id	sid	tid	token	lemma	pos
5712m616c6r	1	1	this	this	DET
5712m616c6r	1	2	dissertation	dissertation	NOUN
5712m616c6r	1	3	pioneers	pioneer	VERB
5712m616c6r	1	4	the	the	DET
5712m616c6r	1	5	macroscopic	macroscopic	ADJ
5712m616c6r	1	6	characterization	characterization	NOUN
5712m616c6r	1	7	of	of	ADP
5712m616c6r	1	8	uranyl	uranyl	ADJ
5712m616c6r	1	9	peroxide	peroxide	NOUN
5712m616c6r	1	10	nanocluster	nanocluster	NOUN
5712m616c6r	1	11	interactions	interaction	NOUN
5712m616c6r	1	12	with	with	ADP
5712m616c6r	1	13	different	different	ADJ
5712m616c6r	1	14	mineral	mineral	NOUN
5712m616c6r	1	15	surfaces	surface	NOUN
5712m616c6r	1	16	.	.	PUNCT
5712m616c6r	2	1	batch	batch	NOUN
5712m616c6r	2	2	sorption	sorption	NOUN
5712m616c6r	2	3	experiments	experiment	NOUN
5712m616c6r	2	4	were	be	AUX
5712m616c6r	2	5	conducted	conduct	VERB
5712m616c6r	2	6	in	in	ADP
5712m616c6r	2	7	order	order	NOUN
5712m616c6r	2	8	to	to	PART
5712m616c6r	2	9	determine	determine	VERB
5712m616c6r	2	10	the	the	DET
5712m616c6r	2	11	effects	effect	NOUN
5712m616c6r	2	12	of	of	ADP
5712m616c6r	2	13	time	time	NOUN
5712m616c6r	2	14	,	,	PUNCT
5712m616c6r	2	15	ph	ph	ADJ
5712m616c6r	2	16	,	,	PUNCT
5712m616c6r	2	17	ionic	ionic	ADJ
5712m616c6r	2	18	strength	strength	NOUN
5712m616c6r	2	19	,	,	PUNCT
5712m616c6r	2	20	sorbate	sorbate	ADJ
5712m616c6r	2	21	concentration	concentration	NOUN
5712m616c6r	2	22	,	,	PUNCT
5712m616c6r	2	23	and	and	CCONJ
5712m616c6r	2	24	sorbent	sorbent	NOUN
5712m616c6r	2	25	concentration	concentration	NOUN
5712m616c6r	2	26	on	on	ADP
5712m616c6r	2	27	the	the	DET
5712m616c6r	2	28	sorption	sorption	NOUN
5712m616c6r	2	29	of	of	ADP
5712m616c6r	2	30	[	[	X
5712m616c6r	2	31	(	(	PUNCT
5712m616c6r	2	32	uo2)(o2)(oh)]6060(u60	uo2)(o2)(oh)]6060(u60	PROPN
5712m616c6r	2	33	)	)	PUNCT
5712m616c6r	2	34	and	and	CCONJ
5712m616c6r	2	35	[	[	X
5712m616c6r	2	36	(	(	PUNCT
5712m616c6r	2	37	uo2)24(o2)24(p2o7)12]48(u24pp12	uo2)24(o2)24(p2o7)12]48(u24pp12	ADJ
5712m616c6r	2	38	)	)	PUNCT
5712m616c6r	2	39	to	to	ADP
5712m616c6r	2	40	hematite	hematite	PROPN
5712m616c6r	2	41	(	(	PUNCT
5712m616c6r	2	42	α	α	PROPN
5712m616c6r	2	43	-	-	PUNCT
5712m616c6r	2	44	fe2o3	fe2o3	NOUN
5712m616c6r	2	45	)	)	PUNCT
5712m616c6r	2	46	,	,	PUNCT
5712m616c6r	2	47	goethite	goethite	NOUN
5712m616c6r	2	48	(	(	PUNCT
5712m616c6r	2	49	α	α	NOUN
5712m616c6r	2	50	-	-	PUNCT
5712m616c6r	2	51	feooh	feooh	NOUN
5712m616c6r	2	52	)	)	PUNCT
5712m616c6r	2	53	,	,	PUNCT
5712m616c6r	2	54	montmorillonite	montmorillonite	NOUN
5712m616c6r	2	55	,	,	PUNCT
5712m616c6r	2	56	quartz	quartz	NOUN
5712m616c6r	2	57	(	(	PUNCT
5712m616c6r	2	58	sio2	sio2	PROPN
5712m616c6r	2	59	)	)	PUNCT
5712m616c6r	2	60	,	,	PUNCT
5712m616c6r	2	61	and	and	CCONJ
5712m616c6r	2	62	anorthite.this	anorthite.this	PROPN
5712m616c6r	2	63	work	work	NOUN
5712m616c6r	2	64	reveals	reveal	VERB
5712m616c6r	2	65	that	that	SCONJ
5712m616c6r	2	66	u60	u60	ADV
5712m616c6r	2	67	persists	persist	VERB
5712m616c6r	2	68	in	in	ADP
5712m616c6r	2	69	the	the	DET
5712m616c6r	2	70	presence	presence	NOUN
5712m616c6r	2	71	of	of	ADP
5712m616c6r	2	72	fe(iii	fe(iii	NOUN
5712m616c6r	2	73	)	)	PUNCT
5712m616c6r	2	74	minerals	mineral	NOUN
5712m616c6r	2	75	,	,	PUNCT
5712m616c6r	2	76	montmorillonite	montmorillonite	NOUN
5712m616c6r	2	77	,	,	PUNCT
5712m616c6r	2	78	and	and	CCONJ
5712m616c6r	2	79	common	common	ADJ
5712m616c6r	2	80	alkali	alkali	ADJ
5712m616c6r	2	81	ions	ion	NOUN
5712m616c6r	2	82	for	for	ADP
5712m616c6r	2	83	months	month	NOUN
5712m616c6r	2	84	.	.	PUNCT
5712m616c6r	3	1	the	the	DET
5712m616c6r	3	2	sorption	sorption	NOUN
5712m616c6r	3	3	behavior	behavior	NOUN
5712m616c6r	3	4	of	of	ADP
5712m616c6r	3	5	u60	u60	ADV
5712m616c6r	3	6	in	in	ADP
5712m616c6r	3	7	the	the	DET
5712m616c6r	3	8	presence	presence	NOUN
5712m616c6r	3	9	of	of	ADP
5712m616c6r	3	10	fe(iii	fe(iii	NOUN
5712m616c6r	3	11	)	)	PUNCT
5712m616c6r	3	12	minerals	mineral	NOUN
5712m616c6r	3	13	mimics	mimic	VERB
5712m616c6r	3	14	that	that	PRON
5712m616c6r	3	15	of	of	ADP
5712m616c6r	3	16	a	a	DET
5712m616c6r	3	17	discrete	discrete	ADJ
5712m616c6r	3	18	anionic	anionic	ADJ
5712m616c6r	3	19	species	specie	NOUN
5712m616c6r	3	20	whose	whose	DET
5712m616c6r	3	21	contacts	contact	NOUN
5712m616c6r	3	22	at	at	ADP
5712m616c6r	3	23	the	the	DET
5712m616c6r	3	24	mineral	mineral	NOUN
5712m616c6r	3	25	-	-	PUNCT
5712m616c6r	3	26	water	water	NOUN
5712m616c6r	3	27	interface	interface	NOUN
5712m616c6r	3	28	are	be	AUX
5712m616c6r	3	29	driven	drive	VERB
5712m616c6r	3	30	by	by	ADP
5712m616c6r	3	31	the	the	DET
5712m616c6r	3	32	formation	formation	NOUN
5712m616c6r	3	33	of	of	ADP
5712m616c6r	3	34	electrostatic	electrostatic	ADJ
5712m616c6r	3	35	,	,	PUNCT
5712m616c6r	3	36	outer	outer	ADJ
5712m616c6r	3	37	-	-	PUNCT
5712m616c6r	3	38	sphere	sphere	NOUN
5712m616c6r	3	39	surface	surface	NOUN
5712m616c6r	3	40	complexes	complex	NOUN
5712m616c6r	3	41	.	.	PUNCT
5712m616c6r	4	1	u60	u60	ADV
5712m616c6r	4	2	also	also	ADV
5712m616c6r	4	3	survives	survive	VERB
5712m616c6r	4	4	the	the	DET
5712m616c6r	4	5	sorption	sorption	NOUN
5712m616c6r	4	6	-	-	PUNCT
5712m616c6r	4	7	desorption	desorption	NOUN
5712m616c6r	4	8	process	process	NOUN
5712m616c6r	4	9	.	.	PUNCT
5712m616c6r	5	1	in	in	ADP
5712m616c6r	5	2	clay	clay	NOUN
5712m616c6r	5	3	mineral	mineral	NOUN
5712m616c6r	5	4	suspensions	suspension	NOUN
5712m616c6r	5	5	,	,	PUNCT
5712m616c6r	5	6	the	the	DET
5712m616c6r	5	7	counter	counter	NOUN
5712m616c6r	5	8	-	-	NOUN
5712m616c6r	5	9	cations	cation	NOUN
5712m616c6r	5	10	associated	associate	VERB
5712m616c6r	5	11	with	with	ADP
5712m616c6r	5	12	the	the	DET
5712m616c6r	5	13	cluster	cluster	NOUN
5712m616c6r	5	14	undergo	undergo	VERB
5712m616c6r	5	15	cation	cation	NOUN
5712m616c6r	5	16	exchange	exchange	NOUN
5712m616c6r	5	17	reactions	reaction	NOUN
5712m616c6r	5	18	with	with	ADP
5712m616c6r	5	19	exchangeable	exchangeable	ADJ
5712m616c6r	5	20	cations	cation	NOUN
5712m616c6r	5	21	associated	associate	VERB
5712m616c6r	5	22	with	with	ADP
5712m616c6r	5	23	the	the	DET
5712m616c6r	5	24	clay	clay	NOUN
5712m616c6r	5	25	.	.	PUNCT
5712m616c6r	6	1	the	the	DET
5712m616c6r	6	2	type	type	NOUN
5712m616c6r	6	3	of	of	ADP
5712m616c6r	6	4	cation	cation	NOUN
5712m616c6r	6	5	(	(	PUNCT
5712m616c6r	6	6	i.e.	i.e.	X
5712m616c6r	6	7	,	,	PUNCT
5712m616c6r	6	8	monovalent	monovalent	NOUN
5712m616c6r	6	9	or	or	CCONJ
5712m616c6r	6	10	divalent	divalent	NOUN
5712m616c6r	6	11	)	)	PUNCT
5712m616c6r	6	12	that	that	PRON
5712m616c6r	6	13	is	be	AUX
5712m616c6r	6	14	exchanged	exchange	VERB
5712m616c6r	6	15	and	and	CCONJ
5712m616c6r	6	16	the	the	DET
5712m616c6r	6	17	amount	amount	NOUN
5712m616c6r	6	18	present	present	ADJ
5712m616c6r	6	19	in	in	ADP
5712m616c6r	6	20	the	the	DET
5712m616c6r	6	21	system	system	NOUN
5712m616c6r	6	22	largely	largely	ADV
5712m616c6r	6	23	dictates	dictate	VERB
5712m616c6r	6	24	the	the	DET
5712m616c6r	6	25	removal	removal	NOUN
5712m616c6r	6	26	of	of	ADP
5712m616c6r	6	27	u60	u60	ADV
5712m616c6r	6	28	from	from	ADP
5712m616c6r	6	29	solution	solution	NOUN
5712m616c6r	6	30	via	via	ADP
5712m616c6r	6	31	surface	surface	NOUN
5712m616c6r	6	32	precipitation	precipitation	NOUN
5712m616c6r	6	33	to	to	PART
5712m616c6r	6	34	form	form	VERB
5712m616c6r	6	35	large	large	ADJ
5712m616c6r	6	36	agglomerates	agglomerate	NOUN
5712m616c6r	6	37	of	of	ADP
5712m616c6r	6	38	clusters	cluster	NOUN
5712m616c6r	6	39	.	.	PUNCT
5712m616c6r	7	1	the	the	DET
5712m616c6r	7	2	sorption	sorption	NOUN
5712m616c6r	7	3	of	of	ADP
5712m616c6r	7	4	u60	u60	ADV
5712m616c6r	7	5	to	to	ADP
5712m616c6r	7	6	minerals	mineral	NOUN
5712m616c6r	7	7	that	that	PRON
5712m616c6r	7	8	have	have	VERB
5712m616c6r	7	9	a	a	DET
5712m616c6r	7	10	low	low	ADJ
5712m616c6r	7	11	point	point	NOUN
5712m616c6r	7	12	of	of	ADP
5712m616c6r	7	13	zero	zero	NUM
5712m616c6r	7	14	charge	charge	NOUN
5712m616c6r	7	15	,	,	PUNCT
5712m616c6r	7	16	(	(	PUNCT
5712m616c6r	7	17	i.e.	i.e.	X
5712m616c6r	7	18	,	,	PUNCT
5712m616c6r	7	19	quartz	quartz	PROPN
5712m616c6r	7	20	and	and	CCONJ
5712m616c6r	7	21	anorthite	anorthite	PROPN
5712m616c6r	7	22	)	)	PUNCT
5712m616c6r	7	23	is	be	AUX
5712m616c6r	7	24	not	not	PART
5712m616c6r	7	25	favorable	favorable	ADJ
5712m616c6r	7	26	under	under	ADP
5712m616c6r	7	27	alkaline	alkaline	NOUN
5712m616c6r	7	28	conditions	condition	NOUN
5712m616c6r	7	29	due	due	ADJ
5712m616c6r	7	30	to	to	ADP
5712m616c6r	7	31	repulsion	repulsion	NOUN
5712m616c6r	7	32	of	of	ADP
5712m616c6r	7	33	the	the	DET
5712m616c6r	7	34	negatively	negatively	ADV
5712m616c6r	7	35	-	-	PUNCT
5712m616c6r	7	36	charged	charge	VERB
5712m616c6r	7	37	mineral	mineral	NOUN
5712m616c6r	7	38	surface	surface	NOUN
5712m616c6r	7	39	and	and	CCONJ
5712m616c6r	7	40	the	the	DET
5712m616c6r	7	41	negatively	negatively	ADV
5712m616c6r	7	42	-	-	PUNCT
5712m616c6r	7	43	charged	charge	VERB
5712m616c6r	7	44	uranyl	uranyl	ADJ
5712m616c6r	7	45	peroxide	peroxide	NOUN
5712m616c6r	7	46	cage	cage	NOUN
5712m616c6r	7	47	.	.	PUNCT
5712m616c6r	8	1	the	the	DET
5712m616c6r	8	2	incorporation	incorporation	NOUN
5712m616c6r	8	3	of	of	ADP
5712m616c6r	8	4	the	the	DET
5712m616c6r	8	5	pyrophosphate	pyrophosphate	NOUN
5712m616c6r	8	6	ligand	ligand	NOUN
5712m616c6r	8	7	(	(	PUNCT
5712m616c6r	8	8	p2o74-	p2o74-	SPACE
5712m616c6r	8	9	)	)	PUNCT
5712m616c6r	8	10	into	into	ADP
5712m616c6r	8	11	the	the	DET
5712m616c6r	8	12	framework	framework	NOUN
5712m616c6r	8	13	of	of	ADP
5712m616c6r	8	14	uranyl	uranyl	ADJ
5712m616c6r	8	15	peroxide	peroxide	NOUN
5712m616c6r	8	16	nanoclusters	nanocluster	NOUN
5712m616c6r	8	17	leads	lead	VERB
5712m616c6r	8	18	to	to	ADP
5712m616c6r	8	19	the	the	DET
5712m616c6r	8	20	formation	formation	NOUN
5712m616c6r	8	21	of	of	ADP
5712m616c6r	8	22	functionalized	functionalize	VERB
5712m616c6r	8	23	uranyl	uranyl	ADJ
5712m616c6r	8	24	peroxide	peroxide	NOUN
5712m616c6r	8	25	nanoclusters	nanocluster	NOUN
5712m616c6r	8	26	.	.	PUNCT
5712m616c6r	9	1	the	the	DET
5712m616c6r	9	2	pyrophosphate	pyrophosphate	NOUN
5712m616c6r	9	3	-	-	PUNCT
5712m616c6r	9	4	functionalized	functionalize	VERB
5712m616c6r	9	5	nanocluster	nanocluster	NOUN
5712m616c6r	9	6	u24pp12	u24pp12	NOUN
5712m616c6r	9	7	may	may	AUX
5712m616c6r	9	8	form	form	VERB
5712m616c6r	9	9	specific	specific	ADJ
5712m616c6r	9	10	interactions	interaction	NOUN
5712m616c6r	9	11	with	with	ADP
5712m616c6r	9	12	hematite	hematite	NOUN
5712m616c6r	9	13	and	and	CCONJ
5712m616c6r	9	14	goethite	goethite	ADJ
5712m616c6r	9	15	surfaces	surface	NOUN
5712m616c6r	9	16	through	through	ADP
5712m616c6r	9	17	the	the	DET
5712m616c6r	9	18	terminal	terminal	ADJ
5712m616c6r	9	19	oxygen	oxygen	NOUN
5712m616c6r	9	20	atoms	atom	NOUN
5712m616c6r	9	21	of	of	ADP
5712m616c6r	9	22	the	the	DET
5712m616c6r	9	23	pyrophosphate	pyrophosphate	NOUN
5712m616c6r	9	24	unit	unit	NOUN
5712m616c6r	9	25	.	.	PUNCT
5712m616c6r	10	1	the	the	DET
5712m616c6r	10	2	removal	removal	NOUN
5712m616c6r	10	3	of	of	ADP
5712m616c6r	10	4	u60	u60	ADJ
5712m616c6r	10	5	and	and	CCONJ
5712m616c6r	10	6	u24pp12	u24pp12	ADJ
5712m616c6r	10	7	are	be	AUX
5712m616c6r	10	8	not	not	PART
5712m616c6r	10	9	due	due	ADJ
5712m616c6r	10	10	to	to	ADP
5712m616c6r	10	11	surface	surface	NOUN
5712m616c6r	10	12	-	-	PUNCT
5712m616c6r	10	13	mediated	mediate	VERB
5712m616c6r	10	14	reduction	reduction	NOUN
5712m616c6r	10	15	of	of	ADP
5712m616c6r	10	16	u(vi	u(vi	NOUN
5712m616c6r	10	17	)	)	PUNCT
5712m616c6r	10	18	to	to	ADP
5712m616c6r	10	19	u(iv	u(iv	PROPN
5712m616c6r	10	20	)	)	PUNCT
5712m616c6r	10	21	by	by	ADP
5712m616c6r	10	22	interactions	interaction	NOUN
5712m616c6r	10	23	with	with	ADP
5712m616c6r	10	24	minor	minor	ADJ
5712m616c6r	10	25	reducing	reduce	VERB
5712m616c6r	10	26	components	component	NOUN
5712m616c6r	10	27	in	in	ADP
5712m616c6r	10	28	goethite	goethite	ADJ
5712m616c6r	10	29	,	,	PUNCT
5712m616c6r	10	30	hematite	hematite	NOUN
5712m616c6r	10	31	and	and	CCONJ
5712m616c6r	10	32	montmorillonite	montmorillonite	NOUN
5712m616c6r	10	33	.	.	PUNCT
5712m616c6r	11	1	the	the	DET
5712m616c6r	11	2	governing	governing	NOUN
5712m616c6r	11	3	rate	rate	NOUN
5712m616c6r	11	4	laws	law	NOUN
5712m616c6r	11	5	describing	describe	VERB
5712m616c6r	11	6	u60	u60	ADV
5712m616c6r	11	7	and	and	CCONJ
5712m616c6r	11	8	u24pp12	u24pp12	ADJ
5712m616c6r	11	9	interactions	interaction	NOUN
5712m616c6r	11	10	with	with	ADP
5712m616c6r	11	11	goethite	goethite	NOUN
5712m616c6r	11	12	and	and	CCONJ
5712m616c6r	11	13	hematite	hematite	NOUN
5712m616c6r	11	14	were	be	AUX
5712m616c6r	11	15	determined	determine	VERB
5712m616c6r	11	16	through	through	ADP
5712m616c6r	11	17	the	the	DET
5712m616c6r	11	18	use	use	NOUN
5712m616c6r	11	19	of	of	ADP
5712m616c6r	11	20	a	a	DET
5712m616c6r	11	21	kinetic	kinetic	ADJ
5712m616c6r	11	22	analysis	analysis	NOUN
5712m616c6r	11	23	derived	derive	VERB
5712m616c6r	11	24	as	as	ADP
5712m616c6r	11	25	a	a	DET
5712m616c6r	11	26	part	part	NOUN
5712m616c6r	11	27	of	of	ADP
5712m616c6r	11	28	this	this	DET
5712m616c6r	11	29	work	work	NOUN
5712m616c6r	11	30	.	.	PUNCT
5712m616c6r	12	1	the	the	DET
5712m616c6r	12	2	rate	rate	NOUN
5712m616c6r	12	3	of	of	ADP
5712m616c6r	12	4	uptake	uptake	NOUN
5712m616c6r	12	5	and	and	CCONJ
5712m616c6r	12	6	the	the	DET
5712m616c6r	12	7	amount	amount	NOUN
5712m616c6r	12	8	of	of	ADP
5712m616c6r	12	9	u24pp12	u24pp12	NOUN
5712m616c6r	12	10	removed	remove	VERB
5712m616c6r	12	11	in	in	ADP
5712m616c6r	12	12	systems	system	NOUN
5712m616c6r	12	13	containing	contain	VERB
5712m616c6r	12	14	goethite	goethite	NOUN
5712m616c6r	12	15	was	be	AUX
5712m616c6r	12	16	greater	great	ADJ
5712m616c6r	12	17	than	than	SCONJ
5712m616c6r	12	18	compared	compare	VERB
5712m616c6r	12	19	to	to	ADP
5712m616c6r	12	20	u60	u60	ADJ
5712m616c6r	12	21	.	.	PUNCT
5712m616c6r	13	1	these	these	DET
5712m616c6r	13	2	results	result	NOUN
5712m616c6r	13	3	demonstrate	demonstrate	VERB
5712m616c6r	13	4	that	that	SCONJ
5712m616c6r	13	5	the	the	DET
5712m616c6r	13	6	rate	rate	NOUN
5712m616c6r	13	7	of	of	ADP
5712m616c6r	13	8	uptake	uptake	NOUN
5712m616c6r	13	9	of	of	ADP
5712m616c6r	13	10	particular	particular	ADJ
5712m616c6r	13	11	uranium	uranium	NOUN
5712m616c6r	13	12	nanoclusters	nanocluster	NOUN
5712m616c6r	13	13	may	may	AUX
5712m616c6r	13	14	be	be	AUX
5712m616c6r	13	15	largely	largely	ADV
5712m616c6r	13	16	dependent	dependent	ADJ
5712m616c6r	13	17	on	on	ADP
5712m616c6r	13	18	the	the	DET
5712m616c6r	13	19	charge	charge	NOUN
5712m616c6r	13	20	density	density	NOUN
5712m616c6r	13	21	of	of	ADP
5712m616c6r	13	22	the	the	DET
5712m616c6r	13	23	clusters	cluster	NOUN
5712m616c6r	13	24	as	as	ADV
5712m616c6r	13	25	well	well	ADV
5712m616c6r	13	26	as	as	ADP
5712m616c6r	13	27	the	the	DET
5712m616c6r	13	28	functionality	functionality	NOUN
5712m616c6r	13	29	of	of	ADP
5712m616c6r	13	30	the	the	DET
5712m616c6r	13	31	linkages	linkage	NOUN
5712m616c6r	13	32	connecting	connect	VERB
5712m616c6r	13	33	uranyl	uranyl	ADJ
5712m616c6r	13	34	peroxide	peroxide	NOUN
5712m616c6r	13	35	polyhedral	polyhedral	ADJ
5712m616c6r	13	36	units	unit	NOUN
5712m616c6r	13	37	.	.	PUNCT