id	sid	tid	token	lemma	pos
0c483j34w7d	1	1	condensed	condense	VERB
0c483j34w7d	1	2	phase	phase	NOUN
0c483j34w7d	1	3	charge	charge	NOUN
0c483j34w7d	1	4	transfer	transfer	NOUN
0c483j34w7d	1	5	mechanisms	mechanism	NOUN
0c483j34w7d	1	6	control	control	VERB
0c483j34w7d	1	7	prominent	prominent	ADJ
0c483j34w7d	1	8	reactions	reaction	NOUN
0c483j34w7d	1	9	in	in	ADP
0c483j34w7d	1	10	all	all	DET
0c483j34w7d	1	11	branches	branch	NOUN
0c483j34w7d	1	12	of	of	ADP
0c483j34w7d	1	13	chemistry	chemistry	NOUN
0c483j34w7d	1	14	,	,	PUNCT
0c483j34w7d	1	15	physics	physics	NOUN
0c483j34w7d	1	16	,	,	PUNCT
0c483j34w7d	1	17	and	and	CCONJ
0c483j34w7d	1	18	biology	biology	NOUN
0c483j34w7d	1	19	.	.	PUNCT
0c483j34w7d	2	1	the	the	DET
0c483j34w7d	2	2	prevalence	prevalence	NOUN
0c483j34w7d	2	3	of	of	ADP
0c483j34w7d	2	4	such	such	ADJ
0c483j34w7d	2	5	reactions	reaction	NOUN
0c483j34w7d	2	6	provides	provide	VERB
0c483j34w7d	2	7	great	great	ADJ
0c483j34w7d	2	8	motivation	motivation	NOUN
0c483j34w7d	2	9	to	to	PART
0c483j34w7d	2	10	further	far	ADV
0c483j34w7d	2	11	develop	develop	VERB
0c483j34w7d	2	12	the	the	DET
0c483j34w7d	2	13	methods	method	NOUN
0c483j34w7d	2	14	by	by	ADP
0c483j34w7d	2	15	which	which	PRON
0c483j34w7d	2	16	they	they	PRON
0c483j34w7d	2	17	are	be	AUX
0c483j34w7d	2	18	studied	study	VERB
0c483j34w7d	2	19	computationally	computationally	ADV
0c483j34w7d	2	20	.	.	PUNCT
0c483j34w7d	3	1	the	the	DET
0c483j34w7d	3	2	work	work	NOUN
0c483j34w7d	3	3	that	that	PRON
0c483j34w7d	3	4	follows	follow	VERB
0c483j34w7d	3	5	introduces	introduce	VERB
0c483j34w7d	3	6	a	a	DET
0c483j34w7d	3	7	powerful	powerful	ADJ
0c483j34w7d	3	8	new	new	ADJ
0c483j34w7d	3	9	approach	approach	NOUN
0c483j34w7d	3	10	for	for	ADP
0c483j34w7d	3	11	computer	computer	NOUN
0c483j34w7d	3	12	simulation	simulation	NOUN
0c483j34w7d	3	13	of	of	ADP
0c483j34w7d	3	14	charge	charge	NOUN
0c483j34w7d	3	15	transfer	transfer	NOUN
0c483j34w7d	3	16	processes	process	NOUN
0c483j34w7d	3	17	in	in	ADP
0c483j34w7d	3	18	condensed	condensed	ADJ
0c483j34w7d	3	19	phase	phase	NOUN
0c483j34w7d	3	20	that	that	PRON
0c483j34w7d	3	21	has	have	VERB
0c483j34w7d	3	22	the	the	DET
0c483j34w7d	3	23	potential	potential	NOUN
0c483j34w7d	3	24	to	to	PART
0c483j34w7d	3	25	transform	transform	VERB
0c483j34w7d	3	26	our	our	PRON
0c483j34w7d	3	27	fundamental	fundamental	ADJ
0c483j34w7d	3	28	understanding	understanding	NOUN
0c483j34w7d	3	29	of	of	ADP
0c483j34w7d	3	30	these	these	DET
0c483j34w7d	3	31	reactions	reaction	NOUN
0c483j34w7d	3	32	,	,	PUNCT
0c483j34w7d	3	33	broadly	broadly	ADV
0c483j34w7d	3	34	complementing	complement	VERB
0c483j34w7d	3	35	the	the	DET
0c483j34w7d	3	36	work	work	NOUN
0c483j34w7d	3	37	of	of	ADP
0c483j34w7d	3	38	scientists	scientist	NOUN
0c483j34w7d	3	39	in	in	ADP
0c483j34w7d	3	40	diverse	diverse	ADJ
0c483j34w7d	3	41	disciplines	discipline	NOUN
0c483j34w7d	3	42	.	.	PUNCT
0c483j34w7d	4	1	condensed	condensed	ADJ
0c483j34w7d	4	2	phase	phase	NOUN
0c483j34w7d	4	3	reactions	reaction	NOUN
0c483j34w7d	4	4	evolve	evolve	VERB
0c483j34w7d	4	5	over	over	ADP
0c483j34w7d	4	6	a	a	DET
0c483j34w7d	4	7	rough	rough	ADJ
0c483j34w7d	4	8	potential	potential	ADJ
0c483j34w7d	4	9	energy	energy	NOUN
0c483j34w7d	4	10	surface	surface	NOUN
0c483j34w7d	4	11	,	,	PUNCT
0c483j34w7d	4	12	often	often	ADV
0c483j34w7d	4	13	depending	depend	VERB
0c483j34w7d	4	14	on	on	ADP
0c483j34w7d	4	15	rare	rare	ADJ
0c483j34w7d	4	16	environmental	environmental	ADJ
0c483j34w7d	4	17	fluctuations	fluctuation	NOUN
0c483j34w7d	4	18	to	to	PART
0c483j34w7d	4	19	drive	drive	VERB
0c483j34w7d	4	20	the	the	DET
0c483j34w7d	4	21	reaction	reaction	NOUN
0c483j34w7d	4	22	from	from	ADP
0c483j34w7d	4	23	reactant	reactant	ADJ
0c483j34w7d	4	24	to	to	ADP
0c483j34w7d	4	25	product	product	NOUN
0c483j34w7d	4	26	.	.	PUNCT
0c483j34w7d	5	1	the	the	DET
0c483j34w7d	5	2	expansion	expansion	NOUN
0c483j34w7d	5	3	of	of	ADP
0c483j34w7d	5	4	reaction	reaction	NOUN
0c483j34w7d	5	5	rate	rate	NOUN
0c483j34w7d	5	6	theory	theory	NOUN
0c483j34w7d	5	7	has	have	AUX
0c483j34w7d	5	8	given	give	VERB
0c483j34w7d	5	9	rise	rise	NOUN
0c483j34w7d	5	10	to	to	ADP
0c483j34w7d	5	11	various	various	ADJ
0c483j34w7d	5	12	computational	computational	ADJ
0c483j34w7d	5	13	methods	method	NOUN
0c483j34w7d	5	14	able	able	ADJ
0c483j34w7d	5	15	to	to	PART
0c483j34w7d	5	16	address	address	VERB
0c483j34w7d	5	17	the	the	DET
0c483j34w7d	5	18	difficult	difficult	ADJ
0c483j34w7d	5	19	task	task	NOUN
0c483j34w7d	5	20	of	of	ADP
0c483j34w7d	5	21	sampling	sample	VERB
0c483j34w7d	5	22	an	an	DET
0c483j34w7d	5	23	ensemble	ensemble	NOUN
0c483j34w7d	5	24	of	of	ADP
0c483j34w7d	5	25	rare	rare	ADJ
0c483j34w7d	5	26	reactive	reactive	ADJ
0c483j34w7d	5	27	events	event	NOUN
0c483j34w7d	5	28	.	.	PUNCT
0c483j34w7d	6	1	transition	transition	NOUN
0c483j34w7d	6	2	path	path	NOUN
0c483j34w7d	6	3	sampling	sampling	NOUN
0c483j34w7d	6	4	(	(	PUNCT
0c483j34w7d	6	5	tps	tps	NOUN
0c483j34w7d	6	6	)	)	PUNCT
0c483j34w7d	6	7	is	be	AUX
0c483j34w7d	6	8	one	one	NUM
0c483j34w7d	6	9	such	such	ADJ
0c483j34w7d	6	10	formalism	formalism	NOUN
0c483j34w7d	6	11	.	.	PUNCT
0c483j34w7d	7	1	tps	tps	NOUN
0c483j34w7d	7	2	is	be	AUX
0c483j34w7d	7	3	a	a	DET
0c483j34w7d	7	4	powerful	powerful	ADJ
0c483j34w7d	7	5	statistical	statistical	ADJ
0c483j34w7d	7	6	framework	framework	NOUN
0c483j34w7d	7	7	that	that	PRON
0c483j34w7d	7	8	provides	provide	VERB
0c483j34w7d	7	9	mechanisms	mechanism	NOUN
0c483j34w7d	7	10	of	of	ADP
0c483j34w7d	7	11	complex	complex	ADJ
0c483j34w7d	7	12	reactions	reaction	NOUN
0c483j34w7d	7	13	without	without	ADP
0c483j34w7d	7	14	the	the	DET
0c483j34w7d	7	15	need	need	NOUN
0c483j34w7d	7	16	to	to	PART
0c483j34w7d	7	17	define	define	VERB
0c483j34w7d	7	18	reaction	reaction	NOUN
0c483j34w7d	7	19	coordinates	coordinate	NOUN
0c483j34w7d	7	20	or	or	CCONJ
0c483j34w7d	7	21	identify	identify	VERB
0c483j34w7d	7	22	transition	transition	NOUN
0c483j34w7d	7	23	states	state	NOUN
0c483j34w7d	7	24	a	a	DET
0c483j34w7d	7	25	priori	priori	X
0c483j34w7d	7	26	.	.	PUNCT
0c483j34w7d	8	1	tps	tps	NOUN
0c483j34w7d	8	2	thereby	thereby	ADV
0c483j34w7d	8	3	enables	enable	VERB
0c483j34w7d	8	4	us	we	PRON
0c483j34w7d	8	5	to	to	PART
0c483j34w7d	8	6	study	study	VERB
0c483j34w7d	8	7	a	a	DET
0c483j34w7d	8	8	great	great	ADJ
0c483j34w7d	8	9	variety	variety	NOUN
0c483j34w7d	8	10	of	of	ADP
0c483j34w7d	8	11	problems	problem	NOUN
0c483j34w7d	8	12	for	for	ADP
0c483j34w7d	8	13	which	which	PRON
0c483j34w7d	8	14	this	this	PRON
0c483j34w7d	8	15	would	would	AUX
0c483j34w7d	8	16	be	be	AUX
0c483j34w7d	8	17	daunting	daunting	ADJ
0c483j34w7d	8	18	task	task	NOUN
0c483j34w7d	8	19	.	.	PUNCT
0c483j34w7d	9	1	condensed	condense	VERB
0c483j34w7d	9	2	phase	phase	NOUN
0c483j34w7d	9	3	charge	charge	NOUN
0c483j34w7d	9	4	transfer	transfer	NOUN
0c483j34w7d	9	5	reactions	reaction	NOUN
0c483j34w7d	9	6	present	present	VERB
0c483j34w7d	9	7	an	an	DET
0c483j34w7d	9	8	additional	additional	ADJ
0c483j34w7d	9	9	challenge	challenge	NOUN
0c483j34w7d	9	10	as	as	SCONJ
0c483j34w7d	9	11	these	these	DET
0c483j34w7d	9	12	complex	complex	ADJ
0c483j34w7d	9	13	reactions	reaction	NOUN
0c483j34w7d	9	14	are	be	AUX
0c483j34w7d	9	15	governed	govern	VERB
0c483j34w7d	9	16	by	by	ADP
0c483j34w7d	9	17	explicit	explicit	ADJ
0c483j34w7d	9	18	quantum	quantum	ADJ
0c483j34w7d	9	19	mechanical	mechanical	ADJ
0c483j34w7d	9	20	phenomena	phenomena	NOUN
0c483j34w7d	9	21	.	.	PUNCT
0c483j34w7d	10	1	to	to	PART
0c483j34w7d	10	2	accurately	accurately	ADV
0c483j34w7d	10	3	describe	describe	VERB
0c483j34w7d	10	4	such	such	ADJ
0c483j34w7d	10	5	reactions	reaction	NOUN
0c483j34w7d	10	6	,	,	PUNCT
0c483j34w7d	10	7	one	one	PRON
0c483j34w7d	10	8	must	must	AUX
0c483j34w7d	10	9	consider	consider	VERB
0c483j34w7d	10	10	the	the	DET
0c483j34w7d	10	11	additional	additional	ADJ
0c483j34w7d	10	12	electronic	electronic	ADJ
0c483j34w7d	10	13	and	and	CCONJ
0c483j34w7d	10	14	vibrational	vibrational	ADJ
0c483j34w7d	10	15	energy	energy	NOUN
0c483j34w7d	10	16	states	state	NOUN
0c483j34w7d	10	17	to	to	PART
0c483j34w7d	10	18	which	which	PRON
0c483j34w7d	10	19	the	the	DET
0c483j34w7d	10	20	ground	ground	NOUN
0c483j34w7d	10	21	potential	potential	ADJ
0c483j34w7d	10	22	energy	energy	NOUN
0c483j34w7d	10	23	surface	surface	NOUN
0c483j34w7d	10	24	is	be	AUX
0c483j34w7d	10	25	coupled	couple	VERB
0c483j34w7d	10	26	.	.	PUNCT
0c483j34w7d	11	1	high	high	ADJ
0c483j34w7d	11	2	computational	computational	ADJ
0c483j34w7d	11	3	cost	cost	NOUN
0c483j34w7d	11	4	,	,	PUNCT
0c483j34w7d	11	5	however	however	ADV
0c483j34w7d	11	6	,	,	PUNCT
0c483j34w7d	11	7	limits	limit	VERB
0c483j34w7d	11	8	their	their	PRON
0c483j34w7d	11	9	investigation	investigation	NOUN
0c483j34w7d	11	10	.	.	PUNCT
0c483j34w7d	12	1	mixed	mix	VERB
0c483j34w7d	12	2	quantum	quantum	NOUN
0c483j34w7d	12	3	-	-	PUNCT
0c483j34w7d	12	4	classical	classical	ADJ
0c483j34w7d	12	5	methods	method	NOUN
0c483j34w7d	12	6	alleviate	alleviate	VERB
0c483j34w7d	12	7	some	some	PRON
0c483j34w7d	12	8	of	of	ADP
0c483j34w7d	12	9	this	this	DET
0c483j34w7d	12	10	cost	cost	NOUN
0c483j34w7d	12	11	by	by	ADP
0c483j34w7d	12	12	separating	separate	VERB
0c483j34w7d	12	13	the	the	DET
0c483j34w7d	12	14	degrees	degree	NOUN
0c483j34w7d	12	15	of	of	ADP
0c483j34w7d	12	16	freedom	freedom	NOUN
0c483j34w7d	12	17	containing	contain	VERB
0c483j34w7d	12	18	intrinsic	intrinsic	ADJ
0c483j34w7d	12	19	quantum	quantum	ADJ
0c483j34w7d	12	20	mechanical	mechanical	ADJ
0c483j34w7d	12	21	character	character	NOUN
0c483j34w7d	12	22	from	from	ADP
0c483j34w7d	12	23	those	those	PRON
0c483j34w7d	12	24	that	that	PRON
0c483j34w7d	12	25	can	can	AUX
0c483j34w7d	12	26	be	be	AUX
0c483j34w7d	12	27	treated	treat	VERB
0c483j34w7d	12	28	classically	classically	ADV
0c483j34w7d	12	29	.	.	PUNCT
0c483j34w7d	13	1	among	among	ADP
0c483j34w7d	13	2	many	many	ADJ
0c483j34w7d	13	3	algorithms	algorithm	NOUN
0c483j34w7d	13	4	,	,	PUNCT
0c483j34w7d	13	5	surface	surface	NOUN
0c483j34w7d	13	6	hopping	hopping	NOUN
0c483j34w7d	13	7	methods	method	NOUN
0c483j34w7d	13	8	provide	provide	VERB
0c483j34w7d	13	9	trajectories	trajectory	NOUN
0c483j34w7d	13	10	access	access	NOUN
0c483j34w7d	13	11	to	to	ADP
0c483j34w7d	13	12	these	these	DET
0c483j34w7d	13	13	excited	excited	ADJ
0c483j34w7d	13	14	states	state	NOUN
0c483j34w7d	13	15	via	via	ADP
0c483j34w7d	13	16	nonadiabatic	nonadiabatic	ADJ
0c483j34w7d	13	17	transitions	transition	NOUN
0c483j34w7d	13	18	.	.	PUNCT
0c483j34w7d	14	1	nonadiabatic	nonadiabatic	ADJ
0c483j34w7d	14	2	path	path	NOUN
0c483j34w7d	14	3	sampling	sample	VERB
0c483j34w7d	14	4	(	(	PUNCT
0c483j34w7d	14	5	naps	nap	NOUN
0c483j34w7d	14	6	)	)	PUNCT
0c483j34w7d	14	7	,	,	PUNCT
0c483j34w7d	14	8	seeks	seek	VERB
0c483j34w7d	14	9	to	to	PART
0c483j34w7d	14	10	generalize	generalize	VERB
0c483j34w7d	14	11	the	the	DET
0c483j34w7d	14	12	tps	tps	ADJ
0c483j34w7d	14	13	formalism	formalism	NOUN
0c483j34w7d	14	14	to	to	PART
0c483j34w7d	14	15	accommodate	accommodate	VERB
0c483j34w7d	14	16	reactions	reaction	NOUN
0c483j34w7d	14	17	involving	involve	VERB
0c483j34w7d	14	18	multiple	multiple	ADJ
0c483j34w7d	14	19	electronic	electronic	ADJ
0c483j34w7d	14	20	and	and	CCONJ
0c483j34w7d	14	21	vibrational	vibrational	ADJ
0c483j34w7d	14	22	energy	energy	NOUN
0c483j34w7d	14	23	states	state	NOUN
0c483j34w7d	14	24	.	.	PUNCT
0c483j34w7d	15	1	naps	nap	NOUN
0c483j34w7d	15	2	will	will	AUX
0c483j34w7d	15	3	enhance	enhance	VERB
0c483j34w7d	15	4	our	our	PRON
0c483j34w7d	15	5	understanding	understanding	NOUN
0c483j34w7d	15	6	of	of	ADP
0c483j34w7d	15	7	charge	charge	NOUN
0c483j34w7d	15	8	transfer	transfer	NOUN
0c483j34w7d	15	9	reactions	reaction	NOUN
0c483j34w7d	15	10	in	in	ADP
0c483j34w7d	15	11	the	the	DET
0c483j34w7d	15	12	condensed	condensed	ADJ
0c483j34w7d	15	13	phase	phase	NOUN
0c483j34w7d	15	14	by	by	ADP
0c483j34w7d	15	15	modeling	model	VERB
0c483j34w7d	15	16	reaction	reaction	NOUN
0c483j34w7d	15	17	timescales	timescale	NOUN
0c483j34w7d	15	18	currently	currently	ADV
0c483j34w7d	15	19	beyond	beyond	ADP
0c483j34w7d	15	20	the	the	DET
0c483j34w7d	15	21	scope	scope	NOUN
0c483j34w7d	15	22	of	of	ADP
0c483j34w7d	15	23	molecular	molecular	ADJ
0c483j34w7d	15	24	simulation	simulation	NOUN
0c483j34w7d	15	25	,	,	PUNCT
0c483j34w7d	15	26	and	and	CCONJ
0c483j34w7d	15	27	identifying	identify	VERB
0c483j34w7d	15	28	specific	specific	ADJ
0c483j34w7d	15	29	molecular	molecular	ADJ
0c483j34w7d	15	30	motions	motion	NOUN
0c483j34w7d	15	31	that	that	PRON
0c483j34w7d	15	32	influence	influence	VERB
0c483j34w7d	15	33	or	or	CCONJ
0c483j34w7d	15	34	control	control	VERB
0c483j34w7d	15	35	the	the	DET
0c483j34w7d	15	36	mechanisms	mechanism	NOUN
0c483j34w7d	15	37	and	and	CCONJ
0c483j34w7d	15	38	kinetics	kinetic	NOUN
0c483j34w7d	15	39	of	of	ADP
0c483j34w7d	15	40	charge	charge	NOUN
0c483j34w7d	15	41	transfer	transfer	NOUN
0c483j34w7d	15	42	reactions	reaction	NOUN
0c483j34w7d	15	43	.	.	PUNCT