADP
c821gh95n7n	7	12	environmental	environmental	ADJ
c821gh95n7n	7	13	molecule	molecule	NOUN
c821gh95n7n	7	14	(	(	PUNCT
c821gh95n7n	7	15	h2o	h2o	PROPN
c821gh95n7n	7	16	or	or	CCONJ
c821gh95n7n	7	17	o2)/iii	o2)/iii	ADJ
c821gh95n7n	7	18	-	-	PUNCT
c821gh95n7n	7	19	v	v	NOUN
c821gh95n7n	7	20	semiconductor	semiconductor	NOUN
c821gh95n7n	7	21	interactions	interaction	NOUN
c821gh95n7n	7	22	and	and	CCONJ
c821gh95n7n	7	23	for	for	ADP
c821gh95n7n	7	24	the	the	DET
c821gh95n7n	7	25	practical	practical	ADJ
c821gh95n7n	7	26	design	design	NOUN
c821gh95n7n	7	27	and	and	CCONJ
c821gh95n7n	7	28	fabrication	fabrication	NOUN
c821gh95n7n	7	29	of	of	ADP
c821gh95n7n	7	30	a	a	DET
c821gh95n7n	7	31	future	future	ADJ
c821gh95n7n	7	32	high	high	ADJ
c821gh95n7n	7	33	-	-	PUNCT
c821gh95n7n	7	34	quality	quality	NOUN
c821gh95n7n	7	35	solar	solar	ADJ
c821gh95n7n	7	36	water	water	NOUN
c821gh95n7n	7	37	splitting	splitting	NOUN
c821gh95n7n	7	38	device	device	NOUN
c821gh95n7n	7	39	.	.	PUNCT